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Aaron Sharpe

Publications and source records attributed to Aaron Sharpe.

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Quantized Transport through a Supermoir\'e Chern Mosaic

Magic-angle helical trilayer graphene---three graphene layers sequentially twisted in the same direction by $\sim1.8^\circ$---relaxes into a mosaic of domains that, at zero field, carry opposite valley-resolved Chern numbers, with boundaries hosting a network of gapless conducting modes. Charge transport through this network depends sensitively on how the modes connect and scatter, making well-quantized transport unlikely. Contrary to this expectation, we observe a field-induced Chern gap with Chern number $C=-6$ emanating from charge neutrality; in this gap, the Hall resistance is quantized to within $2\%$ of the expected value, $-h/6e^2$, at 4.6 K. We explain this behavior using both Hofstadter and orbital Zeeman calculations, which show that a moderate magnetic field drives a valley-selective topological transition. Above the transition, the total Chern number of the occupied states in each spin-valley flavor becomes identical across neighboring domains, and the domain-wall modes can become gapped. Though the central valence-band Chern numbers still differ between the two domain types, the observed quantized transport attests to a global gap.

cond-mat.mes-hall

Fermiology and the Candidate Chiral Superconductor in Rhombohedral Tetralayer Graphene

Chiral superconductivity, in which the phase of the superconducting order parameter winds in momentum space, has long been sought for its close link to topological superconductivity. Recent work reported a superconductor in rhombohedral multilayer graphene emerging from a time-reversal symmetry broken normal state, suggesting that it could be a chiral superconductor. However, the possibility of chirality depends on the symmetry and structure of the normal-state Fermi surface, which have not been directly measured. Here we measure quantum oscillations in rhombohedral tetralayer graphene over a broad range of the phase diagram, including the superconducting region. At densities well above the onset of superconductivity, we reproduce previously-reported oscillations consistent with a spin- and valley-polarized quarter metal with a single simply-connected Fermi pocket. As the carrier density is reduced, we find a transition to a complex "multitone" state that persists through the superconducting region. This state's spectrum of quantum oscillations is incompatible with a simply-connected quarter metal. The next-simplest candidate normal states suggested by our microscopic modeling (fully-polarized annular, nematic, and three-pocket states) are inconsistent with our measurements, albeit difficult to rule out entirely. The normal state is thus seen to be richer than previously envisaged, reshaping the search for the superconducting mechanism and the possible chirality of the pairing channel.

cond-mat.supr-con

Visualizing orbital magnetism in electron doped rhombohedral multilayer graphene

Electron doped rhombohedral multilayer graphene at high displacement field features an exceptionally flat band minimum with near-ideal quantum geometry. Experiments in this regime observe the formation of a 'quarter metal,' in which the electron liquid condenses into a single spin- and valley flavor. Remarkably, recent experiments have found a zero resistance state in the same region of the density- and displacement-field-tuned parameter space, attributed to the formation of a chiral superconductor from an orbitally ferromagnetic normal state. Here, we use nanoSQUID-on-tip magnetometry to map the orbital magnetization of electron-doped rhombohedral graphene devices ranging in thickness between 3 and 15 layers. Magnetization within the quarter metal phases peaks at finite density, consistent with concentration of the Berry curvature in a finite-momentum 'ring of fire'. Correlating transport and local magnetometry data in a superconducting tetralayer sample reveals a finite orbital ferromagnetic moment, providing direct evidence of valley polarization in the superconducting ground state. We further show that widely observed stochastic switching of the resistivity in both metallic and superconducting regimes arises from a density-tuned sign change in the valley-resolved total magnetic moment. This leads to the formation of metastable magnetic domains under typical gate control sequences and can also be harnessed for electric-field controlled switching of the magnetization across the entire device. Finally, high resolution measurements of the magnetization across a superconducting transition allow us to put an upper bound on the 'condensation magnetization' of 0.1 Bohr magneton per carrier, placing a strong quantitative restriction on theoretical models for ferromagnetic superconductivity.

cond-mat.mes-hall

Mesoscopic transport in a Chern mosaic

We analyze mesoscopic electronic transport in a Chern mosaic: a regular pattern of domains whose electronic bands carry differing local Chern numbers. An example platform where a Chern mosaic can arise is a moir\'e heterostructure, where variations in the local moir\'e parameters can produce such domains. We compute resistances at linear response for a variety of domain wall network geometries at zero temperature and magnetic field. Simple domain configurations can exhibit zero, integer, or fractional multiples of the quantum of resistance in both the longitudinal and transverse (Hall) responses. Our simple semi-classical analysis provides a useful computational method and comparative catalog for ongoing experiments in two-dimensional topological materials.

cond-mat.mes-hall

Electrically controllable valence-conduction band reversals in helical trilayer graphene

In moir\'e graphene systems, electronic interactions lift spin and valley degeneracies, leading to symmetry-broken ground states. In helical trilayer graphene (HTG), we uncover a distinct interaction-driven mechanism in which the roles of sublattice-polarized valence and conduction bands are cyclically reversed. Using scanning nano-SQUID magnetometry, we detect a series of sharp magnetic signatures consistent with seesaw-like transitions, where occupied and unoccupied valence and conduction bands interchange repeatedly with doping, accompanied by a novel form of magnetic hysteresis. These transitions occur entirely within metallic regimes and leave only weak fingerprints in transport measurements. Self-consistent Hartree-Fock calculations reveal that interactions reorganize all eight low-energy flat bands, driving abrupt changes in orbital magnetization. Our results establish HTG as the first system where electronic interactions provide doping-controlled access to all three internal degrees of freedom - spin, valley, and sublattice - introducing a new class of correlated phase transitions.

cond-mat.mes-hall

Link between thermodynamic correlation signatures and superconductivity in twisted trilayer graphene

Twisted graphene multilayers exhibit strong electronic correlations, which manifest in a range of experimental signatures. Yet how these signatures relate to each other and the microscopic ground states-and how twist angle and band structure reshape them-remains poorly understood. Here we study this interplay by correlating local thermodynamic and transport measurements in a twisted trilayer graphene (TTG) sample with unequal angles and flat electronic bands. We use a scanning single-electron transistor to map the impact of electron-electron interactions in a region of the sample where the local twist angle evolves smoothly. We observe gapped correlated insulators and a sawtooth in electronic compressibility, both exhibiting pronounced electron-hole (e-h) asymmetry with distinct magic angles for conduction and valence bands. Subsequent transport measurements in the same region reveal robust superconductivity with a similar e-h asymmetry. Our measurements indicate that superconductivity is not directly tied to the correlated insulators. Instead, its critical temperature correlates closely with the strength of the sawtooth in compressibility, suggesting a common origin or link between the two. By combining a local probe with transport measurements, we uncover connections between superconductivity and thermodynamic correlation signatures that are not apparent from either technique in isolation, highlighting the power of our dual approach and establishing their dependence on interlayer twist angles in TTG.

cond-mat.mes-hall

Magic continuum in multi-moir\'e twisted trilayer graphene

Moir\'e lattices provide a highly tunable platform for exploring the interplay between electronic correlations and band topology. Introducing a second moir\'e pattern extends this paradigm: interference between the two moir\'e patterns produces a supermoir\'e modulation, opening a route to further tailor electronic properties. Twisted trilayer graphene generally exemplifies such a system: two distinct moir\'e patterns arise from the relative twists between adjacent graphene layers. Here, we report the observation of correlated phenomena across a wide range of twisted trilayer graphene devices whose twist angles lie along two continuous lines in the twist-angle parameter space. Depending on the degree of lattice relaxation, twisted trilayer graphene falls into two classes: moir\'e polycrystals, composed of periodic domains with locally commensurate moir\'e order, and moir\'e quasicrystals, characterized by smoothly varying local moir\'e configurations. In helically twisted moir\'e polycrystals, we observe an anomalous Hall effect, consistent with topological bands arising from domains with broken $xy$-inversion symmetry. In contrast, superconductivity appears generically in our moir\'e quasicrystals. A subset of these systems exhibits signatures of spatially modulated superconductivity, which we attribute to the supermoir\'e structure. Our findings uncover the organizing principles of the observed correlated phases in twisted trilayer graphene, highlight the critical roles of the supermoir\'e modulation and lattice relaxation, and suggest a broader framework in which magic conditions arise not as isolated points but as extended manifolds within the multi-dimensional twist-angle space of complex moir\'e materials.

cond-mat.mes-hall

Directional ballistic magnetotransport in the delafossite metals PdCoO$_2$ and PtCoO$_2$

Studies of electronic transport in width-restricted channels of PdCoO$_2$ have recently revealed a novel `directional ballistic' regime, in which ballistic propagation of electrons on an anisotropic Fermi surface breaks the symmetries of bulk transport. Here we introduce a magnetic field to this regime, in channels of PdCoO$_2$ and PtCoO$_2$ along two crystallographically distinct directions and over a wide range of widths. We observe magnetoresistance distinct from that in the bulk, with features strongly dependent on channel orientation and becoming more pronounced the narrower the channel. Comparison to semi-classical theory establishes that magnetoresistance arises from field-induced modification of boundary scattering, and helps connect features in the data with specific electronic trajectories. However, the role of bulk scattering in our measurements is yet to be fully understood. Our results demonstrate that finite-size magnetotransport is sensitive to the anisotropy of Fermi surface properties, motivating future work to fully understand and exploit this sensitivity.

cond-mat.mes-hall

Helical trilayer graphene: a moir\'e platform for strongly-interacting topological bands

Quantum geometry of electronic wavefunctions results in fascinating topological phenomena. A prominent example is the intrinsic anomalous Hall effect (AHE) in which a Hall voltage arises in the absence of an applied magnetic field. The AHE requires a coexistence of Berry curvature and spontaneous time-reversal symmetry breaking. These conditions can be realized in two-dimensional moir\'e systems with broken $xy$-inversion symmetry ($C_{2z}$) that host flat electronic bands. Here, we explore helical trilayer graphene (HTG), three graphene layers twisted sequentially by the same angle forming two misoriented moir\'e patterns. Although HTG is globally $C_{2z}$-symmetric, surprisingly we observe clear signatures of topological bands. At a magic angle $\theta_\mathrm{m}\approx 1.8^\circ$, we uncover a robust phase diagram of correlated and magnetic states using magnetotransport measurements. Lattice relaxation leads to large periodic domains in which $C_{2z}$ is broken on the moir\'e scale. Each domain harbors flat topological bands with valley-contrasting Chern numbers $\pm(1,-2)$. We find correlated states at integer electron fillings per moir\'e unit cell $\nu=1,2,3$ and fractional fillings $2/3,7/2$ with the AHE arising at $\nu=1,3$ and $2/3,7/2$. At $\nu=1$, a time-reversal symmetric phase appears beyond a critical electric displacement field, indicating a topological phase transition. Finally, hysteresis upon sweeping $\nu$ points to first-order phase transitions across a spatial mosaic of Chern domains separated by a network of topological gapless edge states. We establish HTG as an important platform that realizes ideal conditions for exploring strongly interacting topological phases and, due to its emergent moir\'e-scale symmetries, demonstrates a novel way to engineer topology.

cond-mat.mes-hall

Magnetic field stabilized Wigner crystal states in a graphene moir\'e superlattice

Wigner crystals are predicted as the crystallization of the dilute electron gas moving in a uniform background when the electron-electron Coulomb energy dominates the kinetic energy. The Wigner crystal has previously been observed in the ultraclean two-dimensional electron gas (2DEG) present on the surface of liquid helium and in semiconductor quantum wells at high magnetic field. More recently, Wigner crystals have also been reported in WS2/WSe2 moir\'e heterostructures. ABC-stacked trilayer graphene on boron nitride (ABC-TLG/hBN) moir\'e superlattices provide a unique tunable platform to explore Wigner crystal states where the electron correlation can be controlled by electric and magnetic field. Here we report the observation of magnetic field stabilized Wigner crystal states in a ABC-TLG/hBN moir\'e superlattice. We show that correlated insulating states emerge at multiple fractional and integer fillings corresponding to v = 1/3, 2/3, 1, 4/3, 5/3 and 2 electrons per moir\'e lattice site under a magnetic field. These correlated insulating states can be attributed to generalized Mott states for the integer fillings (v = 1, 2) and generalized Wigner crystal states for the fractional fillings (v = 1/3, 2/3, 4/3, 5/3). The generalized Wigner crystal states are stabilized by a vertical magnetic field, and they are strongest at one magnetic flux quantum per three moir\'e superlattices. The correlated insulating states at v = 2 persists up to 30 Tesla, which can be described by a Mott-Hofstadter transition at high magnetic field. The tunable Mott and Wigner crystal states in the ABC-TLG/hBN highlight the opportunities to discover new correlated quantum phases due to the interplay between the magnetic field and moir\'e flatbands.

cond-mat.mes-hall