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arXiv · 2509.03583

Magic continuum in multi-moir\'e twisted trilayer graphene

Abstract

Moir\'e lattices provide a highly tunable platform for exploring the interplay between electronic correlations and band topology. Introducing a second moir\'e pattern extends this paradigm: interference between the two moir\'e patterns produces a supermoir\'e modulation, opening a route to further tailor electronic properties. Twisted trilayer graphene generally exemplifies such a system: two distinct moir\'e patterns arise from the relative twists between adjacent graphene layers. Here, we report the observation of correlated phenomena across a wide range of twisted trilayer graphene devices whose twist angles lie along two continuous lines in the twist-angle parameter space. Depending on the degree of lattice relaxation, twisted trilayer graphene falls into two classes: moir\'e polycrystals, composed of periodic domains with locally commensurate moir\'e order, and moir\'e quasicrystals, characterized by smoothly varying local moir\'e configurations. In helically twisted moir\'e polycrystals, we observe an anomalous Hall effect, consistent with topological bands arising from domains with broken $xy$-inversion symmetry. In contrast, superconductivity appears generically in our moir\'e quasicrystals. A subset of these systems exhibits signatures of spatially modulated superconductivity, which we attribute to the supermoir\'e structure. Our findings uncover the organizing principles of the observed correlated phases in twisted trilayer graphene, highlight the critical roles of the supermoir\'e modulation and lattice relaxation, and suggest a broader framework in which magic conditions arise not as isolated points but as extended manifolds within the multi-dimensional twist-angle space of complex moir\'e materials.

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Li-Qiao Xia, Aviram Uri, Jiaojie Yan, Aaron Sharpe, Filippo Gaggioli, Nicole S. Ticea, Julian May-Mann, Kenji Watanabe, Takashi Taniguchi, Liang Fu, Trithep Devakul, Jurgen H. Smet, Pablo Jarillo-Herrero. 2025-09-03. Magic continuum in multi-moir\'e twisted trilayer graphene. https://arxiv.org/abs/2509.03583

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