Tunable Resonant Metasurfaces Empowered by Atomically Thin Semiconductors

Abstract

Nanophotonics has recently gained new momentum with the emergence of a novel class of nanophotonic systems consisting of resonant dielectric nanostructures integrated with single or few layers of transition metal dichalcogenides (2D-TMDs). Thinned to the single layer phase, 2D-TMDs are unique solid-state systems with excitonic states able to persist at room temperature and demonstrate notable tunability of their energies in the optical range. Based on these properties, they offer important opportunities for hybrid nanophotonic systems where a nanophotonic structure serves to enhance the light-matter interaction in the 2D-TMDs, while the 2D-TMDs can provide various active functionalities, thereby dramatically enhancing the scope of nanophotonic structures. In this work, we combine 2D-TMD materials with resonant photonic nanostructures, namely, metasurfaces composed of high-index dielectric nanoparticles. The dependence of the excitonic states on charge carrier density in 2D-TMDs leads to an amplitude modulation of the corresponding optical transitions upon changes of the Fermi level, and thereby to changes of the coupling strength between the 2D-TMDs and resonant modes of the photonic nanostructure. We experimentally implement such a hybrid nanophotonic system and demonstrate voltage tuning of its reflectance as well as its different polarization-dependent behavior. Our results show that hybridization with 2D-TMDs can serve to render resonant photonic nanostructures tunable and time-variant $-$ important properties for practical applications in optical analog computers and neuromorphic circuits.