Searcharxiv⌕ Search

arXiv · 2610.38302

Finite-Temperature Magnetism and Longitudinal Spin Transport in Compensated Half-Metal Ferrimagnets with Near-Zero Magnetization

Abstract

Fully compensated ferrimagnets, characterized by nearly vanishing magnetic moments at zero temperature, perfect spin-polarized electronic structures, and ultrafast spin dynamics, represent a highly promising materials platform for next-generation spintronic devices. By minimizing stray magnetic fields and reducing switching currents, FCFs enable a viable path toward high-speed, low-power spintronic devices. In this work, we present a systematic investigation of the electronic structure, finite-temperature magnetism, and spin-dependent transport properties of the Heusler-type fully compensated half-metallic ferrimagnet Mn3Al in magnetic tunnel junctions. We demonstrate that Mn3Al is a half-metallic FCF with 100% spin polarization and fully compensated magnetization at 0 K. Combining density functional theory with Monte Carlo simulations, we characterize its finite-temperature magnetic properties and show that Mn3Al exhibits a net magnetization below 11.6 emu/cc at 300 K, confirming the robustness of its nearly compensated ferrimagnetic order at room temperature. Furthermore, we predict that the Mn3Al/MgO/Mn3Al MTJ yields a giant tunneling magnetoresistance effect at 0 K, which remains as high as 232% at 300 K. Our results establish Mn3Al and related half-metallic FCFs as excellent candidates for magnetoresistance-based spintronic applications.

Explore related subjects

Keep this discovery

Explore connections, maps & timelines

BibTeXRIS

Jiahao Shentu, Jie Li, Jianting Dong, Meng Zhu, Chen Wang, Qing Zhang, Yizhuo Song, Wenqi Sun, Jia Zhang. 2026-10-28. Finite-Temperature Magnetism and Longitudinal Spin Transport in Compensated Half-Metal Ferrimagnets with Near-Zero Magnetization. https://arxiv.org/abs/2610.38302

Cite the original work for its findings. Save a collection to share your selection of sources.

KEEP EXPLORING

Related papers

Dynamic Peach-Koehler self-force, inertia, and radiation damping of a regularized dislocation

The elastodynamic Peach-Koehler force is computed for a fully-regularized straight dislocation with isotropic core in continuum isotropic elastic elasticity, in compact forms involving partial mass or impulsion functions relative to shear and compressional waves. The force accounts for both dynamic radiation damping and inertia. The expressions are valid indifferently for subsonic or supersonic velocities. Results are compared with the case of a flat-core dislocation of the Peierls-Eshelby type, for a motion of jump from rest to constant velocity. In the steady-state limit, the Lagrangian function relevant to expressing the force in the flat-core case must be replaced by a related but different function for the regularized dislocation. However, by suitably defining the regularizing dislocation width, the steady-state limits of the force for the fully-regularized and flat-core dislocations can be matched exactly.

cond-mat.mtrl-sci↗

LightPFP: A Lightweight Route to Ab Initio Accuracy at Scale

Machine learning interatomic potentials (MLIPs) bridge the gap between quantum-mechanical accuracy and scalable molecular simulations. However, a fundamental trade-off persists: universal MLIPs (u-MLIPs) offer broad transferability but are computationally expensive, whereas task-specific MLIPs (ts-MLIPs) achieve high efficiency at the expense of costly DFT training data. Here we introduce LightPFP, a data-efficient knowledge distillation framework. Instead of relying on expensive DFT calculations, LightPFP constructs a distilled ts-MLIP by using a u-MLIP to generate high-quality, material-specific training data, while employing a pre-trained lightweight model to further improve data efficiency. Across diverse material systems, LightPFP reduces model development time by approximately three orders of magnitude compared with DFT-based workflows, while maintaining DFT-level accuracy. Combined with a LAMMPS/Kokkos inference backend, LightPFP achieves more than three orders of magnitude higher inference efficiency than u-MLIP baselines while enabling simulations of systems thousands of times larger. When the teacher exhibits systematic bias, LightPFP supports few-shot precision correction using as few as 10 high-accuracy DFT configurations, as demonstrated by reproducing MgO's experimental melting point. This u-MLIP-driven distillation establishes a scalable route to high-fidelity, data-efficient MLIPs, accelerating the pace of materials discovery and design.

cond-mat.mtrl-sci↗

First-order polarization process as an alternative to antiferroelectricity

Antiferroelectrics generate significant interest since their polarization versus electric field (P-E) curves show typical double-hysteresis loops appealing for various applications. Unfortunately, antiferroelectrics are rare. In magnetic compounds, magnetization versus magnetic field (M-H) curves can show analogous double hysteresis loops not only in antiferromagnets but also in systems exhibiting field-induced first-order reorientation of the magnetization through a so-called first-order magnetization process. Here, we show that appealing double-hysteresis P-E loops can also appear from an unprecedented first-order polarization process. Focusing on non-polar CaTiO3, which can be turned ferroelectric under tensile strain, we study epitaxial thin films on differently-oriented NdGaO3 substrates using a combination of theoretical and experimental techniques. We uncover that a certain configuration exhibits double-hysteresis P-E loops that we rationalize from a field-induced abrupt rotation of the polarization. Such a first-order polarization process establishes a promising alternative pathway to achieve double hysteresis P-E loops appealing for practical applications.

cond-mat.mtrl-sci↗