Observation of collective charge excitations in a cuprate superconductor

Abstract

Emergent symmetry breakings in condensed matter systems are often intimately linked to collective excitations. For example, the intertwined spin-charge stripe order in cuprate superconductors is associated with spin and charge excitations. While the collective behavior of spin excitations is well established, the nature of charge excitations remains to be understood. Here we present a high-resolution resonant inelastic x-ray scattering (RIXS) study of charge excitations in the stripe-ordered cuprate La$_{1.675}$Eu$_{0.2}$Sr$_{0.125}$CuO$_4$. The RIXS spectra consist of both charge and phonon excitations around the charge ordering wave vector. By modeling the momentum-dependent phonon intensity, the charge-excitation spectral weight is extracted for a wide range of energy. As such, we reveal the highly dispersive nature of the charge excitations, with an energy scale comparable to the spin excitations. Since charge order and superconductivity in cuprates are possibly driven by the same electronic correlations, determining the interaction strength underlying charge order is essential to establishing a comprehensive microscopic model of high-temperature superconductivity.