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Thermal relaxation in charge ordered Pr$_{0.63}$ Ca$_{0.37}$ MnO$_3$ in presence of a magnetic field

A. K. Raychaudhuri·Ayan Guha·I. Das·R. Rawat·C. N. R. Rao
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Abstract

We report observation of substantial thermal relaxation in single crystal of charge ordered system Pr$_{0.63}$Ca$_{0.37}$MnO$_3$ in an applied magnetic field of H = 8T. The relaxation is observed when the temperature is scanned in presence of a magnetic field in the temperature interval $T_{MH}<T<T_{CO}$ where $T_{CO}$ is the charge ordering temperature and $T_{MH}$ is charge melting temperature in a field. In this temperature range the system has coexisting charged ordered insulator (COI) and ferromagnetic metallic (FMM) phases. No such relaxation is observed in the COI state in H = 0T or in the FMM phase at $T < T_{MH}$ in presence of a magnetic field. We conclude that the thermal relaxation is due to two coexisting phases with nearly same free energies but separated by a potential barrier. This barrier makes the transformation from one phase to the other time-dependent in the scale of the specific heat experiment and gives rise to the thermal relaxation.

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A. K. Raychaudhuri, Ayan Guha, I. Das, R. Rawat, C. N. R. Rao. 2001-05-23. Thermal relaxation in charge ordered Pr$_{0.63}$ Ca$_{0.37}$ MnO$_3$ in presence of a magnetic field. https://doi.org/10.1016/s0038-1098(01)00332-5

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