Intrinsic translational symmetry-breaking charge stripes in underdoped iron pnictides

Abstract

Despite being well established in cuprates, an intrinsic translational symmetry-breaking charge order has not been clearly identified in iron-based superconductors. Using spectroscopic-imaging scanning tunneling microscopy on epitaxial Ca(Fe1-xCox)2As2 (x = 0 ~ 0.055) thin films, we observe smectic, near-commensurate charge-stripe order in the underdoped regime that intervenes between the nematic parent phase and optimally doped superconductivity. Distinct from the bidirectional checkerboard-like order in cuprates, these charge stripes are unidirectional along the antiferromagnetic Fe-Fe bond direction and are accompanied by a van Hove singularity near the Fermi level, inherited from the Fermi surface reconstruction driven by intertwined antiferromagnetic and nematic correlations. Both local and global suppression of the charge-stripe instability enhance superconductivity, tunable via epitaxial strain and Co doping. These results establish charge-stripe order as an intermediate electronic phase in iron pnictides and reveal a coherent pathway from nematicity to superconductivity. Our findings highlight charge ordering as a unifying element across different families of high-temperature superconductors.