Change of 7Be decay rate in exohedral and endohedral C60 fullerene compounds and its implications

Abstract

The half-life of 7Be implanted in a C60 pellet and gold foil has been measured to be about the same within about 0.2%. Using a radiochemical technique, we also measured that the probability of formation of endohedral 7Be@C60 by nuclear implantation technique was (5.6+-0.45)%. It is known from earlier works that the half-life of endohedral 7Be@C60 is about 1.2% shorter than that of 7Be implanted in gold. An analysis of these results using linear muffin-tin orbital method calculations indicates that most of the implanted 7Be ions in fullerene C60 stay at a distance of about 5.3 Angstrom from the centers of nearest C60 molecules forming exohedral compounds and those who enter the fullerene cages go to the centers of the cages forming endohedral 7Be@C60 compounds.