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arXiv · 2312.09476

Emergence of 6-particle "hexciton'' states in WS$_2$ and MoSe$_2$ monolayers

J. Choi·J. Li·D. Van Tuan·H. Dery·S. A. Crooker
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Abstract

When doped with a high density of mobile charge carriers, monolayer transition-metal dichalcogenide (TMD) semiconductors can host new types of composite many-particle exciton states that do not exist in conventional semiconductors. Such multi-particle bound states arise when a photoexcited electron-hole pair couples to not just a single Fermi sea that is quantum-mechanically distinguishable (as for the case of conventional charged excitons or trions), but rather couples simultaneously to \textit{multiple} Fermi seas, each having distinct spin and valley quantum numbers. Composite six-particle ``hexciton'' states were recently identified in electron-doped WSe$_2$ monolayers, but under suitable conditions they should also form in all other members of the monolayer TMD family. Here we present spectroscopic evidence demonstrating the emergence of many-body hexcitons in charge-tunable WS$_2$ monolayers (at the A-exciton) and MoSe$_2$ monolayers (at the B-exciton). The roles of distinguishability and carrier screening on the stability of hexcitons are discussed.

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J. Choi, J. Li, D. Van Tuan, H. Dery, S. A. Crooker. 2023-12-15. Emergence of 6-particle "hexciton'' states in WS$_2$ and MoSe$_2$ monolayers. https://doi.org/10.1103/physrevb.109.l041304

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