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arXiv · 2403.09424

Inelastic neutron scattering and muon spin relaxation investigations of the deuterated Kondo lattices CeNiSnD$ _x $

X. Y. Zheng·D. T. Adroja·B. Chevalier·Z. Y. Shan·A. D. Hillier·H. Q. Yuan·M. Smidman
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Abstract

CeNiSn is a Kondo semimetal where a gap opens at low temperatures due to hybridization between 4$f$ and conduction electrons, but a full insulating state fails to develop. Upon the insertion of hydrogen, long range magnetic order is induced. Here we report zero-field muon-spin relaxation and inelastic neutron scattering measurements of polycrystalline samples of the deuterides CeNiSnD$_x$ ($x$=1.0, 1.8). The muon-spin relaxation results confirm magnetic ordering in the whole sample of CeNiSnD below around 4.7 K, while inelastic neutron scattering reveals two well-defined crystalline-electric field (CEF) excitations at around 13 meV and 34 meV in CeNiSnD, and 5 meV and 27 meV for CeNiSnD$_{1.8}$. These results suggest that hydrogenation leads to the localization of the Ce-4$f$ electrons, giving rise to long-range magnetic order. We propose CEF level schemes for both systems, which predict a ground state moment of 0.96$\mu_{\rm B}$/Ce within the $ab$-plane for CeNiSnD$_{1.8}$ and a saturated moment of 1.26$\mu_{\rm B}$/Ce along the easy $c$ axis for CeNiSnD, that account for the observed magnetic properties.

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X. Y. Zheng, D. T. Adroja, B. Chevalier, Z. Y. Shan, A. D. Hillier, H. Q. Yuan, M. Smidman. 2024-03-14. Inelastic neutron scattering and muon spin relaxation investigations of the deuterated Kondo lattices CeNiSnD$ _x $. https://doi.org/10.1103/physrevb.109.064401

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