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arXiv · 2410.18547

Beyond Electric-Dipole Treatment of Light-Matter Interactions in Materials: Nondipole Harmonic Generation in Bulk Si

Simon Vendelbo Bylling Jensen·Nicolas Tancogne-Dejean·Angel Rubio·Lars Bojer Madsen
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Abstract

A beyond electric-dipole light-matter theory is needed to describe emerging X-ray and THz applications for characterization and control of quantum materials but inaccessible as nondipole lattice-aperiodic terms impede on the use of Bloch's theorem. To circumvent this, we derive a formalism that captures dominant nondipole effects in intense electromagnetic fields while conserving lattice translational symmetry. Our approach enables the first accurate nondipole first-principles microscopic simulation of nonperturbative harmonic generation in Si. We reveal nondipole-induced transverse currents generating perturbative even-ordered harmonics and display the onset of nondipole high harmonic generation near the laser damage threshold.

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Simon Vendelbo Bylling Jensen, Nicolas Tancogne-Dejean, Angel Rubio, Lars Bojer Madsen. 2024-10-24. Beyond Electric-Dipole Treatment of Light-Matter Interactions in Materials: Nondipole Harmonic Generation in Bulk Si. https://doi.org/10.1103/physrevlett.134.196902

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