Self-organized Layered Structures of Nitrogen-Vacancy Centers with Preferential Orientation in Heteroepitaxial Diamond Films

Vadim Lebedev; Alejandro Martínez-Méndez; Jesús Moreno-Meseguer; Jan Engels; Jürgen Weippert; Jan Kustermann; Felix Hoffmann; Javier Prior; Jan Jeske

arXiv · 2610.03150

Self-organized Layered Structures of Nitrogen-Vacancy Centers with Preferential Orientation in Heteroepitaxial Diamond Films

Vadim Lebedev·Alejandro Martínez-Méndez·Jesús Moreno-Meseguer·Jan Engels·Jürgen Weippert·Jan Kustermann·Felix Hoffmann·Javier Prior·Jan Jeske

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Abstract

Here, we report the fabrication and characterization of single crystal diamond films on a two-inch wafer-scale containing three-dimensional layered structures of negatively charged nitrogen-vacancy color centers (NV$^{-}$). The (100)-oriented layered diamond films were grown by chemical vapor deposition (CVD) to create spatially separated regions of enhanced emission associated with NV$^{-}$ centers. Such localized emission enhancement as well as 2D and 3D arrays of spins could enable close-packed architectures for emerging quantum devices, such as data processors, memory cells, and magnetic sensors. A cyclic sequence of CVD growth and oxygen-plasma etching is employed, resulting in the in-situ formation of layered inverted pyramidal structures with flat $\{$111$\}$ sidewalls. These pits are subsequently overgrown by nitrogen-doped diamond to achieve NV$^{-}$-rich facets with a uniform N-V bond arrangement and improved nitrogen incorporation efficiency.

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BibTeX RIS

Vadim Lebedev, Alejandro Martínez-Méndez, Jesús Moreno-Meseguer, Jan Engels, Jürgen Weippert, Jan Kustermann, Felix Hoffmann, Javier Prior, Jan Jeske. 2026-10-02. Self-organized Layered Structures of Nitrogen-Vacancy Centers with Preferential Orientation in Heteroepitaxial Diamond Films. https://arxiv.org/abs/2610.03150

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