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arXiv · 2509.16361

Observation of mirror-odd and mirror-even spin texture in ultrathin epitaxially strained RuO2 films

Yichen Zhang·Seung Gyo Jeong·Luca Buiarelli·Seungjun Lee·Yucheng Guo·Jiaqin Wen·Hang Li·Sreejith Nair·In Hyeok Choi·Zheng Ren·Ziqin Yue·Jounghoon Hyun·Tieqiong Zhang·Alexei Fedorov·Sung-Kwan Mo·Hojoon Lim·Adrian Hunt·Iradwikanari Waluyo·Junichiro Kono·Jan Minar·Jong Seok Lee·Tony Low·Turan Birol·Rafael M. Fernandes·Milan Radovic·Bharat Jalan·Ming Yi
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Abstract

Recently, rutile ruthenium dioxide (RuO$_2$) has attracted renewed interest due to expectations of prominent altermagnetic spin splitting. However, accumulating experimental evidence suggests that, in its bulk and thick-film forms, RuO$_2$ does not display any form of magnetic ordering. Despite this, the spin structure of RuO$_2$ remains largely unexplored in the ultrathin limit, where substrate-imposed epitaxial strain can be substantial. Here, we use spin-resolved angle-resolved photoemission spectroscopy, supported by ab initio calculations, to reveal the electronic structure of 2-nanometer-thick epitaxial RuO$_2$ heterostructures. We observe an unconventional spin texture characterized by the coexistence of mirror-even and mirror-odd momentum-dependent components. A comprehensive symmetry analysis rules out nonmagnetic origins of this spin texture. These findings suggest an emergent nonrelativistic spin structure enabled by epitaxial strain in the ultrathin limit, marking a distinct departure from the behavior of relaxed or bulk RuO$_2$. Our work opens previously unexplored perspectives for exploring symmetry-breaking mechanisms and spin textures in oxide heterostructures.

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Yichen Zhang, Seung Gyo Jeong, Luca Buiarelli, Seungjun Lee, Yucheng Guo, Jiaqin Wen, Hang Li, Sreejith Nair, In Hyeok Choi, Zheng Ren, Ziqin Yue, Jounghoon Hyun, Tieqiong Zhang, Alexei Fedorov, Sung-Kwan Mo, Hojoon Lim, Adrian Hunt, Iradwikanari Waluyo, Junichiro Kono, Jan Minar, Jong Seok Lee, Tony Low, Turan Birol, Rafael M. Fernandes, Milan Radovic, Bharat Jalan, Ming Yi. 2025-09-19. Observation of mirror-odd and mirror-even spin texture in ultrathin epitaxially strained RuO2 films. https://doi.org/10.1126/sciadv.aec2917

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