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Junseo Yoo

Publications and source records attributed to Junseo Yoo.

4 recordsLinked to original sources

Quenching of Nonrelativistic $p$-Wave Spin Splitting by Reduced $c\text{-}f$ Coupling in $\text{CeNiAsO}$

The application of spin-space group symmetries to noncollinear antiferromagnets has led to the prediction of odd-parity, nonrelativistic spin splittings, making the physical realization of a practical $p$-wave magnet a central pursuit in spintronics. The layered heavy-fermion oxypnictide $\text{CeNiAsO}$ has been widely regarded as a prototypical platform to verify this paradigm. Here, we investigate the electronic structure of single-crystal $\text{CeNiAsO}$ using high-resolution, ultra-low-temperature and resonant angle-resolved photoemission spectroscopy (ARPES), and $ab-initio$ calculations. Across the consecutive magnetic transitions into the ordered phases, our spectroscopic data reveal neither the expected band folding associated with a spin density wave nor any observable $p$-wave spin splitting, demonstrating that the conduction bands retain full degeneracy. By tracking the temperature dependence of the Ce 4$f$ spectral weight via resonant ARPES, we find negligible $c\text{-}f$ hybridization near the Fermi level within magnetically ordered states, confirming that the Ce 4$f$ electrons reside close to the localized limit. Our findings establish a clear many-body constraint on the projection of real-space magnetic symmetries onto momentum-space electronic bands, demonstrating that symmetry classifications constitute a necessary framework but are not a sufficient condition for nonrelativistic spin splittings in the presence of strong electronic correlations.

cond-mat.str-el

Observation of spin-free interatomic orbital angular momentum in a chiral crystal

The inherent spin-orbit interaction of electrons inevitably couples spin to the orbital angular momentum (OAM), posing a fundamental challenge to spin-free orbital transport. Here, we propose a novel strategy to achieve spin-decoupled OAM states in crystalline solids. Using angle-resolved photoemission spectroscopy (ARPES), we resolve well-isolated s-orbital bands in a chiral Te crystal, clearly separated from the p-orbital manifold. Combined circular dichroism ARPES and first-principles calculations reveal that these bands host OAM arising exclusively from interatomic hopping, with no intra-atomic contribution. Spin-resolved ARPES further confirms the absence of spin angular momentum (SAM), providing decisive evidence of spin-free OAM states. These findings establish the existence of OAM without spin polarization in crystalline solids and highlight the essential role of inter-atomic OAM. This work provides a general framework for designing spinless OAM states, opening an opportunity toward pure orbital currents for orbitronics.

cond-mat.mtrl-sci

Fragility of Topology under Electronic Correlations in Iron Chalcogenides

The interplay between electronic correlations and topology is a central topic in the study of quantum materials. In this work, we investigate the impact of the orbital-selective Mott phase (OSMP) on the topological properties of FeTe1-xSex (FTS), an iron chalcogenide superconductor known to host both non-trivial Z2 topology and strong electronic correlations. Using angle-resolved photoemission spectroscopy, we track the evolution of topological surface states across various doping levels and temperatures. We identify a topological phase transition between trivial and non-trivial topology as a function of selenium content, with critical behavior observed between x = 0.04 and x = 0.09. Additionally, we find that at elevated temperatures, the coherence of the topological surface state deteriorates due to the emergence of OSMP, despite the topological invariant remaining intact. Our results demonstrate that the non-trivial topology in iron chalcogenide is fragile under strong electronic correlations.

cond-mat.str-el

Picsou: Enabling Replicated State Machines to Communicate Efficiently

Replicated state machines (RSMs) cannot communicate effectively today as there is no formal framework or efficient protocol to do so. To address this issue, we introduce a new primitive, Cross-Cluster Consistent Broadcast (C3B) and present PICSOU, a practical implementation of the C3B primitive. PICSOU draws inspiration from networking and TCP to allow two RSMs to communicate with constant metadata overhead in the failure-free case and a minimal number of message resends in the case of failures. PICSOU is flexible and allows both crash fault tolerant and Byzantine fault tolerant consensus protocols to communicate. At the heart of PICSOU's good performance and generality is the concept of QUACKs (quorum acknowledgments). QUACKs allow nodes in each RSM to precisely determine when messages have definitely been received, or likely lost. Our results are promising: we obtain up to 24x better performance than prior solutions on microbenchmarks and applications, ranging from disaster recovery to data reconciliation.

cs.DC