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Impurity-Induced Antiferromagnetic Ordering in the Spin Gap System TlCuCl_3

A. Oosawa·T. Ono·H. Tanaka
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Abstract

The magnetization measurements have been performed on the doped spin gap system TlCu_{1-x}Mg_xCl_3 with x <= 0.025. The parent compound TlCuCl_3 is a three-dimensional coupled spin dimer system with the excitation gap Delta/k_B = 7.7 K. The impurity-induced antiferromagnetic ordering was clearly observed. The easy axis lies in the (0,1,0) plane. It was found that the transition temperature increases with increasing Mg^{2+} concentration x, while the spin-flop transition field is almost independent of x. The magnetization curve suggests that the impurity-induced antiferromagnetic ordering coexists with the spin gap for x <= 0.017.

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A. Oosawa, T. Ono, H. Tanaka. 2002-07-29. Impurity-Induced Antiferromagnetic Ordering in the Spin Gap System TlCuCl_3. https://doi.org/10.1103/physrevb.66.020405

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