arXiv subjects

B. Canals

Publications and source records attributed to B. Canals.

At least 19 recordsLinked to original sources

arXiv2025

Amp\`ere phase in frustrated magnets

We report a new class of algebraic spin liquids, in which the macroscopically degenerate ground state manifold is not Coulombic, like in spin ices, but Amp\`ere-like. The local constraint characterizing an Amp\`ere phase is not a Gauss law, but rather an Amp\`ere law, i.e., a condition on the curl of the magnetization vector field and not on its divergence. As a consequence, the excitations evolving in such a manifold are not magnetically charged scalar quasiparticles, the so-called magnetic monopoles in Coulomb phases, but instead vectorial magnetic loops (or fictional current lines). We demonstrate analytically that in a macroscopically degenerate manifold inheriting the properties of a cooperative paramagnet and subject to a local curl-free contraint, magnetic correlations decay in space with a power law whose exponent is the space dimension d: the Amp\`ere phase is a d-algebraic spin liquid. Using Monte Carlo simulations with appropriate cluster dynamics, we confirm this physics numerically in two- and three-dimensional examples, and illustrate how the Amp\`ere phase compares to its Coulomb counterpart.

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arXiv2023

Effective interaction quenching in artificial kagom\'e spin chains

Achieving thermal equilibrium in two-dimensional lattices of interacting nanomagnets has been a key issue on the route to study exotic phases in artificial frustrated magnets. We revisit this issue in artificial one-dimensional kagom\'e spin chains. Imaging arrested micro-states generated by a field demagnetization protocol and analyzing their pairwise spin correlations in real space, we unveil a non-equilibrated physics. Remarkably, this physics can be reformulated into an at-equilibrium one by rewriting the associated spin Hamiltonian in such a way that one of the coupling constants is quenched. We ascribe this effective behavior to a kinetic hinderance during the demagnetization protocol, which induces the formation of local flux closure spin configurations that sometimes compete with the magnetostatic interaction.

cond-mat.dis-nn↗

arXiv2023

Corrugation in a molecular C60 monolayer as a frustrated magnet

Under certain experimental conditions, the deposition of C60 molecules onto an atomically flat copper surface gives rise to the formation of corrugated islands. This corrugation, which reflects a molecular displacement perpendicular to the surface plane, presents an astonishing pattern: it is well described by a frustrated Ising spin Hamiltonian whose thermodynamics is compatible with a spin liquid about to transit towards an ordered zigzag state. Here we study the statistical properties of such a molecular corrugation using tools generally employed in frustrated magnetism. More specifically, the real and reciprocal space analysis of pairwise molecule correlations allows us to demonstrate that the C60/Cu system, in which magnetism is totally absent, has all the characteristics of a triangular Ising antiferromagnet. Our results indicate that the organization of two-dimensional matter, at the molecular length scale, sometimes turns out to be particularly close to that encountered in highly frustrated magnets.

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arXiv2020

Signatures of long range dipolar interactions in artificial square ice

Analyzing the magnetic structure factor of a field demagnetized artificial square ice, qualitative deviations from what would predict the square ice model are observed. Combining micromagnetic and Monte Carlo simulations, we demonstrate that these deviations signal the presence of interactions between nanomagnets that extend beyond nearest neighbors. Including further neighbor, dipolar-like couplings in the square ice model, we find that the first seven or eight coupling strengths are needed to reproduce semi-quantitatively the main features of the magnetic structure factor measured experimentally. An alternative, more realistic numerical scenario is also proposed in which the ice condition is slightly detuned. In that case as well, the features evidenced in the experimental magnetic structure factor are only well-described when further neighbor couplings are taken into account. Our results show that long range dipolar interactions are not totally washed out in a field demagnetized artificial square ice, and cannot be neglected as they impact the magnetic correlations within or at the vicinity of the ice manifold.

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arXiv2019

Artificial vertex systems by design

Arrays of interacting magnetic nanostructures were introduced recently as a powerful approach to investigate experimentally the exotic many-body physics of frustrated spin models. Following a similar strategy based on lithographically-patterned magnetic lattices, we provide a first attempt to fabricate a lab-on-chip platform to explore the physics of vertex models. The central idea of this work is to replace the spin degree of freedom of artificial frustrated spin systems by a local micromagnetic knob, which can be finely tuned by a proper design of the vertex geometry. This concept is demonstrated both numerically and experimentally on the celebrated six vertex model, and we show how all variants of this model can be apprehended through the engineering of magnetic square lattices. Our results open new avenues to design arrays of magnetic nanostructures not only to study a wide range of frustrated spin models, but to explore vertex models as well.

cond-mat.mes-hall↗

arXiv2017

Topological quantum phase transition in the Ising-like antiferromagnetic spin chain BaCo$_2$V$_2$O$_8$

Since the seminal ideas of Berezinskii, Kosterlitz and Thouless, topological excitations are at the heart of our understanding of a whole novel class of phase transitions. In most of the cases, those transitions are controlled by a single type of topological objects. There are however some situations, still poorly understood, where two dual topological excitations fight to control the phase diagram and the transition. Finding experimental realization of such cases is thus of considerable interest. We show here that this situation occurs in BaCo$_2$V$_2$O$_8$, a spin-1/2 Ising-like quasi-one dimensional antiferromagnet when subjected to a uniform magnetic field transverse to the Ising axis. Using neutron scattering experiments, we measure a drastic modification of the quantum excitations beyond a critical value of the magnetic field. This quantum phase transition is identified, through a comparison with theoretical calculations, to be a transition between two different types of solitonic topological objects, which are captured by different components of the dynamical structure factor.

cond-mat.str-el↗

arXiv2017

Competing interactions in artificial spin chains

The low-energy magnetic configurations of artificial frustrated spin chains are investigated using magnetic force microscopy and micromagnetic simulations. Contrary to most studies on two-dimensional artificial spin systems where frustration arises from the lattice geometry, here magnetic frustration originates from competing interactions between neighboring spins. By tuning continuously the strength and sign of these interactions, we show that different magnetic phases can be stabilized. Comparison between our experimental findings and predictions from the one-dimensional Anisotropic Next-Nearest-Neighbor Ising (ANNNI) model reveals that artificial frustrated spin chains have a richer phase diagram than initially expected. Besides the observation of several magnetic orders and the potential extension of this work to highly-degenerated artificial spin chains, our results suggest that the micromagnetic nature of the individual magnetic elements allows observation of metastable spin configurations.

cond-mat.mes-hall↗

arXiv2017

Magnetic charge injection in spin ice: a new way to fragmentation

The complexity embedded in condensed matter fertilizes the discovery of new states of matter, enriched by ingredients like frustration. Illustrating examples in magnetic systems are Kitaev spin liquids, skyrmions phases, or spin ices. These unconventional ground states support exotic excitations, for example the magnetic charges in spin ices, also called monopoles. Beyond their discovery, an important challenge is to be able to control and manipulate them. Here, we propose a new mechanism to inject monopoles in a spin ice through a staggered magnetic field. We show theoretically, and demonstrate experimentally in the Ho$_2$Ir$_2$O$_7$ pyrochlore iridate, that it results in the stabilization of a monopole crystal, which exhibits magnetic fragmentation. In this new state of matter, the magnetic moment fragments into an ordered part and a persistently fluctuating one. Compared to conventional spin ices, the different nature of the excitations in this fragmented state opens the way to novel tunable field-induced and dynamical behaviors.

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arXiv2017

Field driven magnetostructural transitions in GeCo$_2$O$_4$

In the spinel compound GeCo$_2$O$_4$, the Co$^{2+}$ pyrochlore sublattice presents remarkable magnetic field-induced behaviors that we unveil through neutron and X-ray single-crystal diffraction. The Néel ordered magnetic phase is entered through a structural lowering of the cubic symmetry. In this phase, when a magnetic field is applied along a 2-fold cubic direction, a spin-flop transition of one fourth of the magnetic moments releases the magnetic frustration and triggers magnetostructural effects. At high field, these ultimately lead to an unusual spin reorientation associated to structural changes.

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arXiv2016

Observation of magnetic fragmentation in spin ice

Fractionalised excitations that emerge from a many body system have revealed rich physics and concepts, from composite fermions in two-dimensional electron systems, revealed through the fractional quantum Hall effect, to spinons in antiferromagnetic chains and, more recently, fractionalisation of Dirac electrons in graphene and magnetic monopoles in spin ice. Even more surprising is the fragmentation of the degrees of freedom themselves, leading to coexisting and a priori independent ground states. This puzzling phenomenon was recently put forward in the context of spin ice, in which the magnetic moment field can fragment, resulting in a dual ground state consisting of a fluctuating spin liquid, a so-called Coulomb phase, on top of a magnetic monopole crystal. Here we show, by means of neutron scattering measurements, that such fragmentation occurs in the spin ice candidate Nd$_2$Zr$_2$O$_7$. We observe the spectacular coexistence of an antiferromagnetic order induced by the monopole crystallisation and a fluctuating state with ferromagnetic correlations. Experimentally, this fragmentation manifests itself via the superposition of magnetic Bragg peaks, characteristic of the ordered phase, and a pinch point pattern, characteristic of the Coulomb phase. These results highlight the relevance of the fragmentation concept to describe the physics of systems that are simultaneously ordered and fluctuating.

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arXiv2016

Ground-State Candidate for the Dipolar Kagome Ising Antiferromagnet

We have investigated the low-temperature thermodynamic properties of the dipolar kagome Ising antiferromagnet using at-equilibrium Monte Carlo simulations, in the quest for the ground-state manifold. In spite of the limitations of a single spin-flip approach, we managed to identify certain ordering patterns in the low-temperature regime and we propose a candidate for this unknown state. This novel configuration presents some intriguing features and passes several test-criteria, making it a very likely choice for the dipolar long-range order of this kagome Ising antiferromagnet.

cond-mat.dis-nn↗

arXiv2015

Longitudinal and Transverse Zeeman Ladders in the Ising-Like Chain Antiferromagnet BaCo2V2O8

We explore the spin dynamics emerging from the Néel phase of the chain compound antiferromagnet BaCo2V2O8. Our inelastic neutron scattering study reveals unconventional discrete spin excitations, so called Zeeman ladders, understood in terms of spinon confinement, due to the interchain attractive linear potential. These excitations consist in two interlaced series of modes, respectively with transverse and longitudinal polarization. The latter have no classical counterpart and are related to the zero-point fluctuations that weaken the ordered moment in weakly coupled quantum chains. Our analysis reveals that BaCo2V2O8, with moderate Ising anisotropy and sizable interchain interactions, remarkably fulfills the conditions necessary for the observation of these longitudinal excitations.

cond-mat.str-el↗

arXiv2015

Neutron diffraction investigation of the H-T phase diagram above the longitudinal incommensurate phase of BaCo2V2O8

The quasi-one-dimensional antiferromagnetic Ising-like compound BaCo2V2O8 has been shown to be describable by the Tomonaga-Luttinger liquid theory in its gapless phase induced by a magnetic field applied along the Ising axis. Above 3.9 T, this leads to an exotic field-induced low-temperature magnetic order, made of a longitudinal incommensurate spin-density wave, stabilized by weak interchain interactions. By single-crystal neutron diffraction we explore the destabilization of this phase at a higher magnetic field. We evidence a transition at around 8.5 T towards a more conventional magnetic structure with antiferromagnetic components in the plane perpendicular to the magnetic field. The phase diagram boundaries and the nature of this second field-induced phase are discussed with respect to previous results obtained by means of nuclear magnetic resonance and electron spin resonance, and in the framework of the simple model based on the Tomonaga-Luttinger liquid theory, which obviously has to be refined in this complex system.

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arXiv2015

Spin dynamics in the presence of competing ferro- and antiferro-magnetic correlations in Yb2Ti2O7

In this work, we show that the zero field excitation spectra in the quantum spin ice candidate pyrochlore compound \ybti\ is a continuum characterized by a very broad and almost flat dynamical response which extends up to $1-1.5$ meV, coexisting or not with a quasi-elastic response depending on the wave-vector. The spectra do not evolve between 50 mK and 2 K, indicating that the spin dynamics is only little affected by the temperature in both the short-range correlated and ordered regimes. Although classical spin dynamics simulations qualitatively capture some of the experimental observations, we show that they fail to reproduce this broad continuum. In particular, the simulations predict an energy scale twice smaller than the experimental observations. This analysis is based on a careful determination of the exchange couplings, able to reproduce both the zero field diffuse scattering and the spin wave spectrum rising in the field polarized state. According to this analysis, \ybti\ lies at the border between a ferro and an antiferromagnetic phase. These results suggest that the unconventional ground state of \ybti\ is governed by strong quantum fluctuations arising from the competition between those phases. The observed spectra may correspond to a continuum of deconfined spinons as expected in quantum spin liquids.

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arXiv2014

Kinetic pathways to the magnetic charge crystal in artificial dipolar spin ice

We investigate experimentally magnetic frustration effects in thermally active artificial kagome spin ice. Starting from a paramagnetic state, the system is cooled down below the Curie temperature of the constituent material. The resulting magnetic configurations show that our arrays are locally brought into the so-called spin ice 2 phase, predicted by at-equilibrium Monte Carlo simulations and characterized by a magnetic charge crystal embedded in a disordered kagome spin lattice. However, by studying our arrays on a larger scale, we find unambiguous signature of an out-of-equilibrium physics. Comparing our findings with numerical simulations, we interpret the efficiency of our thermalization procedure in terms of kinetic pathways that the system follows upon cooling and which drive the arrays into degenerate low-energy manifolds that are hardly accessible otherwise.

cond-mat.mes-hall↗

arXiv2014

Non-universality of artificial frustrated spin systems

Magnetic frustration effects in artificial kagome arrays of nanomagnets with out-of-plane magnetization are investigated using Magnetic Force Microscopy and Monte Carlo simulations. Experimental and theoretical results are compared to those found for the artificial kagome spin ice, in which the nanomagnets have in-plane magnetization. In contrast with what has been recently reported, we demonstrate that long range (i.e. beyond nearest-neighbors) dipolar interactions between the nanomagnets cannot be neglected when describing the magnetic configurations observed after demagnetizing the arrays using a field protocol. As a consequence, there are clear limits to any universality in the behavior of these two artificial frustrated spin systems. We provide arguments to explain why these two systems show striking similarities at first sight in the development of pairwise spin correlations.

cond-mat.mes-hall↗

arXiv2014

Far from equilibrium monopole dynamics in spin ice

Condensed matter in the low temperature limit reveals much exotic physics associated with unusual orders and excitations, examples ranging from helium superfluidity to magnetic monopoles in spin ice. The far-from-equilibrium physics of such low temperature states may be even more exotic, yet to access it in the laboratory remains a challenge. Here we demonstrate a simple and robust technique, the 'magnetothermal avalanche quench', and its use in the controlled creation of nonequilibrium populations of magnetic monopoles in spin ice at millikelvin temperatures. These populations are found to exhibit spontaneous dynamical effects that typify far-from-equilibrium systems, yet are captured by simple models. Our method thus opens the door to the study of far-from-equilibrium states in spin ice and other exotic magnets.

cond-mat.str-el↗

arXiv2014

Energy levels of interacting curved nano-magnets in a frustrated geometry: increasing accuracy when using finite difference methods

The accuracy of finite difference methods is related to the mesh choice and cell size. Concerning the micromagnetism of nano-objects, we show here that discretization issues can drastically affect the symmetry of the problem and therefore the resulting computed properties of lattices of interacting curved nanomagnets. In this paper, we detail these effects for the multiaxe kagome lattice. Using the Oommf finite difference method, we propose an alternative way of discretizing the nanomagnet shape via a variable moment per cell scheme. This method is shown to be efficient in reducing discretization effects.

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