arXiv subjects

Jan Jeske

Publications and source records attributed to Jan Jeske.

At least 19 recordsLinked to original sources

arXiv2026

Characterizing the nitrogen-vacancy center singlet transition and its phonon sideband for absorption-based room-temperature magnetometry

Magnetometry with nitrogen-vacancy (NV) centers in diamond has shown great promise in recent years. In particular, absorption-based magnetometry techniques, employing a cavity to enhance the absorption length, can improve the contrast and sensitivity compared to conventional techniques based on reading out the NV$^-$ triplet fluorescence. The absorption techniques rely on magnetic-field-dependent absorption at the NV$^-$ singlet zero phonon line at 1042$\,$nm and its phonon sideband. In a cavity-enhanced spectroscopy approach, we study pump-laser- and microwave-induced cavity signal changes at room temperature over a spectral range of 680-1050$\,$nm. Through normalization, we eliminate the cavity-enhancement effect and provide quasi-single-pass values for the absorption and optically detected magnetic resonance (ODMR) contrast. The highest contrast is found at 1042$\,$nm, but multiple points of high contrast are found at the peaks of the phonon sideband. Additionally, cavity-enhanced ODMR contrasts in the range of 50-80$\,\%$ are presented. We further measure the broadband singlet absorption cross section at room temperature with a novel method through microwave-induced signal changes. This method is insensitive to pump-laser-induced signal changes by other defects and quantifies the room-temperature absorption strength of the singlet transition and its entire phonon sideband. We determine the absorption cross section at 1042$\,$nm to be $\sigma^{\,\bigstar}_{1042}=(0.89\pm0.14)\cdot 10^{-21}\,\text{m}^2$ or $\sigma^{\,\blacktriangle}_{1042}=(2.9\pm0.5)\cdot 10^{-21}\,\text{m}^2$. depending on the employed 532$\,$nm NV$^-$ absorption cross section.

quant-ph↗

arXiv2026

A robust laser cavity platform for NV-diamond singlet infrared absorption magnetometry

The negatively charged nitrogen-vacancy center (NV$^-$) in diamond is a versatile platform for quantum magnetometry under ambient conditions. Recently, laser threshold magnetometry (LTM) has been proposed as a means to significantly enhance the sensitivity of NV-based magnetometers by incorporating a diamond hosting NV$^-$ centers within a laser cavity and operating near threshold. While demonstrations have validated the concept, practical implementations remain technically demanding, requiring high pump powers and precise alignment of free-space cavities. It remains unclear whether the benefits of operating near threshold will outpace increased laser noise. In this work, we integrate an NV-diamond with a high NV$^-$ content into a compact external cavity diode laser and demonstrate singlet infrared absorption optically detected magnetic resonance (ODMR). The system exhibits exceptional threshold current stability, enabling ODMR using the threshold current as the read-out parameter. We report a five-fold enhancement in the ODMR contrast by operating near threshold. The best magnetic field sensitivity of $7.6~\mathrm{nT/\sqrt{Hz}}$ (DC-500 Hz) is achieved well above threshold, while near threshold sensitivity is limited by increased probe laser noise. These results establish a compact and mechanically robust platform for singlet absorption-based NV$^-$ magnetometry and highlight key trade-offs between contrast enhancement and laser noise near threshold.

quant-ph↗

arXiv2026

Quantum theory for phonon lasing and non-classical state generation in mixed-species and single trapped ions

In this article we present a comprehensive theoretical investigation of phonon lasing with mixed-species trapped ions, as demonstrated in [T. Behrle, Phys. Rev. Lett. 131 (2023)], employing both a semi-classical mean-field description and a full quantum theory. We derive an analytic expression for the second-order coherence function, confirming the experimental observation of the system's lasing behaviour above threshold. Building on the successful implementation of the two-ion lasing scheme, we propose a novel approach for achieving phonon lasing with a single trapped ion, offering significant experimental advantages and making the implementation of multiple phonon lasers within a single setup feasible. Furthermore, we explore lasing in a squeezed basis and in different regimes of the Lamb-Dicke approximation, highlighting the potential to produce non-classical states with promising applications in precision sensing. Our analysis of a sensing protocol based on squeezed states, using experimentally feasible parameters, shows a sensitivity enhancement of up to two orders of magnitude.

quant-ph↗

arXiv2025

Laser-enhanced quantum sensing boosts sensitivity and dynamic range

Magnetometers based on nitrogen-vacancy (NV) centers in diamond have emerged as the most important solid-state quantum sensors. However, ensembles are limited in optical contrast to typically a few percent and high-sensitivity variants usually possess only a few $\mathrm{\upmu}$T dynamic range. Here, we demonstrate a laser threshold magnetometry-based NV system that avoids these limitations. By integrating the NV centers into a laser cavity and showing magnetic-field-dependent shifts of the laser threshold, we observe 100\,\% optical contrast, i.\,e., we are able to entirely switch off the laser system with the NV centers magnetic resonance. At the same time we achieve strong output signals up to 50\,mW. The system exhibits a photon-shot-noise-limited (PSNL) sensitivity of $<$400\,fT/$\sqrt{\textrm{Hz}}$ for all vector components, which we demonstrate to improve super-linearly with contrast. The ratio of the sensing-relevant parameters PSNL sensitivity and dynamic range, that can be traded at the cost of each other, marks an improvement factor of up to 590 over typical fluorescence-based readout and vapor cell sensors while also adding vector magnetometry capabilities. Such performance improvements provide a perspective for a highly sensitive magnetometer, which could be operated outside a magnetically-shielded room. This could bring a new generation of sensors for applications including magnetoencephalography, magnetic navigation, and magnetic anomaly detection.

quant-ph↗

arXiv2025

The properties of the nitrogen-vacancy center in milled chemical vapor deposition nanodiamonds

Fluorescent nanodiamonds (FNDs) containing negatively charged nitrogen-vacancy (NV-) centers are vital for many emerging quantum sensing applications from magnetometry to intracellular sensing in biology. However, developing a scalable fabrication method for FNDs hosting color centers with consistent bulk-like photoluminescence (PL) and spin coherence properties remains a highly desired but unrealized goal. Here, we investigate optimized ball milling of single-crystal diamonds produced via chemical vapor deposition (CVD) and containing 2 ppm of substitutional nitrogen and 0.3 ppm of NV- to achieve this goal. The NV charge state, PL lifetime, and spin properties of bulk CVD diamond samples are directly compared to milled CVD FNDs and commercial high-pressure high-temperature (HPHT) FNDs. We find that on average, the relative contribution of the NV- charge state to the total NV PL is lower and the NV PL lifetime is longer in CVD FNDs compared to HPHT FNDs, both likely due to the lower Ns0 concentration in CVD FNDs. The CVD bulk and CVD FNDs on average show similar average T1 spin relaxation times of 3.2 $\pm$ 0.7 ms and 4.7 $\pm$ 1.6 ms, respectively, compared to 0.17 $\pm$ 0.01 ms for commercial HPHT FNDs. Our results demonstrate that ball milling of CVD diamonds enables the large-scale fabrication of NV ensembles in FNDs with bulk-like T1 spin relaxation properties.

cond-mat.mes-hall↗

arXiv2025

Two-media laser threshold magnetometry: A magnetic-field-dependent laser threshold

Nitrogen-vacancy (NV) centers in diamond are a promising platform for high-precision magnetometry. In contrast to the use of spontaneous emission in a number of NV-magnetometers, laser threshold magnetometry (LTM) exploits stimulated emission of NV centers by placing an NV-doped diamond inside an optical cavity. The NV laser system is predicted to reach a high magnetic-field-dependent contrast and coherent signal strength, leading to an improved magnetic field sensitivity combined with a high linearity. Here, we consider a two-media setup where the cavity additionally includes a vertical external cavity surface emitting laser. This optically active material compensates cavity losses at \SI{750}{nm} while still allowing for magnetic-field-dependent effects from the NV-diamond. We demonstrate a magnetic-field-dependent laser threshold and investigate the effects of pump laser induced absorption of the diamond. The experimental data is supported by an analytical simulation based on a rate model. Furthermore, we derive a generalized formula to compute the shot-noise-limited magnetic field sensitivity in the regime of high contrast yielding 49.07(33) pT/$\sqrt{\text{Hz}}$ for the present setup. Simulations with an optimized NV-diamond suggest that values down to 4.9 ft/$\sqrt{\text{Hz}}$ are possible.

physics.optics↗

arXiv2024

The $N_2V$ color center: a ubiquitous visible and near-infrared-II quantum emitter in nitrogen-doped diamond

Photoluminescent defects in diamond, like the nitrogen-vacancy (NV) color center, are at the forefront of emerging optical quantum technologies. Most emit in the visible and near-infrared spectral region below 1000 nm (NIR-I), limiting their applications in photonics, fiber communications, and biology. Here, we show that the nitrogen-vacancy-nitrogen ($N_2V$) center, which emits in the visible and near-infrared-II (NIR-II, 1000-1700 nm), is ubiquitous in as-synthesized and processed nitrogen-doped diamond from bulk samples to nanoparticles. We demonstrate that $N_2V$ is also present in commercially available state-of-the-art NV diamond sensing chips made via chemical vapor deposition (CVD). In high-pressure high-temperature (HPHT) diamonds, the photoluminescence (PL) intensity of both $N_2V$ charge states, $N_2V^0$ in the visible and $N_2V^-$ in the NIR-II, increases with increasing substitutional nitrogen concentration. We determine the PL lifetime of $N_2V^-$ to be 0.3 ns and compare a quantum optical and density functional theory model of the $N_2V^-$ with experimental PL spectra. Finally, we show that detonation nanodiamonds (DND) show stable PL in the NIR-II, which we attribute to the $N_2V$ color center, and use this NIR-II PL to image DNDs inside skin cells. Our results will contribute to the scientific and technological exploration and development of the $N_2V$ color center and inspire more research into its effect on other color centers in diamond.

cond-mat.mes-hall↗

arXiv2024

High-contrast absorption magnetometry in the visible to near-infrared range with nitrogen-vacancy ensembles

Magnetometry with nitrogen-vacancy (NV) centers has so far been measured via emission of light from NV centers or via absorption at the singlet transition at 1042 nm. Here, we demonstrate a phenomenon of broadband optical absorption by the NV centers starting in the emission wavelength and reaching up to 1000 nm. The measurements are enabled by a high-finesse cavity, which is used for room temperature continuous wave pump-probe experiments. The red to infrared probe beam shows the typical optically detected magnetic resonance (ODMR) signal of the NV spin with contrasts up to 42 %. This broadband optical absorption is not yet reported in terms of NV magnetometry. We argue that the lower level of the absorbing transition could be the energetically lower NV singlet state, based on the increased optical absorption for a resonant microwave field and the spectral behavior. Investigations of the photon-shot-noise-limited sensitivity show improvements with increasing probe wavelength, reaching an optimum of 7.5 pT/$\sqrt{\mathrm{Hz}}$. The results show significantly improved ODMR contrast compared to emission-based magnetometry. This opens a new detection wavelength regime with coherent laser signal detection for high-sensitivity NV magnetometry.

physics.app-ph↗

arXiv2024

Spin coherence in strongly coupled spin baths in quasi-two-dimensional layers

We investigate the spin-coherence decay of NV$^-$-spins interacting with the strongly-coupled bath of nitrogen defects in diamond layers. For thin diamond layers, we demonstrate that the spin-coherence times exceed those of bulk diamond, thus allowing to surpass the limit imposed by high defect concentrations in bulk. We show that the stretched-exponential parameter for the short-time spin-coherence decay is governed by the hyperfine interaction in the bath, thereby constraining random-noise models. We introduce a novel method based on the cluster-correlation expansion applied to strongly-interacting bath partitions. Our results facilitate material development for quantum-technology devices.

quant-ph↗

arXiv2023

Continuous-wave nitrogen-vacancy diamond laser system assisted by a red diode laser

Diamond has long been identified as a potential host material for laser applications. This potential arises due to its exceptional thermal properties, ultra-wide bandgap, and color centers which promise gain across the visible spectrum. More recently, coherent laser methods offer new approaches to magnetometry. However, diamond fabrication is difficult in comparison to other crystalline matrices, and many optical loss channels are not yet understood. Here, we demonstrate the first continuous-wave nitrogen-vacancy (NV) color center laser system. To achieve this, we constructed a laser cavity with both, an NV-diamond medium and an intra-cavity anti-reflection coated diode laser. This dual-medium approach compensates intrinsic losses of the cavity by providing a fixed additional gain below threshold of the diode laser. We observe the first clear continuous-wave laser threshold in the output of the laser system as well as linewidth narrowing with increasing green pump power on the NV centers. Our results are a major development towards coherent approaches to magnetometry.

quant-ph↗

arXiv2021

Proximal nitrogen reduces the fluorescence quantum yield of nitrogen-vacancy centres in diamond

The nitrogen-vacancy colour centre in diamond is emerging as one of the most important solid-state quantum systems. It has applications to fields including high-precision sensing, quantum computing, single photon communication, metrology, nanoscale magnetic imaging and biosensing. For all of these applications, a high quantum yield of emitted photons is desirable. However, diamond samples engineered to have high densities of nitrogen-vacancy centres show levels of brightness varying significantly within single batches, or even within the same sample. Here we show that nearby nitrogen impurities quench emission of nitrogen-vacancy centres via non-radiative transitions, resulting in a reduced fluorescence quantum yield. We monitored the emission properties of nitrogen-vacancy centre ensembles from synthetic diamond samples with different concentrations of nitrogen impurities. While at low nitrogen densities of 1.81 ppm we measured a lifetime of 13.9 ns, we observed a strong reduction in lifetime with increasing nitrogen density. We measure a lifetime as low as 4.4 ns at a nitrogen density of 380 ppm. The change in lifetime matches a reduction in relative fluorescence quantum yield from 77.4 % to 32 % with an increase in nitrogen density from 88 ppm to 380 ppm, respectively. These results will inform the conditions required to optimise the properties of diamond crystals devices based on the fluorescence of nitrogen-vacancy centres. Furthermore, this work provides insights into the origin of inhomogeneities observed in high-density nitrogen-vacancy ensembles within diamonds and nanodiamonds.

quant-ph↗

arXiv2021

Absorptive laser threshold magnetometry: combining visible diamond Raman lasers and nitrogen-vacancy centres

We propose a high-sensitivity magnetometry scheme based on a diamond Raman laser with visible pump absorption by an ensemble of coherently microwave driven negatively charged nitrogen-vacancy centres (NV) in the same diamond crystal. The NV centres' absorption and emission are spin-dependent. We show how the varying absorption of the NV centres changes the Raman laser output. A shift in the diamond Raman laser threshold and output occurs with the external magnetic-field and microwave driving. We develop a theoretical framework including steady-state solutions to describe the effects of coherently driven NV centres in a diamond Raman laser. We discuss that such a laser working at the threshold can be employed for magnetic-field sensing. In contrast to previous studies on NV magnetometry with visible laser absorption, the laser threshold magnetometry method is expected to have low technical noise, due to low background light in the measurement signal. For magnetic-field sensing, we project a shot-noise limited DC sensitivity of a few $\mathrm{pT}/\sqrt{\mathrm{Hz}}$ in a well-calibrated cavity with realistic parameters. This sensor employs the broad visible absorption of NV centres and unlike previous laser threshold magnetometry proposals it does not rely on active NV centre lasing or an infrared laser medium at the specific wavelength of the NV centre's infrared absorption line.

quant-ph↗

arXiv2019

Amplification by stimulated emission of nitrogen vacancy centres in a diamond-loaded fibre cavity

Laser-threshold magetometry using the negatively charged nitrogen-vacancy (NV-) centre in diamond as a gain medium has been proposed as a technique to dramatically enhance the sensitivity of room-temperature magnetometry. We experimentally explore a diamond-loaded open tunable fibre-cavity system as a potential contender for the realization of lasing with NV- centres. We observe amplification of the transmission of a cavity-resonant seed laser at 721 nm when the cavity is pumped at 532 nm, and attribute this to stimulated emission. Changes in the intensity of spontaneously emitted photons accompany the amplification, and a qualitative model including stimulated emission and ionisation dynamics of the NV- centre captures the dynamics in the experiment very well. These results highlight important considerations in the realization of an NV- laser in diamond.

quant-ph↗

arXiv2018

The effects of thermal and correlated noise on magnons in a quantum ferromagnet

The dynamics and thermal equilibrium of spin waves (magnons) in a quantum ferromagnet as well as the macroscopic magnetisation are investigated. Thermal noise due to an interaction with lattice phonons and the effects of spatial correlations in the noise are considered. We first present a Markovian master equation approach with analytical solutions for any homogeneous spatial correlation function of the noise. We find that spatially correlated noise increases the decay rate of magnons with low wave vectors to their thermal equilibrium, which also leads to a faster decay of the ferromagnet's magnetisation to its steady-state value. For long correlation lengths and higher temperature we find that additionally there is a component of the magnetisation which decays very slowly, due to a reduced decay rate of fast magnons. This effect could be useful for fast and noise-protected quantum or classical information transfer and magnonics. We further compare ferromagnetic and antiferromagnetic behaviour in noisy environments and find qualitatively similar behaviour in Ohmic but fundamentally different behaviour in super-Ohmic environments.

quant-ph↗

arXiv2016

Signatures of spatially correlated noise and non-secular effects in two-dimensional electronic spectroscopy

We investigate how correlated fluctuations affect oscillatory features in rephasing and non-rephasing two-dimensional (2D) electronic spectra of a model dimer system. Based on a beating map analysis, we show that non-secular environmental couplings induced by uncorrelated fluctuations lead to oscillations centered at both cross- and diagonal-peaks in rephasing spectra as well as in non-rephasing spectra. Using an analytical approach, we provide a quantitative description of the non-secular effects in terms of the Feynman diagrams and show that the environment-induced mixing of different inter-excitonic coherences leads to oscillations in the rephasing diagonal-peaks and non-rephasing cross-peaks. We demonstrate that as correlations in the noise increase, the lifetime of oscillatory 2D signals is enhanced at rephasing cross-peaks and non-rephasing diagonal-peaks, while the other non-secular oscillatory signals are suppressed. We discuss that the asymmetry of 2D lineshapes in the beating map provides information on the degree of correlations in environmental fluctuations. Finally we investigate how the oscillatory features in 2D spectra are affected by inhomogeneous broadening.

quant-ph↗

arXiv2016

Stimulated emission from NV centres in diamond

Stimulated emission is the process fundamental to laser operation, thereby producing coherent photon output. Despite negatively-charged nitrogen-vacancy (NV$^-$) centres being discussed as a potential laser medium since the 1980's, there have been no definitive observations of stimulated emission from ensembles of NV$^-$ to date. Reasons for this lack of demonstration include the short excited state lifetime and the occurrence of photo-ionisation to the neutral charge state by light around the zero-phonon line. Here we show both theoretical and experimental evidence for stimulated emission from NV$^-$ states using light in the phonon-sidebands. Our system uses a continuous wave pump laser at 532 nm and a pulsed stimulating laser that is swept across the phononic sidebands of the NV$^-$. Optimal stimulated emission is demonstrated in the vicinity of the three-phonon line at 700 nm. Furthermore, we show the transition from stimulated emission to photoionisation as the stimulating laser wavelength is reduced from 700nm to 620 nm. While lasing at the zero-phonon line is suppressed by ionisation, our results open the possibility of diamond lasers based on NV centres, tuneable over the phonon-sideband. This broadens the applications of NV magnetometers from single centre nanoscale sensors to a new generation of ultra-precise ensemble laser sensors, which exploit the contrast and signal amplification of a lasing system.

quant-ph↗

arXiv2016

Remote Nanodiamond Magnetometry

Optical fibres have transformed the way people interact with the world and now permeate many areas of science. Optical fibres are traditionally thought of as insensitive to magnetic fields, however many application areas from mining to biomedicine would benefit from fibre-based remote magnetometry devices. In this work, we realise such a device by embedding nanoscale magnetic sensors into tellurite glass fibres. Remote magnetometry is performed on magnetically active defect centres in nanodiamonds embedded into the glass matrix. Standard optical magnetometry techniques are applied to initialize and detect local magnetic field changes with a measured sensitivity of 26 micron Tesla/square root(Hz). Our approach utilizes straight-forward optical excitation, simple focusing elements, and low power components. We demonstrate remote magnetometry by direct reporting of the magnetic ground states of nitrogen-vacancy defect centres in the optical fibres. In addition, we present and describe theoretically an all-optical technique that is ideally suited to remote fibre-based sensing. The implications of our results broaden the applications of optical fibres, which now have the potential to underpin a new generation of medical magneto-endoscopes and remote mining sensors.

physics.optics↗

arXiv2016

Laser threshold magnetometry

We propose a new type of sensor, which uses diamond containing the optically active nitrogen-vacancy (NV$^-$) centres as a laser medium. The magnetometer can be operated at room-temperature and generates light that can be readily fibre coupled, thereby permitting use in industrial applications and remote sensing. By combining laser pumping with a radio-frequency Rabi-drive field, an external magnetic field changes the fluorescence of the NV$^-$ centres. We use this change in fluorescence level to push the laser above threshold, turning it on with an intensity controlled by the external magnetic field, which provides a coherent amplification of the readout signal with very high contrast. This mechanism is qualitatively different from conventional NV$^-$--based magnetometers which use fluorescence measurements, based on incoherent photon emission. We term our approach laser threshold magnetometry (LTM). We predict that an NV$^-$--based laser threshold magnetometer with a volume of 1mm$^3$ can achieve shot-noise limited d.c.~sensitivity of 1.86 fT$/\sqrt{\rm{Hz}}$ and a.c.~sensitivity of 3.97fT$/\sqrt{\rm{Hz}}$.

quant-ph↗