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arXiv · 2403.10028

Nonmagnetic Ground State in RuO$_2$ Revealed by Muon Spin Rotation

M. Hiraishi·H. Okabe·A. Koda·R. Kadono·T. Muroi·D. Hirai·Z. Hiroi
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Abstract

The magnetic ground state of single crystalline RuO$_2$ was investigated by the muon spin rotation/relaxation ($\mu$SR) experiment. The spin precession signal due to the spontaneous internal magnetic field $B_{\rm loc}$, which is expected in the magnetically ordered phase, was not observed in the temperature range 5--400~K. Muon sites were evaluated by first-principles calculations using dilute hydrogen simulating muon as pseudo-hydrogen, and $B_{\rm loc}$ was simulated for the antiferromagnetic (AFM) structures with a Ru magnetic moment $|{\bf m}_{\rm Ru}|\approx0.05\mu_\mathrm{B}$ suggested from diffraction experiments. As a result, the possibility was ruled out that muons are localized at sites where $B_{\rm loc}$ accidentally cancels. Conversely, assuming that the slow relaxation observed in $\mu$SR spectra was part of the precession signal, the upper limit for the magnitude of $|{\bf m}_{\rm Ru}|$ was estimated to be $4.8(2)\times10^{-4}\mu_{\rm B}$, which is significantly less than $0.05\mu_\mathrm{B}$. These results indicate that the AFM order, as reported, is unlikely to exist in the bulk crystal.

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M. Hiraishi, H. Okabe, A. Koda, R. Kadono, T. Muroi, D. Hirai, Z. Hiroi. 2024-03-15. Nonmagnetic Ground State in RuO$_2$ Revealed by Muon Spin Rotation. https://doi.org/10.1103/physrevlett.132.166702

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