arXiv subjects

J. Choi

Publications and source records attributed to J. Choi.

At least 19 recordsLinked to original sources

arXiv2026

Orbital Separation of Charge Order and Superconductivity in La$_{2-x}$Sr$_{x}$CuO$_4$

We report a combined x-ray absorption (XAS) and oxygen $K$-edge resonant inelastic x-ray scattering (RIXS) study of charge order in underdoped La$_{2-x}$Sr$_x$CuO$_4$ ($x=0.125$) under uniaxial $c$-axis pressure. We find that compressive $c$-axis strain modifies the charge order only within the superconducting state, with a striking polarization dependence: suppression in the $d_{x^2-y^2}$ channel and enhancement in the $d_{z^2}$ channel. X-ray absorption spectra reveal concomitant strain-induced modifications of the oxygen pre-edge and upper Hubbard band, consistent with increased $d_{z^2}$ orbital admixture. Our results suggest that $c$-axis pressure drives an orbital separation between superconductivity, rooted in $d_{x^2-y^2}$ states, and charge order, which gradually shifts to the $d_{z^2}$ channel. This orbital separation reveals a way for superconductivity and charge order to coexist in the cuprates with minimal competition. Furthermore, it suggests that the multi-order phase diagram of La$_{2-x}$Sr$_{x}$CuO$_4$ cannot be realistically described within single band models usually used to describe cuprate physics.

cond-mat.supr-con↗

arXiv2025

Impact of Electron Correlations on Infinite-Layer Cuprates and Nickelates

Optimization of unconventional superconductivity involves a balance of interaction strengths. Precise determination of correlation strength across different material families is therefore important. Here, we present a combined X-ray absorption spectroscopy (XAS) and resonant inelastic X-ray scattering (RIXS) study of infinite-layer PrNiO$_2$ and SrCuO$_2$ that enables fair comparison of their interaction strengths. For both compounds, we study the orbital and magnetic excitations and extract their dispersions along high-symmetry directions. Using a single-band Hubbard model and including higher-order exchange interactions, we derive the correlation factor $U/t$ for both compounds. A key finding is that despite a smaller Coulomb repulsion $U$, PrNiO$_2$ exhibits a correlation strength that is 20% stronger than that of its isostructural cuprate counterpart SrCuO$_2$. This indicates that a moderation of the correlation strength may further optimize superconductivity in nickelates.

cond-mat.supr-con↗

arXiv2025

From Commissioning to Precision Data-Taking: Resolving Operational Challenges in the Nab Detector Systems

Our understanding of the weak mixing of quarks, described by the Cabibbo Kobayashi Maskawa (CKM) matrix, currently presents an anomaly. Thanks to major strides in both theory and experiment, improved precision in determinations of the first row of matrix elements has revealed disagreement with the expectation of unitarity. The Nab experiment at the Spallation Neutron Source is designed to precisely extract the first matrix element $V_{ud}$ and shed light on experimental tensions within the neutron beta decay dataset. Nab's asymmetric spectrometer allows coincident reconstruction of the decay proton and electron energies, which will be used to determine the electron-neutrino correlation coefficient, and thus (with the neutron lifetime) determine $V_{ud}$. This unique approach has provided a more comprehensive view of neutron beta decay, including a first observation of the full momentum phase space of the decay above detector thresholds and limits on exotic neutron states. Recent upgrades to the Nab detector system have improved the robustness and stability of the detector performance in terms of proton detection efficiency, noise performance, and detector segment availability, setting the stage for high precision physics data-taking.

physics.ins-det↗

arXiv2025

Observation of collective charge excitations in a cuprate superconductor

Emergent symmetry breakings in condensed matter systems are often intimately linked to collective excitations. For example, the intertwined spin-charge stripe order in cuprate superconductors is associated with spin and charge excitations. While the collective behavior of spin excitations is well established, the nature of charge excitations remains to be understood. Here we present a high-resolution resonant inelastic x-ray scattering (RIXS) study of charge excitations in the stripe-ordered cuprate La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. The RIXS spectra consist of both charge and phonon excitations around the charge ordering wave vector. By modeling the momentum-dependent phonon intensity, the charge-excitation spectral weight is extracted for a wide range of energy. As such, we reveal the highly dispersive nature of the charge excitations, with an energy scale comparable to the spin excitations. Since charge order and superconductivity in cuprates are possibly driven by the same electronic correlations, determining the interaction strength underlying charge order is essential to establishing a comprehensive microscopic model of high-temperature superconductivity.

cond-mat.supr-con↗

arXiv2025

Dynamic Competition between Cooper-Pair and Spin-Density-Wave Condensation

Quantum matter phases may co-exist microscopically even when they display competing tendencies. A fundamental question is whether such a competition can be avoided through the elimination of one phase while the other one condenses into the ground state. Here, we present a high-resolution neutron spectroscopy study of the low-energy spin excitations in the high-temperature superconductor La1.855Sr0.145CuO4. In the normal state, we find low-energy magnetic fluctuations at incommensurate reciprocal lattice positions where spin-density-wave order emerges at lower Sr concentration or at high magnetic fields. While these spin excitations are largely suppressed by the emergence of the superconducting spin gap, some low-energy magnetic fluctuations persist deep inside the superconducting state. We interpret this result in terms of a dynamic competition between superconductivity and magnetism, where superconductivity impedes the condensation of low-energy magnetic fluctuations through the formation of magnetically-mediated Cooper pairs.

cond-mat.supr-con↗

arXiv2024

Public Quantum Network: The First Node

We present a quantum network that distributes entangled photons between the University of Illinois Urbana-Champaign and a public library in Urbana. The network allows members of the public to perform measurements on the photons. We describe its design and implementation and outreach based on the network. Over 400 instances of public interaction have been logged with the system since it was launched in November 2023.

quant-ph↗

arXiv2024

Decoupling of Static and Dynamic Charge Correlations revealed by Uniaxial Strain in a Cuprate Superconductor

We use uniaxial strain in combination with ultra-high-resolution Resonant Inelastic X-ray Scattering (RIXS) at the oxygen K- and copper L3-edges to study the excitations stemming from the charge ordering wave vector in La1.875Sr0.125CuO4. By detwinning stripe ordering, we demonstrate that the optical phonon anomalies do not show any stripe anisotropy. The low-energy charge excitations also retain an in-plane four-fold symmetry. As such, we find that both phonon and charge excitations are decoupled entirely from the strength of static charge ordering. The almost isotropic character of charge excitations is indicative of a quantum critical behaviour and remains a possible source for the strange metal properties found in the normal state of cuprate superconductors.

cond-mat.str-el↗

arXiv2024

Daily modulations and broadband strategy in axion searches. An application with CAST-CAPP detector

It has been previously advocated that the presence of the daily and annual modulations of the axion flux on the Earth's surface may dramatically change the strategy of the axion searches. The arguments were based on the so-called Axion Quark Nugget (AQN) dark matter model which was originally put forward to explain the similarity of the dark and visible cosmological matter densities $\Omega_{\rm dark}\sim \Omega_{\rm visible}$. In this framework, the population of galactic axions with mass $ 10^{-6} {\rm eV}\lesssim m_a\lesssim 10^{-3}{\rm eV}$ and velocity $\langle v_a\rangle\sim 10^{-3} c$ will be accompanied by axions with typical velocities $\langle v_a\rangle\sim 0.6 c$ emitted by AQNs. Furthermore, in this framework, it has also been argued that the AQN-induced axion daily modulation (in contrast with the conventional WIMP paradigm) could be as large as $(10-20)\%$, which represents the main motivation for the present investigation. We argue that the daily modulations along with the broadband detection strategy can be very useful tools for the discovery of such relativistic axions. The data from the CAST-CAPP detector have been used following such arguments. Unfortunately, due to the dependence of the amplifier chain on temperature-dependent gain drifts and other factors, we could not conclusively show the presence or absence of a dark sector-originated daily modulation. However, this proof of principle analysis procedure can serve as a reference for future studies.

hep-ex↗

arXiv2024

The origin of magnetism in a supposedly nonmagnetic osmium oxide

A supposedly nonmagnetic 5d$^1$ double perosvkite oxide is investigated by a combination of spectroscopic and theoretical methods, namely resonant inelastic X-ray scattering, X-ray absorption spectroscopy, magnetic circular dichroism, and multiplet ligand field calculations. We found that the large spin-orbit coupling admixes the 5d $t_{2g}$ and $e_g$ orbitals, covalency raises the 5d population well above the nominal value, and the local symmetry is lower than $O_h$. The obtained electronic interactions account for the finite magnetic moment of Os in this compound and, in general, of 5d$^1$ ions. Our results provide direct evidence of elusive Jahn-Teller distortions, hinting at a strong electron-lattice coupling.

cond-mat.str-el↗

arXiv2023

Universal orbital and magnetic structures in infinite-layer nickelates

We conducted a comparative study of the rare-earth infinite-layer nickelates films, RNiO2 (R = La, Pr, and Nd) using resonant inelastic X-ray scattering (RIXS). We found that the gross features of the orbital configurations are essentially the same, with minor variations in the detailed hybridization. For low-energy excitations, we unambiguously confirm the presence of damped magnetic excitations in all three compounds. By fitting to a linear spin-wave theory, comparable spin exchange coupling strengths and damping coefficients are extracted, indicating a universal magnetic structure in the infinite-layer nickelates. Interestingly, while signatures of a charge order are observed in LaNiO2 in the quasi-elastic region of the RIXS spectrum, it is absent in NdNiO2 and PrNiO2. This prompts further investigation into the universality and the origins of charge order within the infinite-layer inickelates.

cond-mat.str-el↗

arXiv2023

Emergence of 6-particle "hexciton'' states in WS$_2$ and MoSe$_2$ monolayers

When doped with a high density of mobile charge carriers, monolayer transition-metal dichalcogenide (TMD) semiconductors can host new types of composite many-particle exciton states that do not exist in conventional semiconductors. Such multi-particle bound states arise when a photoexcited electron-hole pair couples to not just a single Fermi sea that is quantum-mechanically distinguishable (as for the case of conventional charged excitons or trions), but rather couples simultaneously to \textit{multiple} Fermi seas, each having distinct spin and valley quantum numbers. Composite six-particle ``hexciton'' states were recently identified in electron-doped WSe$_2$ monolayers, but under suitable conditions they should also form in all other members of the monolayer TMD family. Here we present spectroscopic evidence demonstrating the emergence of many-body hexcitons in charge-tunable WS$_2$ monolayers (at the A-exciton) and MoSe$_2$ monolayers (at the B-exciton). The roles of distinguishability and carrier screening on the stability of hexcitons are discussed.

cond-mat.mes-hall↗

arXiv2023

Resolving the Orbital Character of Low-energy Excitations in Mott Insulator with Intermediate Spin-orbit Coupling

Multi-band Mott insulators with moderate spin-orbit and Hund's coupling are key reference points for theoretical concept developments of correlated electron systems. The ruthenate Mott insulator Ca$_{2}$RuO$_{4}$ has therefore been intensively studied by spectroscopic probes. However, it has been challenging to resolve the fundamental excitations emerging from the hierarchy of electronic energy scales. Here we apply state-of-the-art resonant inelastic x-ray scattering to probe deeper into the electronic excitations found in Ca$_{2}$RuO$_{4}$. In this fashion, we probe a series of spin-orbital excitations at low energies and resolve the level splitting of the intra-$t_{2g}$ structure due to spin-orbit coupling and crystal field splitting. Most importantly, the low-energy excitations exhibit strong orbital character. Such direct determination of relevant electronic energy scales is important, as it sharpens the target for theory developments of Mott insulators' orbital degree of freedom.

cond-mat.str-el↗

arXiv2023

Engineering Phase Competition Between Stripe Order and Superconductivity in La$_{1.88}$Sr$_{0.12}$CuO$_4$

Unconventional superconductivity often couples to other electronic orders in a cooperative or competing fashion. Identifying external stimuli that tune between these two limits is of fundamental interest. Here, we show that strain perpendicular to the copper-oxide planes couples directly to the competing interaction between charge stripe order and superconductivity in La$_{1.88}$Sr$_{0.12}$CuO$_4$ (LSCO). Compressive $c$-axis pressure amplifies stripe order within the superconducting state, while having no impact on the normal state. By contrast, strain dramatically diminishes the magnetic field enhancement of stripe order in the superconducting state. These results suggest that $c$-axis strain acts as tuning parameter of the competing interaction between charge stripe order and superconductivity. This interpretation implies a uniaxial pressure-induced ground state in which the competition between charge order and superconductivity is reduced.

cond-mat.str-el↗

arXiv2023

Strain-Tuned Magnetic Frustration in a Square Lattice $J_1$-$J_2$ Material

Magnetic frustration is a route that can lead to the emergence of novel ground states, including spin liquids and spin ices. Such frustration can be introduced through either the geometry of lattice structures or by incompatible exchange interactions. Identifying suitable strategies to control the degree of magnetic frustration in real systems is an active field of research. In this study, we devise a design principle for the tuning of frustrated magnetism on the square lattice through the manipulation of nearest (NN) and next-nearest neighbor (NNN) antiferromagnetic (AF) exchange interactions. By studying the magnon excitations in epitaxially-strained La$_2$NiO$_4$ films using resonant inelastic x-ray scattering (RIXS) we show that, in contrast to the cuprates, the dispersion peaks at the AF zone boundary. This indicates the presence of an AF-NNN spin interaction. Using first principles simulations and an effective spin-model, we demonstrate the AF-NNN coupling to be a consequence of the two-orbital nature of La$_2$NiO$_4$. Our results demonstrate that compressive strain can enhance this coupling, providing a design principle for the tunability of frustrated magnetism on a square lattice.

cond-mat.str-el↗

arXiv2023

Machine Learning based tool for CMS RPC currents quality monitoring

The muon system of the CERN Compact Muon Solenoid (CMS) experiment includes more than a thousand Resistive Plate Chambers (RPC). They are gaseous detectors operated in the hostile environment of the CMS underground cavern on the Large Hadron Collider where pp luminosities of up to $2\times 10^{34}$ $\text{cm}^{-2}\text{s}^{-1}$ are routinely achieved. The CMS RPC system performance is constantly monitored and the detector is regularly maintained to ensure stable operation. The main monitorable characteristics are dark current, efficiency for muon detection, noise rate etc. Herein we describe an automated tool for CMS RPC current monitoring which uses Machine Learning techniques. We further elaborate on the dedicated generalized linear model proposed already and add autoencoder models for self-consistent predictions as well as hybrid models to allow for RPC current predictions in a distant future.

physics.ins-det↗

arXiv2023

Low-energy quasi-circular electron correlations with charge order wavelength in $\textrm{Bi}_2\textrm{Sr}_2\textrm{Ca}\textrm{Cu}_2\textrm{O}_{8+\delta}$

In the study of dynamic charge order correlations in the cuprates, most high energy-resolution resonant inelastic x-ray scattering (RIXS) measurements have focused on momenta along the high-symmetry directions of the copper oxide plane. However, electron scattering along other in-plane directions should not be neglected as they may contain information relevant, for example, to the origin of charge order correlations or to our understanding of the isotropic scattering responsible for strange metal behavior in cuprates. We report high-resolution resonant inelastic x-ray scattering (RIXS) experiments that reveal the presence of dynamic electron correlations over the $q_x$-$q_y$ scattering plane in underdoped $\textrm{Bi}_2\textrm{Sr}_2\textrm{Ca}\textrm{Cu}_2\textrm{O}_{8+\delta}$ with $T_c=54$ K. We use the softening of the RIXS-measured bond stretching phonon line as a marker for the presence of charge-order-related dynamic electron correlations. The experiments show that these dynamic correlations exist at energies below approximately $70$ meV and are centered around a quasi-circular manifold in the $q_x$-$q_y$ scattering plane with radius equal to the magnitude of the charge order wave vector, $q_{CO}$. We also demonstrate how this phonon-tracking procedure provides the necessary experimental precision to rule out fluctuations of short-range directional charge order (i.e. centered around $[q_x=\pm q_{CO}, q_y=0]$ and $[q_x=0, q_y=\pm q_{CO}]$) as the origin of the observed correlations.

cond-mat.str-el↗

arXiv2022

RPC based tracking system at CERN GIF++ facility

With the HL-LHC upgrade of the LHC machine, an increase of the instantaneous luminosity by a factor of five is expected and the current detection systems need to be validated for such working conditions to ensure stable data taking. At the CERN Gamma Irradiation Facility (GIF++) many muon detectors undergo such studies, but the high gamma background can pose a challenge to the muon trigger system which is exposed to many fake hits from the gamma background. A tracking system using RPCs is implemented to clean the fake hits, taking profit of the high muon efficiency of these chambers. This work will present the tracking system configuration, used detector analysis algorithm and results.

physics.ins-det↗

arXiv2022

Search for Dark Matter Axions with CAST-CAPP

The CAST-CAPP axion haloscope, operating at CERN inside the CAST dipole magnet, has searched for axions in the 19.74 $\mu$eV to 22.47 $\mu$eV mass range. The detection concept follows the Sikivie haloscope principle, where Dark Matter axions convert into photons within a resonator immersed in a magnetic field. The CAST-CAPP resonator is an array of four individual rectangular cavities inserted in a strong dipole magnet, phase-matched to maximize the detection sensitivity. Here we report on the data acquired for 4124 h from 2019 to 2021. Each cavity is equipped with a fast frequency tuning mechanism of 10 MHz/min between 4.774 GHz and 5.434 GHz. In the present work, we exclude axion-photon couplings for virialized galactic axions down to $g_{a{\gamma}{\gamma}} = 8 \times {10^{-14}}$ $GeV^{-1}$ at the 90% confidence level. The here implemented phase-matching technique also allows for future large-scale upgrades.

hep-ex↗