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Clear Experimental Signature of Charge-Orbital density wave in Nd$_{1-x}$Ca$_{1+x}$MnO$_{4}$

Sher Alam·A. T. M. N. Islam·T. Nagai·M. Xu·Y. Matsui·I. Tanaka
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Abstract

Single Crystals of Nd$_{1-x}$Ca$_{1+x}$MnO$_{4}$ have been prepared by the travelling floating-zone method, and possible evidence of a charge -orbital density wave in this material presented earlier [PRB68,092405 (2003)] using High Resolution Electron Microscopy [HRTEM] and Electron Diffraction [ED]. In the current note we present direct evidence of charge-orbital ordering in this material using heat capacity measurements. Our heat capacity measurements indicate a clear transition consistent with prior observation. We find two main transitions, one at temperature $T_{_H}=310-314$ K, and other at $T_{_A}=143$ K. In addition, we may also conclude that there is a strong electron-phonon coupling in this material.

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Sher Alam, A. T. M. N. Islam, T. Nagai, M. Xu, Y. Matsui, I. Tanaka. 2005-09-29. Clear Experimental Signature of Charge-Orbital density wave in Nd$_{1-x}$Ca$_{1+x}$MnO$_{4}$. https://doi.org/10.1103/physrevb.75.205134

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