Searcharxiv⌕ Search
Home/Archive/arXiv

arXiv · 2603.08912

Isotopic Measurements of SNM using a Portable Neutron Resonance Transmission System for Arms Control

Mital A. Zalavadia·Ethan A. Klein·Michael E. Moore·Jonathan A. Kulisek·Farheen Naqvi·Glen A. Warren·Areg Danagoulian
View original source ↗Read source document ↗Export metadata ↓

Abstract

Neutron Resonance Transmission Analysis (NRTA) was explored as an arms control verification approach to support potential future nuclear weapon limiting treaties. A compact and portable neutron Time of Flight (ToF) system was developed to enable proof-of-concept NRTA measurements of special nuclear material (SNM). Using a short 2-meter flight path, the NRT system is sensitive to cross-section resonances of isotopes such as 235U, 238U, 239Pu and 240Pu between 1-100 eV incident neutron energies due to their physical nuclear structure. The detected neutron ToF spectrum exhibits transmission dips at resonance energies that are characteristic of SNM isotopic composition in the inspected item. The proof-of-concept measurements of Highly Enriched Uranium (HEU), Depleted Uranium (DU), and Reactor Grade Plutonium (RGPu) confirmed the characteristic resonance features within two hours of data collection time. Analysis via the REFIT resonance fitting tool accurately predicted the 235U enrichment and Pu isotopic composition within 5% and 6% of the known values, respectively.

Explore related subjects

physics.ins-detnucl-exphysics.soc-ph

Keep this discovery

BibTeXRIS

Mital A. Zalavadia, Ethan A. Klein, Michael E. Moore, Jonathan A. Kulisek, Farheen Naqvi, Glen A. Warren, Areg Danagoulian. 2026-03-09. Isotopic Measurements of SNM using a Portable Neutron Resonance Transmission System for Arms Control. https://arxiv.org/abs/2603.08912

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

arXiv2026

High-Speed Semi-FE Readout Module for ATLAS MDT at HL-LHC: Design and Production-Level Characterization

The High-Luminosity upgrade of the Large Hadron Collider (HL-LHC) introduces increased demands on the ATLAS Muon Spectrometer, particularly in terms of data throughput, timing distribution and system reliability. The Phase-II Chamber Service Module (CSM) is a key component of the upgraded Monitored Drift Tube (MDT) trigger and readout system, providing a high-speed interface between the front-end electronics and the backend systems. This paper describes the design and implementation of the Phase-II CSM, together with its validation. The results show that the CSM supports two independent optical uplinks, each operating at a line rate of 10.24 Gbps, together with clock distribution and slow control in the expected operating environment. Integration with small-diameter MDT (sMDT) chambers and tests with the prototype L0MDT trigger system are also presented. The CSM boards are now in production and will be used for installation and integration during the upcoming LHC Long Shutdown.

physics.ins-det↗
arXiv2026

Spectral Discrimination of Deposited Gamma-Ray Energies in a Simulated CeBr$_3$ Scintillator

We show that wavelength measurements of individual detected optical photons may provide additional information about gamma-ray energy deposited in a CeBr$_3$ crystal when the detected-photon-count distributions overlap for nearby gamma-ray energies. Monoenergetic 662 and 629 keV gammas are used in a Geant4 simulation of a $25\times25\times20~\mathrm{mm^3}$ CeBr$_3$ crystal. Assuming a light yield of $6.0\times10^4$ photons/MeV, a wavelength-independent photon-detection efficiency of 30%, and a wavelength resolution of $\sigma_{\lambda}=40$ nm, we find that the fraction of photons reconstructed above 385 nm gives an event-level separation of $\sim$ 2 standard deviations between the 662 and 629 keV event populations selected within the same $\sim$ 1%-wide detected-photon-count interval. No timing or reconstructed interaction-position information is used. The result demonstrates, within the present simulation model, that event-dependent optical spectra can retain energy information beyond an undifferentiated photon count.

physics.ins-det↗
arXiv2026

Operation of a negative ion gas time projection chamber without electronegative fill gases

The high fidelity reconstruction of particle tracks in micropatterned gaseous time projection chambers renders this technology ideal for future rare-event searches, including direction-sensitive dark matter experiments. Large drift distances are typically required for such experiments, so that the overall spatial resolution is limited by diffusion. Negative ion drift exhibits lower diffusion than electron drift and is thus an attractive option for realising a large-scale detector. The use of electronegative gases to create negative ions introduces technical challenges, most notably a reduction in gain when compared to conventional gas mixtures. In this study, we demonstrate a new method for negative ion generation via dissociative electron attachment using the conventional molecular fill gas CF$_4$. Our optical measurements of negative ion drift indicate electron attachment lengths of $<$1 mm and comparable gain to electron avalanches. The individual negative ion avalanches were also time-resolved, allowing the number of ions reaching the readout to be counted. We measure an improved energy resolution by single ion counting, relative to an integrated electron avalanche signal measured under identical gain conditions.

physics.ins-det↗