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arXiv · 2402.04106

Hybrid moir\'e excitons and trions in twisted MoTe$_2$-MoSe$_2$ heterobilayers

Shen Zhao·Xin Huang·Roland Gillen·Zhijie Li·Song Liu·Kenji Watanabe·Takashi Taniguchi·Janina Maultzsch·James Hone·Alexander Högele·Anvar S. Baimuratov
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Abstract

We report experimental and theoretical studies of MoTe$_2$-MoSe$_2$ heterobilayers with rigid moir\'e superlattices controlled by the twist angle. Using an effective continuum model that combines resonant interlayer electron tunneling with stacking-dependent moir\'e potentials, we identify the nature of moir\'e excitons and the dependence of their energies, oscillator strengths and Land\'e $g$-factors on the twist angle. Within the same framework, we interpret distinct signatures of bound complexes among electrons and moir\'e excitons in nearly collinear heterostacks. Our work provides fundamental understanding of hybrid moir\'e excitons and trions in MoTe$_2$-MoSe$_2$ heterobilayers, and establishes the material system as a prime candidate for optical studies of correlated phenomena in moir\'e lattices.

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Shen Zhao, Xin Huang, Roland Gillen, Zhijie Li, Song Liu, Kenji Watanabe, Takashi Taniguchi, Janina Maultzsch, James Hone, Alexander Högele, Anvar S. Baimuratov. 2024-02-06. Hybrid moir\'e excitons and trions in twisted MoTe$_2$-MoSe$_2$ heterobilayers. https://doi.org/10.1021/acs.nanolett.4c00541

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