THz-induced phonomagnetism in diamagnetic quantum paraelectric KTaO$_3$

C. Kadlec; F. Kadlec; D. Repček; P. Kužel; M. Basini; J. -C. Deinert; S. Kovalev; T. Tadano; M. Udina; I. Ilyakov; T. V. A. G. de Oliveira; A. Ponomaryov; A. Arshad; A. Maia; S. Bonetti; S. Kamba

arXiv · 2608.27060

THz-induced phonomagnetism in diamagnetic quantum paraelectric KTaO$_3$

C. Kadlec·F. Kadlec·D. Repček·P. Kužel·M. Basini·J. -C. Deinert·S. Kovalev·T. Tadano·M. Udina·I. Ilyakov·T. V. A. G. de Oliveira·A. Ponomaryov·A. Arshad·A. Maia·S. Bonetti·S. Kamba

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Abstract

The current efforts striving to develop new ways of data manipulation are aimed at ultrafast control of magnetization in magnetic materials, as well as at inducing magnetic moments in diamagnetics. We demonstrate that in the diamagnetic quantum paraelectric KTaO$_3$, the electric field of circularly polarized THz pulses with an amplitude of $\sim 300\,$kV/cm induces a transient magnetic-like response by resonantly exciting its degenerate soft polar phonon. This phonon-mediated response was measured using the THz pump---optical probe technique via the time-resolved magneto-optic Faraday effect. Our detection scheme was set up to cancel out the major part of the electro-optic Kerr effect which also usually significantly contributes to the transient response. The Kerr-effect-related signal was further suppressed by subtracting the experimental data related to oppositely circularly polarized THz radiation. Thus, we were able to unambiguously identify a temperature-dependent magnetic-like behavior of the KTaO$_3$ crystal manifested by the extracted Faraday rotation. We developed a theoretical model describing well quantitatively the measured curves of the transient Faraday effect signal. However, their amplitudes exhibit an unexpected temperature dependence, which might be a key to a deeper understanding of the observed phonomagnetic effect.

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C. Kadlec, F. Kadlec, D. Repček, P. Kužel, M. Basini, J. -C. Deinert, S. Kovalev, T. Tadano, M. Udina, I. Ilyakov, T. V. A. G. de Oliveira, A. Ponomaryov, A. Arshad, A. Maia, S. Bonetti, S. Kamba. 2026-08-27. THz-induced phonomagnetism in diamagnetic quantum paraelectric KTaO$_3$. https://arxiv.org/abs/2608.27060

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