Low-temperature magnetism and spin dynamics in the disordered triangular-lattice Yb$^{3+}$ compound LiCaYb$_5$(BO$_3$)$_6$

Monika Jawale; Saikat Nandi; Prashanta K. Mukharjee; Philipp Gegenwart; A. V. Mahajan

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arXiv · 2608.26946

Low-temperature magnetism and spin dynamics in the disordered triangular-lattice Yb$^{3+}$ compound LiCaYb$_5$(BO$_3$)$_6$

Monika Jawale·Saikat Nandi·Prashanta K. Mukharjee·Philipp Gegenwart·A. V. Mahajan

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Abstract

The interplay between geometric frustration, spin--orbit coupling, and structural disorder can give rise to unconventional magnetic ground states in rare-earth triangular-lattice magnets. We report low-temperature magnetic and $^7$Li NMR investigations of the disordered triangular-lattice compound LiCaYb$_5$(BO$_3$)$_6$ (LCYBO). Rietveld refinement confirms a hexagonal $P6_522$ structure with partial Ca/Yb antisite disorder and fractional Li occupancy. Magnetic susceptibility and magnetization measurements indicate a well-isolated effective $J_{\mathrm{eff}}=1/2$ Kramers doublet with weak antiferromagnetic interactions ($\theta_{\mathrm{CW}} \approx -0.54$~K). The specific heat reveals a weak anomaly near 0.43 K, suggesting the development of short-range correlated magnetism rather than conventional long-range order. $^7$Li NMR spectra broaden strongly upon cooling, consistent with increasingly inhomogeneous internal magnetic fields. The spin-lattice relaxation exhibits two relaxation components consistent with disorder-induced distributions of local magnetic environments arising from antisite disorder and competing exchange pathways. Our results establish LCYBO as a structurally disordered frustrated triangular-lattice magnet with correlated low-energy spin dynamics.

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Monika Jawale, Saikat Nandi, Prashanta K. Mukharjee, Philipp Gegenwart, A. V. Mahajan. 2026-08-27. Low-temperature magnetism and spin dynamics in the disordered triangular-lattice Yb$^{3+}$ compound LiCaYb$_5$(BO$_3$)$_6$. https://arxiv.org/abs/2608.26946

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