arXiv · cond-mat/0104188
Photon Counting Statistics for Single Molecule Spectroscopy
Abstract
We present a general relation between Mandel's $Q$ parameter describing variance of number of photons emitted from a single molecule and a three time correlation function describing a spectral diffusion process the molecule is undergoing. For a prototype of such a stochastic process an exact solution is found which exhibits rich types of physical behaviors.
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Eli Barkai, YounJoon Jung, Robert Silbey. 2001-04-11. Photon Counting Statistics for Single Molecule Spectroscopy. https://arxiv.org/abs/cond-mat/0104188
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