Final results of the measurement to search for rare decays of naturally occurring osmium isotopes with ultra-low background gamma-ray spectrometry

Abstract

A long-term measurement was conducted to search for $\alpha$, double-$\alpha$ and double-$\beta$ decays with $\gamma$ quanta emission in naturally occurring osmium isotopes. This study took advantage of two ultra-low background HPGe detectors and one ultra-low background BEGe detector at the Gran Sasso National Laboratory (LNGS) of the INFN. Over almost 5 years of data were taken using high-purity osmium samples of approximately 173 g. The half-life limits set for a decays of $^{184}$Os to the first $2^+$ 103.6 keV excited level of $^{180}$W ($T_{1/2} > 9.3 \times 10^{15}$ yr) and of $^{186}$Os to the first $2^+$ 100.1 keV of $^{182}$W ($T_{1/2} > 4.8 \times 10^{17}$ yr) exceed substantially the present theoretical predictions that are at level of $T_{1/2} \sim (0.6 - 3) \times 10^{15}$ yr for $^{184}$Os and $T_{1/2} \sim (0.3 - 2) \times 10^{17}$ yr for $^{186}$Os. New half-life limits on the 2EC and EC$\beta^+$ decay of $^{184}$Os to the ground and excited levels of $^{184}$W were set at level of $T_{1/2} > 10^{16} - 10^{17}$ yr; a lower limit on the $2\beta^-$ decay of $^{192}$Os to the $2^+$ 316.5 keV excited level of $^{192}$Pt was estimated as $T_{1/2} > 6.1 \times 10^{20}$ yr. The half-life limits for $2\alpha$ decay of $^{189}$Os and $^{192}$Os were set for the first time at level of $T_{1/2} > 10^{20}$ yr.