arXiv subjects

F. Kadlec

Publications and source records attributed to F. Kadlec.

6 recordsLinked to original sources

arXiv2026

THz-induced phonomagnetism in diamagnetic quantum paraelectric KTaO$_3$

The current efforts striving to develop new ways of data manipulation are aimed at ultrafast control of magnetization in magnetic materials, as well as at inducing magnetic moments in diamagnetics. We demonstrate that in the diamagnetic quantum paraelectric KTaO$_3$, the electric field of circularly polarized THz pulses with an amplitude of $\sim 300\,$kV/cm induces a transient magnetic-like response by resonantly exciting its degenerate soft polar phonon. This phonon-mediated response was measured using the THz pump---optical probe technique via the time-resolved magneto-optic Faraday effect. Our detection scheme was set up to cancel out the major part of the electro-optic Kerr effect which also usually significantly contributes to the transient response. The Kerr-effect-related signal was further suppressed by subtracting the experimental data related to oppositely circularly polarized THz radiation. Thus, we were able to unambiguously identify a temperature-dependent magnetic-like behavior of the KTaO$_3$ crystal manifested by the extracted Faraday rotation. We developed a theoretical model describing well quantitatively the measured curves of the transient Faraday effect signal. However, their amplitudes exhibit an unexpected temperature dependence, which might be a key to a deeper understanding of the observed phonomagnetic effect.

cond-mat.mtrl-sci↗

arXiv2025

Antiferromagnetic resonance in $\alpha$-MnTe

Antiferromagnetic resonance in a bulk $\alpha$-MnTe crystal is investigated using both frequency-domain and time-domain THz spectroscopy techniques. At low temperatures, an excitation at the photon energy of $(3.5\pm 0.1)$~meV is observed and identified as a magnon mode through its distinctive dependence on temperature and magnetic field. This behavior is reproduced using a simplified model for antiferromagnetic resonance in an easy-plane antiferromagnet. The results of our experiments, when compared to exchange constants established in the literature, allow us to extract the out-of-plane component of the single-ion magnetic anisotropy reaching $(40\pm10)$~$\mu$eV.

cond-mat.mtrl-sci↗

arXiv2021

Onset of superconductor-insulator transition in an ultrathin NbN film under in-plane magnetic field studied by terahertz spectroscopy

Optical conductivity of a moderately disordered superconducting NbN film was investigated by terahertz time-domain spectroscopy in external magnetic field applied along the film plane. The film thickness of about 5 nm was comparable with the coherence length, so vortices should not form. This was confirmed by the fact that no marked difference between the spectra with terahertz electric field set perpendicular and parallel to the external magnetic field was observed. Simultaneous use of Maxwell-Garnett effective medium theory and the model of optical conductivity by Herman and Hlubina proved to correctly reproduce the terahertz spectra obtained experimentally in a magnetic field of up to 7 T. This let us conclude that the magnetic field tends to suppress the superconductivity, resulting in an inhomogeneous state where superconducting domains are enclosed within a normal-state matrix. The scattering rate due to pair-breaking effects was found to linearly increase with magnetic field.

cond-mat.supr-con↗

arXiv2015

Spin and lattice excitations of a BiFeO3 thin film and ceramics

We present a comprehensive study of polar and magnetic excitations in BiFeO3 ceramics and a thin film epitaxially grown on an orthorhombic (110) TbScO3 substrate. Infrared reflectivity spectroscopy was performed at temperatures from 5 to 900 K for the ceramics and below room temperature for the thin film. All 13 polar phonons allowed by the factor-group analysis were observed in theceramic samples. The thin-film spectra revealed 12 phonon modes only and an additional weak excitation, probably of spin origin. On heating towards the ferroelectric phase transition near 1100 K, some phonons soften, leading to an increase in the static permittivity. In the ceramics, terahertz transmission spectra show five low-energy magnetic excitations including two which were not previously known to be infrared active; at 5 K, their frequencies are 53 and 56 cm-1. Heating induces softening of all magnetic modes. At a temperature of 5 K, applying an external magnetic field of up to 7 T irreversibly alters the intensities of some of these modes. The frequencies of the observed spin excitations provide support for the recently developed complex model of magnetic interactions in BiFeO3 (R.S. Fishman, Phys. Rev. B 87, 224419 (2013)). The simultaneous infrared and Raman activity of the spin excitations is consistent with their assignment to electromagnons.

cond-mat.mtrl-sci↗

arXiv2013

Far-infrared electrodynamics of thin superconducting NbN film in magnetic field

We studied a thin superconducting NbN film in magnetic fields up to 8 T above the zero- temperature limit by means of time-domain terahertz and scanning tunneling spectroscopies in order to understand the vortex response. Scanning tunneling spectroscopy was used to determine the optical gap and the upper critical field of the sample. The obtained values were subsequently used to fit the terahertz complex conductivity spectra in the magnetic field in the Faraday geometry above the zero temperature limit. These spectra are best described in terms of the Coffey-Clem self-consistent solution of a modified London equation in the flux creep regime.

cond-mat.supr-con↗

arXiv2004

High-temperature phase transitions in SrBi_2Ta_2O_9 film: a study by THz spectroscopy

Time-domain THz transmission experiment was performed on a $\rm SrBi_2Ta_2O_9$ film deposited on sapphire substrate. Temperatures between 300 and 923 K were investigated and complex permittivity spectra of the film were determined. The lowest frequency optic phonon near 28 cm$^{-1}$ reveals a slow monotonic decrease in frequency on heating with no significant anomaly near the phase transitions. We show that the dielectric anomaly near the ferroelectric phase transition can be explained by slowing down of a relaxational mode, observed in the THz spectra. A second harmonic generation signal observed in a single crystal confirms a loss of center of symmetry in the ferroelectric phase and a presence of polar clusters in the intermediate ferroelastic phase.

cond-mat.mtrl-sci↗