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Magnetic ordering in Gd2Sn2O7: the archetypal Heisenberg pyrochlore antiferromagnet

A. S. Wills·M. E. Zhitomirsky·B. Canals·J. P. Sanchez·P. Bonville·P. Dalmas de Reotier·A. Yaouanc
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Abstract

Low-temperature powder neutron diffraction measurements are performed in the ordered magnetic state of the pyrochlore antiferromagnet Gd2Sn2O7. Symmetry analysis of the diffraction data indicates that this compound has the ground state predicted theoretically for a Heisenberg pyrochlore antiferromagnet with dipolar interactions. The difference in magnetic structures of Gd2Sn2O7 and of nominally analogous Gd2Ti2O7 is found to be determined by a specific type of third-neighbor superexchange interaction on the pyrochlore lattice between spins across empty hexagons.

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A. S. Wills, M. E. Zhitomirsky, B. Canals, J. P. Sanchez, P. Bonville, P. Dalmas de Reotier, A. Yaouanc. 2006-02-06. Magnetic ordering in Gd2Sn2O7: the archetypal Heisenberg pyrochlore antiferromagnet. https://doi.org/10.1088/0953-8984%2F18%2F3%2Fl02

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