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Evidence of quantum criticality in the doped Haldane system Y2BaNiO5

C. Payen·E. Janod·K. Schoumacker·C. D. Batista·K. Hallberg·A. A. Aligia
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Abstract

Experimental bulk susceptibility X(T) and magnetization M(H,T) of the S=1-Haldane chain system doped with nonmagnetic impurities, Y2BaNi1-xZnxO5 (x=0.04,0.06,0.08), are analyzed. A numerical calculation for the low-energy spectrum of non-interacting open segments describes very well experimental data above 4 K. Below 4 K, we observe power-law behaviors, X(T)=T^-alpha and M(H,T)/T^(1-alpha)=f(alpha,(H/T)), with alpha (<1) depending on the doping concentration x.This observation suggests the appearance of a gapless quantum phase due to a broad distribution of effective couplings between the dilution-induced moments.

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C. Payen, E. Janod, K. Schoumacker, C. D. Batista, K. Hallberg, A. A. Aligia. 2000-03-09. Evidence of quantum criticality in the doped Haldane system Y2BaNiO5. https://doi.org/10.1103/physrevb.62.2998

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