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arXiv · 2605.21124

Observation of spin-free interatomic orbital angular momentum in a chiral crystal

Dongjin Oh·Sungsoo Hahn·Chiara Pacella·Junseo Yoo·Angel Rubio·Domenico Di Sante·Changyoung Kim
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Abstract

The inherent spin-orbit interaction of electrons inevitably couples spin to the orbital angular momentum (OAM), posing a fundamental challenge to spin-free orbital transport. Here, we propose a novel strategy to achieve spin-decoupled OAM states in crystalline solids. Using angle-resolved photoemission spectroscopy (ARPES), we resolve well-isolated s-orbital bands in a chiral Te crystal, clearly separated from the p-orbital manifold. Combined circular dichroism ARPES and first-principles calculations reveal that these bands host OAM arising exclusively from interatomic hopping, with no intra-atomic contribution. Spin-resolved ARPES further confirms the absence of spin angular momentum (SAM), providing decisive evidence of spin-free OAM states. These findings establish the existence of OAM without spin polarization in crystalline solids and highlight the essential role of inter-atomic OAM. This work provides a general framework for designing spinless OAM states, opening an opportunity toward pure orbital currents for orbitronics.

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Dongjin Oh, Sungsoo Hahn, Chiara Pacella, Junseo Yoo, Angel Rubio, Domenico Di Sante, Changyoung Kim. 2026-05-20. Observation of spin-free interatomic orbital angular momentum in a chiral crystal. https://arxiv.org/abs/2605.21124

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