arXiv subjects

Duk-Yong Choi

Publications and source records attributed to Duk-Yong Choi.

At least 19 recordsLinked to original sources

arXiv2026

Gallium phosphide on insulator for nanophotonics and quantum technologies

Gallium phosphide is a promising material platform for visible and near-infrared photonics and quantum technologies owing to its high refractive index, low optical absorption, and strong second-order nonlinearity. Here, we demonstrate the fabrication of GaP-on-insulator substrates by ion slicing. The splitting depth and exfoliation behavior of bulk GaP are tailored by controlling the He$^{+}$ ion implantation energy and fluence, enabling thin-film transfer onto amorphous substrates by anodic bonding and plasma-enhanced direct wafer bonding. Channeling Rutherford backscattering spectrometry and X-ray diffraction confirm that the transferred layers retain their single-crystalline structure, while implantation-induced disorder and optical absorption are substantially reduced by annealing at 500 °C and subsequent polishing. The annealed films exhibit linear optical properties approaching those of bulk GaP. In addition, a (110)-oriented GaP thin film shows the characteristic polarization dependence expected from the zinc-blende second-order nonlinear susceptibility tensor, demonstrating a near-pristine second-order nonlinear response. This flexible fabrication approach enables the integration of high-quality single-crystalline GaP with variable orientation for free-space and integrated nanophotonics as well as nonlinear and quantum optical devices.

physics.optics↗

arXiv2026

Strong enhancement of Er3+ emission at room temperature in Si3N4 metasurfaces

We report a significant enhancement of room-temperature photoluminescence from trivalent erbium-doped (Er3+) silicon nitride (Si3N4) metasurfaces at the telecommunication wavelength prepared via ion implantation. The metasurfaces, consisting of periodic nanocylinder arrays, are designed to support Mie-type resonances that tailor the local density of optical states. By systematically optimizing the nanocylinder radii, we achieve a photoluminescence (PL) enhancement factor of ~18 at a radius of 390 nm after thermal annealing, which is in excellent agreement with our simulations. Time-resolved PL measurements reveal a nearly ten-fold reduction in luminescence lifetime, confirming that the enhancement is primarily driven by the Purcell effect. Furthermore, we demonstrate that the PL intensity is strongly dependent on the Er3+ ion implantation depth, with a four-fold increase in emission observed from 20 nm to 80 nm ion range. These results provide a robust pathway for integrating efficient, active light sources into CMOS-compatible photonic device.

physics.optics↗

arXiv2026

Towards Polarization Routing of Magnetic and Electric Dipolar Emission with Dielectric Metasurfaces

We investigate the polarization properties of emission associated with the magnetic dipole and electric dipole transitions of europium(III) coupled to an anisotropic dielectric metasurface with polarization-engineered electric and magnetic photonic local density of states. The metasurface consists of a square array of Mie-resonant elliptical a-Si:H dimers situated on an SiO$_2$ substrate and embedded in a PMMA film containing Eu(TTA)$_3$. Based on reciprocity principle, it was designed to achieve maximum electric (magnetic) field enhancement in the dimer gap at 610 nm (590 nm) for $x$-polarized ($y$-polarized) normally incident light in order to selectively enhance the electric dipole (magnetic dipole) emission into the $x$-polarized ($y$-polarized) emission channel, respectively. Momentum-resolved spectroscopy and back-focal plane imaging of emission of the fabricated light-emitting metasurface clearly reveal the intended polarization-dependent emission behaviour, with the $x$-polarized ($y$-polarized) emission showing a reduced (enhanced) ratio of the magnetic-/electric dipole emission intensity, correspondingly where the magnetic dipole emission is enhanced with a magnetic field enhancement from the nanostructures. The demonstrated polarization-dependent interaction of a designed nanostructure with the electric- and magnetic dipolar transitions of trivalent lanthanide ions opens an avenue towards routing of emission of different multipolar orders into different polarization channels.

physics.optics↗

arXiv2025

Polarization Dependent Enhancement of Magnetic Dipolar Emission with Silicon Nanodimers

Eu(TTA)3 complexes are used as an emission source in the presence of high refractive index dielectric nanostructures. These nanostructures support Mie-type resonances that modify the local density of optical states. Specifically, the silicon dimer provides polarization-dependent electric and magnetic field enhancement in the dimer gap to modify the electric dipolar and magnetic dipolar emissions of the Eu3+ at 610 nm and 590 nm, respectively. Finite element method simulations are used to determine the optimal parameters for the sample and to demonstrate the polarization-dependent emission enhancement of dipolar emitters in the gap. A two-step electron beam lithography process is used to fabricate the hybrid nanoscopic structures, with a Eu3+ doped electron beam resist located only in the center of the dimer. The results demonstrate the potential of these nanostructures to selectively tailor the emission of the two distinct dipolar transitions by engineering the resonant nanostructures. Our work highlights the potential of magnetic light-matter interactions as a novel degree of freedom.

physics.optics↗

arXiv2025

Tunable Resonant Metasurfaces Empowered by Atomically Thin Semiconductors

Nanophotonics has recently gained new momentum with the emergence of a novel class of nanophotonic systems consisting of resonant dielectric nanostructures integrated with single or few layers of transition metal dichalcogenides (2D-TMDs). Thinned to the single layer phase, 2D-TMDs are unique solid-state systems with excitonic states able to persist at room temperature and demonstrate notable tunability of their energies in the optical range. Based on these properties, they offer important opportunities for hybrid nanophotonic systems where a nanophotonic structure serves to enhance the light-matter interaction in the 2D-TMDs, while the 2D-TMDs can provide various active functionalities, thereby dramatically enhancing the scope of nanophotonic structures. In this work, we combine 2D-TMD materials with resonant photonic nanostructures, namely, metasurfaces composed of high-index dielectric nanoparticles. The dependence of the excitonic states on charge carrier density in 2D-TMDs leads to an amplitude modulation of the corresponding optical transitions upon changes of the Fermi level, and thereby to changes of the coupling strength between the 2D-TMDs and resonant modes of the photonic nanostructure. We experimentally implement such a hybrid nanophotonic system and demonstrate voltage tuning of its reflectance as well as its different polarization-dependent behavior. Our results show that hybridization with 2D-TMDs can serve to render resonant photonic nanostructures tunable and time-variant $-$ important properties for practical applications in optical analog computers and neuromorphic circuits.

physics.optics↗

arXiv2025

Brillouin lasers in Bragg grating microresonators

Chip-scale coherent light sources are required in applications spanning metrology and sensing to telecommunications. Brillouin lasers (BLs) offer a route to ultra-coherent optical sources in compact microresonators with free spectral range (FSR) matched to the Brillouin frequency shift (BFS). However, BFS - FSR matching typically facilitates cascaded Brillouin scattering, constraining achievable BL output power and coherence. Here, we demonstrate inhibition of cascading in a planar-integrated chalcogenide microresonator by exploiting the photonic bandgap (PBG) associated with a post-fabrication inscribed, reconfigurable intracavity Bragg grating. The PBG inhibits energy transfer within the target Brillouin scattering pathway, such as from pump to first-order Stokes wave. As a quantitative measure of Brillouin scattering inhibition, we report at least six-fold increase in threshold for onset of BL oscillation, which is ultimately limited by thermorefraction. For on-chip pump power of 399 mW, sufficient for a tenth-order Brillouin cascade, complete inhibition was achieved. Our work positions Bragg grating microresonators as an enabling platform for high performance on-chip BL sources, with reconfigurable modes of operation.

physics.optics↗

arXiv2024

A mid-infrared Brillouin laser using ultra-high-Q on-chip resonators

Ultra-high-Q optical resonators have facilitated recent advancements in on-chip photonics by effectively harnessing nonlinear phenomena providing useful functionalities. While these breakthroughs, primarily focused on the near-infrared region, have extended interest to longer wavelengths holding importance for monitoring and manipulating molecules, the absence of ultra-high-Q resonators in this region remains a significant challenge. Here, we have developed on-chip microresonators with a remarkable Q-factor of 38 million, surpassing previous mid-infrared records by over 30 times. Employing innovative fabrication techniques, including the spontaneous formation of light-guiding geometries during material deposition, resonators with internal multilayer structures have been seamlessly created and passivated with chalcogenide glasses within a single chamber. Major loss factors, especially airborne-chemical absorption, were thoroughly investigated and mitigated by extensive optimization of resonator geometries and fabrication procedures. This allowed us to access the fundamental loss performance offered by doubly purified chalcogenide glass sources, as demonstrated in their fiber form. Exploiting this ultra-high-Q resonator, we successfully demonstrated Brillouin lasing on a chip for the first time in the mid-infrared, with a threshold power of 91.9 μW and a theoretical Schawlow-Townes linewidth of 83.45 Hz, far surpassing carrier phase noise. Our results showcase the effective integration of cavity-enhanced optical nonlinearities into on-chip mid-infrared photonics.

physics.optics↗

arXiv2023

On-Chip Stimulated Brillouin Scattering via Surface Acoustic Waves

Surface acoustic wave (SAW) devices are ubiquitously used for signal processing and filtering, as well as mechanical, chemical and biological sensing, and show promise as quantum transducers. However, nowadays most SAWs are excited and driven via electromechanical coupling and interdigital transducers (IDTs), limiting operation bandwidth and flexibility. Novel ways to coherently excite and detect SAWs all-optically interfaced with photonic integrated circuits are yet elusive. Backward Stimulated Brillouin scattering (SBS) provides strong coherent interactions between optical and acoustic waves in chip-scale waveguides, however, demonstrations have been limited to single longitudinal waves in the waveguide core. Here, we numerically model and experimentally demonstrate surface acoustic wave stimulated Brillouin scattering (SAW-SBS) on a photonic chip. We designed and fabricated tailored waveguides made out of GeAsSe glass that show good overlap between SAWs at 3.81 GHz and guided optical modes, without requiring a top cladding. We measure a 225 W$^{-1}$m$^{-1}$ Brillouin gain coefficient of the surface acoustic resonance and linewidth narrowing to 40 MHz. Experimentally accessing this new regime of stimulated Brillouin scattering opens the door for novel on-chip sensing and signal processing applications, strong Brillouin interactions in materials that do not provide sufficient acoustic guidance in the waveguide core as well as excitation of surface acoustic waves in non-piezoelectric materials.

physics.optics↗

arXiv2022

Nonlinear imaging of nanoscale topological corner states

Topological states of light represent counterintuitive optical modes localized at boundaries of finite-size optical structures that originate from the properties of the bulk. Being defined by bulk properties, such boundary states are insensitive to certain types of perturbations, thus naturally enhancing robustness of photonic circuitries. Conventionally, the N-dimensional bulk modes correspond to (N-1)-dimensional boundary states. The higher-order bulk-boundary correspondence relates N-dimensional bulk to boundary states with dimensionality reduced by more than 1. A special interest lies in miniaturization of such higher-order topological states to the nanoscale. Here, we realize nanoscale topological corner states in metasurfaces with C6-symmetric honeycomb lattices. We directly observe nanoscale topology-empowered edge and corner localizations of light and enhancement of light-matter interactions via a nonlinear imaging technique. Control of light at the nanoscale empowered by topology may facilitate miniaturization and on-chip integration of classical and quantum photonic devices.

physics.optics↗

arXiv2020

High-harmonic generation from metasurfaces empowered by bound states in the continuum

The concept of optical bound states in the continuum (BICs) underpins the existence of strongly localized waves embedded into the radiation spectrum that can enhance the electromagnetic fields in subwavelength photonic structures. Early studies of optical BICs in waveguides and photonic crystals uncovered their topological properties, and the concept of quasi-BIC metasurfaces facilitated applications of strong light-matter interactions to biosensing, lasing, and low-order nonlinear processes. Here we employ BIC-empowered dielectric metasurfaces to generate efficiently high optical harmonics up to the 11th order. We optimize a BIC mode for the first few harmonics and observe a transition between perturbative and nonperturbative nonlinear regimes. We also suggest a general strategy for designing subwavelength structures with strong resonances and nonperturbative nonlinearities. Our work bridges the fields of perturbative and nonperturbative nonlinear optics on the subwavelength scale.

physics.optics↗

arXiv2019

Photosensitive chalcogenide metasurfaces supporting bound states in the continuum

We study, both theoretically and experimentally, tunable metasurfaces supporting sharp Fano-resonances inspired by optical bound states in the continuum. We explore the use of arsenic trisulfide (a photosensitive chalcogenide glass) having optical properties which can be finely tuned by light absorption at the post-fabrication stage. We select the resonant wavelength of the metasurface corresponding to the energy below the arsenic trisulfide bandgap, and experimentally control the resonance spectral position via exposure to the light of energies above the bandgap.

physics.optics↗

arXiv2019

Universal light-guiding geometry for high-nonlinear resonators having molecular-scale roughness

By providing an effective way to leverage nonlinear phenomena in chip-scale, high-Q optical resonators have induced the recent advances of on-chip photonics represented by micro-combs and ultra-narrow linewidth lasers. These achievements mainly relying on Si, SiO$_{2}$, and Si$_{3}$N$_{4}$ are expected to be further improved by introducing new materials having higher nonlinearity. However, establishing fabrication processes to shape a new material into the resonator geometries having extremely smooth surfaces on a chip has been a challenging task. Here we describe a universal method to implement high-Q resonators with any materials which can be deposited in high vacuum. This approach, by which light-guiding cores having surface roughness in molecular-scale is automatically defined along the prepatterned platform structures during the deposition, is verified with As$_{2}$S$_{3}$, a typical chalcogenide glass of high-nonlinearity. The Q-factor of the developed resonator is 14.4 million approaching the loss of chalcogenide fibers, which is measured in newly proposed tunable waveguide-to-resonator coupling scheme with high ideality. Lasing by stimulated Brillouin process is demonstrated with threshold power of 0.53 mW which is 100 times lower than the previous record based on chalcogenide glasses. This approach paves the way for bringing various materials of distinguished virtues to the on-chip domain while keeping the loss performance comparable to that of bulk form.

physics.optics↗

arXiv2019

Third-harmonic generation in photonic topological metasurfaces

We study nonlinear effects in two-dimensional photonic metasurfaces supporting topologically-protected helical edge states at the nanoscale. We observe strong third-harmonic generation mediated by optical nonlinearities boosted by multipolar Mie resonances of silicon nanoparticles. Variation of the pump-beam wavelength enables independent high-contrast imaging of either bulk modes or spin-momentum-locked edge states. We demonstrate topology-driven tunable localization of the generated harmonic fields and map the pseudospin-dependent unidirectional waveguiding of the edge states bypassing sharp corners. Our observations establish dielectric metasurfaces as a promising platform for the robust generation and transport of photons in topological photonic nanostructures.

physics.optics↗

arXiv2019

Nonlinear metasurfaces governed by bound states in the continuum

Nonlinear nanostructured surfaces provide a paradigm shift in nonlinear optics with new ways to control and manipulate frequency conversion processes at the nanoscale, also offering novel opportunities for applications in photonics, chemistry, material science, and biosensing. Here, we develop a general approach to employ sharp resonances in metasurfaces originated from the physics of bound states in the continuum for both engineering and enhancing the nonlinear response. We study experimentally the third-harmonic generation from metasurfaces composed of symmetry-broken silicon meta-atoms and reveal that the harmonic generation intensity depends critically on the asymmetry parameter. We employ the concept of the critical coupling of light to the metasurface resonances to uncover the effect of radiative and nonradiative losses on the nonlinear conversion efficiency.

physics.app-ph↗

arXiv2018

Extreme Huygens' metasurfaces based on quasi-bound states in the continuum

We introduce the concept and a generic approach to realize Extreme Huygens' Metasurfaces by bridging the concepts of Huygens' conditions and optical bound states in the continuum. This novel paradigm allows creating Huygens' metasurfaces whose quality factors can be tuned over orders of magnitudes, generating extremely dispersive phase modulation. We validate this concept with a proof-of-concept experiment at the near-infrared wavelengths, demonstrating all-dielectric Huygens' metasurfaces with different quality factors. Our study points out a practical route for controlling the radiative decay rate while maintaining the Huygens' condition, complementing existing Huygens' metasurfaces whose bandwidths are relatively broad and complicated to tune. This novel feature can provide new insight for various applications, including optical sensing, dispersion engineering and pulse-shaping, tunable metasurfaces, metadevices with high spectral selectivity, and nonlinear meta-optics.

physics.optics↗

arXiv2018

Chip-based Brillouin processing for carrier recovery in coherent optical communications

Modern fiber-optic coherent communications employ advanced spectrally-efficient modulation formats that require sophisticated narrow linewidth local oscillators (LOs) and complex digital signal processing (DSP). Here, we establish a novel approach to carrier recovery harnessing large-gain stimulated Brillouin scattering (SBS) on a photonic chip for up to 116.82 Gbit/sec self-coherent optical signals, eliminating the need for a separate LO. In contrast to SBS processing on-fiber, our solution provides phase and polarization stability while the narrow SBS linewidth allows for a record-breaking small guardband of ~265 MHz, resulting in higher spectral-efficiency than benchmark self-coherent schemes. This approach reveals comparable performance to state-of-the-art coherent optical receivers without requiring advanced DSP. Our demonstration develops a low-noise and frequency-preserving filter that synchronously regenerates a low-power narrowband optical tone that could relax the requirements on very-high-order modulation signaling and be useful in long-baseline interferometry for precision optical timing or reconstructing a reference tone for quantum-state measurements.

physics.app-ph↗

arXiv2018

On-chip correlation-based Brillouin sensing: design, experiment and simulation

Wavelength-scale SBS waveguides are enabling novel on-chip functionalities. The micro- and nano-scale SBS structures and the complexity of the SBS waveguides require a characterization technique to monitor the local geometry-dependent SBS responses along the waveguide. In this work, we experimentally demonstrate detection of longitudinal features down to 200$μ$m on a silicon-chalcogenide waveguide using the Brillouin optical correlation domain analysis (BOCDA) technique. We provide simulation and analysis on how multiple acoustic and optical modes and geometrical variations influence the Brillouin spectrum.

physics.app-ph↗

arXiv2018

Brillouin spectroscopy of a hybrid silicon-chalcogenide waveguide with geometrical variations

Recent advances in design and fabrication of photonic-phononic waveguides have enabled stimulated Brillouin scattering (SBS) in silicon-based platforms, such as under-etched silicon waveguides and hybrid waveguides. Due to the sophisticated design and more importantly high sensitivity of the Brillouin resonances to geometrical variations in micro- and nano-scale structures, it is necessary to have access to the localized opto-acoustic response along those waveguides to monitor their uniformity and maximize their interaction strength. In this work, we design and fabricate photonic-phononic waveguides with a deliberate width variation on a hybrid silicon-chalcogenide photonic chip and confirm the effect of the geometrical variation on the localized Brillouin response using a distributed Brillouin measurement.

physics.optics↗