Discovery of spontaneous mesoscopic strain waves in nematic domains using dark-field X-ray microscopy

Abstract

Electronic nematic order is a correlated phase of matter in which low-energy electronic states spontaneously break a discrete rotational symmetry of a crystal lattice. Bilinear coupling between the electronic nematic and strains of the same symmetry yields a single pseudoproper ferroelastic phase transition at which both the nematic and lattice strain onset concurrently. To minimize elastic energy, the crystal forms structural twin domains, each with a distinct orientation of the nematic director (i.e. each with a specific sign of the induced shear strain). While the effects of externally induced strains on these domains are well established, the intrinsic behavior of spontaneous strain fields within individual domains has been hitherto unexplored, largely due to the lack of appropriate experimental tools. Here, we report the discovery of spontaneous mesoscopic strain waves within individual nematic domains of an underdoped iron-based superconductor, observed using dark-field X-ray microscopy (DFXM). This technique combines high spatial and reciprocal-space resolution with full-field, bulk-sensitive imaging, enabling direct visualization of subdomain strain modulations emerging concurrently with the onset of nematic order. The elastic compatibility relations that govern inhomogeneous strains in continuous solids provide a natural mechanism for the emergent strain waves that we observe. Our findings reveal a broadly relevant form of strain self-organization and position DFXM as a powerful tool for probing the local interplay between lattice strain and electronic order.