Interplay of Kondo Physics with Incommensurate Charge Density Waves in CeTe$_3$

Aymeric Saunot; Vesna Miksic Trontl; Ilya I. Klimovskikh; Denis V. Vyalikh; Alex Louat; Cephise Cacho; Asish K. Kumar; Elio Vescovo; Ivana Vobornik; Alexander Fedorov; Cedomir Petrovic; Tonica Valla

doi:10.1063/5.0313165

arXiv · 2502.04814

Interplay of Kondo Physics with Incommensurate Charge Density Waves in CeTe$_3$

Aymeric Saunot·Vesna Miksic Trontl·Ilya I. Klimovskikh·Denis V. Vyalikh·Alex Louat·Cephise Cacho·Asish K. Kumar·Elio Vescovo·Ivana Vobornik·Alexander Fedorov·Cedomir Petrovic·Tonica Valla

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Abstract

CeTe$_3$ is a 2--dimensional (2D) Van der Waals (VdW) material with incommensurate charge density waves (CDW), extremely high transition temperature ($T_{CDW}$) and a large momentum--dependent CDW gap that leaves a significant portion of the Fermi surface intact. It is also considered to be a weak Kondo system, a property unexpected for a material with incommensurate CDW, where each atomic site is slightly different. Here, we study the properties of the CDW state in several RTe$_3$ (R is rare earth) materials and examine the hybridization of itinerant states with the localized Ce $4f$ multiplet in CeTe$_3$ by using angle resolved photoemission spectroscopy (ARPES). We find that the renormalization of the itinerant states originating from the hybridization with the deeper localized $4f$ states at $-260$ meV is $k-$dependent and extends to the Fermi level. As these localized states are far from the Fermi level, the observed hybridization affects the effective masses only marginally and does not lead to heavy fermions. However, since the same renormalizing mechanism normally leads to the heavy fermion physics when the localized $4f$ states are near the Fermi level, our observation of its strong $k-$dependence suggests that this could be the reason for discrepancy between the heavy masses in specific heat and light ones in Shubnikov de Haas oscillations, often observed in heavy fermions.

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Aymeric Saunot, Vesna Miksic Trontl, Ilya I. Klimovskikh, Denis V. Vyalikh, Alex Louat, Cephise Cacho, Asish K. Kumar, Elio Vescovo, Ivana Vobornik, Alexander Fedorov, Cedomir Petrovic, Tonica Valla. 2025-02-07. Interplay of Kondo Physics with Incommensurate Charge Density Waves in CeTe$_3$. https://doi.org/10.1063/5.0313165

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