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Beta-NMR of Isolated Lithium in Nearly Ferromagnetic Palladium

T. J. Parolin·Z. Salman·J. Chakhalian·Q. Song·K. H. Chow·M. D. Hossain·T. A. Keeler·R. F. Kiefl·S. R. Kreitzman·C. D. P. Levy·R. I. Miller·G. D. Morris·M. R. Pearson·H. Saadaoui·D. Wang·W. A. MacFarlane
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Abstract

The temperature dependence of the frequency shift and spin-lattice relaxation rate of isolated, nonmagnetic Li-8 impurities implanted in a nearly ferromagnetic host (Pd) are measured by means of beta-detected nuclear magnetic resonance (b-NMR). The shift is negative, very large and increases monotonically with decreasing T in proportion to the bulk susceptibility of Pd for T > T*~ 100 K. Below T*, an additional shift occurs which we attribute to the response of Pd to the defect. The relaxation rate is much slower than expected for the large shift and is linear with T below T*, showing no sign of additional relaxation mechanisms associated with the defect.

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T. J. Parolin, Z. Salman, J. Chakhalian, Q. Song, K. H. Chow, M. D. Hossain, T. A. Keeler, R. F. Kiefl, S. R. Kreitzman, C. D. P. Levy, R. I. Miller, G. D. Morris, M. R. Pearson, H. Saadaoui, D. Wang, W. A. MacFarlane. 2007-01-17. Beta-NMR of Isolated Lithium in Nearly Ferromagnetic Palladium. https://doi.org/10.1103/physrevlett.98.047601

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