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N. Madhavan

Publications and source records attributed to N. Madhavan.

11 recordsLinked to original sources

Determining the dynamic deformation of $^{140}$Ce by constraining coupled-channels parameters for fusion

We present a systematic study of the dynamic deformation of 140Ce using 16O and 36S projectiles in heavy-ion fusion reactions, combining experimental data, a Gaussian analytic-barrier framework and coupled-channels calculations. Fusion cross sections for 16O+140Ce are measured from ~17% above to ~12.4% below the Bass barrier. Fusion data for 36S+140Ce are obtained from the literature. Deformation parameters of 140Ce are extracted via chi-square minimization and Bayesian analysis, with independent Bayesian Model Averaging yielding beta_2 = 0.09 +/- 0.03 and beta_3 = 0.18 +/- 0.02, consistent across both systems. The extracted parameters are tested in the 28Si+140Ce system, where coupled-channels calculations including transfer of a pair of neutrons (2n) reproduce both the fusion excitation function and the barrier distribution. The positive Q-value 2n-pickup channel enhances fusion in this reaction, while the projectile's vibrational or rotational nature results in similar structure of the barrier distribution. This study demonstrates that the Gaussian analytic recipe is quite effective in deriving the fusion barrier distribution which proves to be a sensitive probe of intrinsic nuclear deformation. Further, coupled-channels analysis across multiple systems ensures robustness of the extracted deformation parameters.

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First results of evaporation residue cross-section measurements of $^{32}$S+$^{208}$Pb system

The dynamics of heavy ion-induced reactions play a critical role in forming super heavy elements (SHE), and one clear signature of the SHE formation is the evaporation residue (ER). In our pursuit of SHE, we present the heaviest element populated in India for ER cross-section measurements. These are the first-ever measurements of the Evaporation Residue (ER) cross-sections for the nuclear reactions between $^{32}$S and $^{208}$Pb. These measurements were conducted above the Coulomb barrier at four distinct beam energies in the laboratory frame, ranging from 176 to 191 MeV at the pelletron Linac facility at the Inter-University Accelerator Centre (IUAC), New Delhi. The Hybrid Recoil Mass Analyzer (HYRA) in a gas-filled mode was employed for these experiments. The obtained range of ER cross-sections enriches our knowledge and helps advance the field of heavy ion-induced reactions, especially in the context of super heavy element formation.

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Determination of $1p$ and $2p$ stripping excitation functions for $^{16}$O+$^{142}$Ce using a Recoil Mass Spectrometer

We report the first direct measurement of differential transfer cross sections using a Recoil Mass Spectrometer. Absolute differential $1p$ and $2p$-stripping cross sections at $θ_\mathrm{c.m.}=180^\circ$ have been determined for the system $^{16}$O+$^{142}$Ce by detecting the heavier target-like ions at the focal plane of the Heavy Ion Reaction Analyzer. Focal plane spectra have been compared with the results of a semi-microscopic Monte-Carlo simulation to unambiguously identify the transfer channels. Transmission efficiency of the target-like ions through the spectrometer has also been estimated using the simulation. The methodology adopted in this work can be applied to other recoil separators. The measured excitation functions for the reactions $^{142}\mathrm{Ce(}^{16}\mathrm{O,}^{15}\mathrm{N)}^{143}\mathrm{Pr}$ and $^{142}\mathrm{Ce(}^{16}\mathrm{O,}^{14}\mathrm{C)}^{144}\mathrm{Nd}$ have been compared with coupled reaction channel calculations. An excellent matching between measurement and theory has been obtained. For $1p$-stripping, major contribution to the cross section has been found to be the transfer of a proton from $^{16}\mathrm{O}$ to the $2d_{\frac{5}{2}}$ excited state of $^{143}\mathrm{Pr}$, leaving behind $^{15}\mathrm{N}$ in the $1p_{\frac{1}{2}}$ ground state. Transfer of a cluster of two protons from $^{16}\mathrm{O}$ to the $2^{+}$ excited state of $^{144}\mathrm{Nd}$, resulting in $^{14}\mathrm{C}$ in the $0^{+}$ ground state, appears to be the most probable cause for $2p$-stripping. Measured transfer probabilities for $1p$ and $2p$ channels have been compared with Time-Dependent Hartree-Fock calculations. Proton stripping channels are found to be more favourable compared to neutron pick-up channels. However, the theory overpredicts measurement hinting at the need for extended approaches with explicit treatment of pairing correlations in the calculations.

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Search for stabilizing effects of $\bm{Z=82}$ shell closure against fission

Presence of closed proton and/or neutron shells causes deviation from macroscopic properties of nuclei which are understood in terms of the liquid drop model. It is important to investigate experimentally the stabilizing effects of shell closure, if any, against fission. This work aims to investigate probable effects of proton shell ($Z = 82$) closure in the compound nucleus, in enhancing survival probability of the evaporation residues formed in heavy ion-induced fusion-fission reactions. Evaporation residue cross sections have been measured for the reactions $^{19}$F+$^{180}$Hf, $^{19}$F+$^{181}$Ta and $^{19}$F+$^{182}$W from $\simeq9\%$ below to $\simeq42\%$ above the Coulomb barrier, leading to formation of compound nuclei with same number of neutrons ($N = 118$) but different number of protons across $Z = 82$. Measured excitation functions have been compared with statistical model calculation, in which reduced dissipation coefficient is the only adjustable parameter. Evaporation residue cross section, normalized by capture cross section, is found to decrease gradually with increasing fissility of the compound nucleus. Measured evaporation residue cross sections require inclusion of nuclear viscosity in the model calculations. Reduced dissipation coefficient in the range of 1\textendash3 $\times$ $10^{21}$ s$^{-1}$ reproduces the data quite well. No abrupt enhancement of evaporation residue cross sections has been observed in the reaction forming compound nucleus with $Z = 82$. Thus, this work does not find enhanced stabilizing effects of $Z = 82$ shell closure against fission in the compound nucleus. One may attempt to measure cross sections of individual exit channels for further confirmation of our observation.

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Effect of direct reaction channels on deep sub-barrier fusion in asymmetric systems

A steeper fall of fusion excitation function, compared to the predictions of coupled-channels models, at energies below the lowest barrier between the reaction partners, is termed as deep sub-barrier fusion hindrance. This phenomenon has been observed in many symmetric and nearly-symmetric systems. Different physical origins of the hindrance have been proposed. This work aims to study the probable effects of direct reactions on deep sub-barrier fusion cross sections. Fusion (evaporation residue) cross sections have been measured for the system $^{19}$F+$^{181}$Ta, from above the barrier down to the energies where fusion hindrance is expected to come into play. Coupled-channels calculation with standard Woods-Saxon potential gives a fair description of the fusion excitation function down to energies $\simeq 14\%$ below the barrier for the present system. This is in contrast with the observation of increasing fusion hindrance in asymmetric reactions induced by increasingly heavier projectiles, \textit{viz.} $^{6,7}$Li, $^{11}$B, $^{12}$C and $^{16}$O. The asymmetric reactions, which have not shown any signature of fusion hindrance within the measured energy range, are found to be induced by projectiles with lower $α$ break-up threshold, compared to the reactions which have shown signatures of fusion hindrance. In addition, most of the $Q$-values for light particles pick-up channels are negative for the reactions which have exhibited strong signatures of fusion hindrance, \textit{viz.} $^{12}$C+$^{198}$Pt and $^{16}$O+$^{204,208}$Pb. Thus, break-up of projectile and particle transfer channels with positive $Q$-values seem to compensate for the hindrance in fusion deep below the barrier. Inclusion of break-up and transfer channels within the framework of coupled-channels calculation would be of interest.

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Superdeformation and alpha - cluster structure in 35Cl

A superdeformed (SD) band has been identified in a non - alpha - conjugate nucleus 35Cl. It crosses the negative parity ground band above 11/2- and becomes the yrast at 15/2-. Lifetimes of all relevant states have been measured to follow the evolution of collectivity. Enhanced B(E2), B(E1) values as well as energetics provide evidences for superdeformation and existence of parity doublet cluster structure in an odd-A nucleus for the first time in A = 40 region. Large scale shell model calculations assign (sd)16(pf)3 as the origin of these states. Calculated spectroscopic factors correlate the SD states in 35Cl to those in 36Ar.

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Band crossing in Shears band of $^{108}$Cd

The level lifetimes have been measured for a Shears band of $^{108}$Cd which exhibits bandcrossing. The observed level energies and B(M1) rates have been successfully described by a semi-classical geometric model based on shear mechanism. In this geometric model, the bandcrossing in Shears band has been described as the reopening of the angle between the blades of a shear.

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Study of nuclei in the vicinity of the "Island of Inversion" through fusion-evaporation reaction

We report the first observation of high-spin states in nuclei in the vicinity of the "island of inversion", populated via the 18O+18O fusion reaction at an incident beam energy of 34 MeV. The fusion reaction mechanism circumvents the limitations of non-equilibrated reactions used to populate these nuclei. Detailed spin-parity measurements in these difficult to populate nuclei have been possible from the observed coincidence anisotropy and the linear polarization measurements. The spectroscopy of 33,34P and 33S is presented in detail along with the results of calculations within the shell model framework.

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Astrophysical S_{17}(0) factor from a measurement of d(7Be,8B)n reaction at E_{c.m.} = 4.5 MeV

Angular distribution measurements of $^2$H($^7$Be,$^7$Be)$^2$H and $^2$H($^7$Be,$^8$B)$n$ reactions at $E_{c.m.}\sim$~4.5 MeV were performed to extract the astrophysical $S_{17}(0)$ factor using the asymptotic normalization coefficient (ANC) method. For this purpose a pure, low emittance $^7$Be beam was separated from the primary $^7$Li beam by a recoil mass spectrometer operated in a novel mode. A beam stopper at 0$^{\circ}$ allowed the use of a higher $^7$Be beam intensity. Measurement of the elastic scattering in the entrance channel using kinematic coincidence, facilitated the determination of the optical model parameters needed for the analysis of the transfer data. The present measurement significantly reduces errors in the extracted $^7$Be(p,$γ$) cross section using the ANC method. We get $S_{17}$~(0)~=~20.7~$\pm$~2.4 eV~b.

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Change of 7Be decay rate in exohedral and endohedral C60 fullerene compounds and its implications

The half-life of 7Be implanted in a C60 pellet and gold foil has been measured to be about the same within about 0.2%. Using a radiochemical technique, we also measured that the probability of formation of endohedral 7Be@C60 by nuclear implantation technique was (5.6+-0.45)%. It is known from earlier works that the half-life of endohedral 7Be@C60 is about 1.2% shorter than that of 7Be implanted in gold. An analysis of these results using linear muffin-tin orbital method calculations indicates that most of the implanted 7Be ions in fullerene C60 stay at a distance of about 5.3 Angstrom from the centers of nearest C60 molecules forming exohedral compounds and those who enter the fullerene cages go to the centers of the cages forming endohedral 7Be@C60 compounds.

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Absence of M2 Retardation in $^{35}Cl$: Evidence for Stronger Isospin-Mixing Effects in A=35 Mirror Nuclei

The lifetime of the 3163 keV, 7/2$^-$ isomeric state in $^{35}Cl$ that decays by a stretched M2 transition to the $3/2^+$ ground state, has been re-measured using the Doppler Shift Attenuation Method, by gating on the 1185 keV transition which directly feeds this state. This eliminates the uncertainties in the measurement arising from the direct feedings from the continuum. A mean life of 0.6$^{+0.5}_{-0.2}$ ps has been obtained from the present work. This is considerably smaller than the adopted value 45.3(6) ps. Implication of this major reduction in the lifetime has been pointed out.

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