arXiv subjects

A. Algora

Publications and source records attributed to A. Algora.

At least 37 records · Page 2Linked to original sources

arXiv2022

Bulk and decay properties of neutron-deficient odd-mass Hg isotopes around A = 185

Ground and isomeric states of the neutron-deficient odd-$A$ isotopes $^{183}$Hg, $^{185}$Hg, and $^{187}$Hg are described from a microscopic calculation based on a self-consistent, axially-deformed Hartree-Fock mean field with the Skyrme functional and pairing within BCS approximation. For each equilibrium shape and different odd-neutron states, results on mean square charge radii and magnetic dipole moments are given and analyzed in the context of their sensitivity to the nuclear deformation and to the spin and parity. Spin-isospin correlations within proton-neutron quasiparticle random phase approximation are then introduced in the nuclear states to obtain the distributions of Gamow-Teller strength and the $β^+/EC$ half-lives of these isotopes, whose measurements are planned at ISOLDE-CERN using total absorption gamma-ray spectroscopy techniques.

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arXiv2022

Long-term evolution of the neutron rate at the Canfranc Underground Laboratory

We report results on the long-term variation of the neutron counting rate at the Canfranc Underground Laboratory, of importance for several low-background experiments installed there, including rare-event searches. The measurement campaign was performed employing the High Efficiency Neutron Spectrometry Array (HENSA) mounted in Hall A and lasted 412 live days. The present study is the first long-term measurement of the neutron rate with sensitivity over a wide range of neutron energies (from thermal up to 0.1 GeV and beyond) performed in any underground laboratory so far. Data on the environmental variables inside the experimental hall (radon concentration, air temperature, air pressure and humidity) were also acquired during all the measurement campaign. We have investigated for the first time the evolution of the neutron rate for different energies of the neutrons and its correlation with the ambient variables.

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arXiv2022

Total absorption $γ$-ray spectroscopy of the $β$ decays of $^{96\text{gs,m}}$Y

The $β$ decays of the ground state (gs) and isomeric state (m) of $^{96}$Y have been studied with the total absorption $γ$-ray spectroscopy technique at the Ion Guide Isotope Separator On-Line facility. The separation of the 8$^{+}$ isomeric state from the 0$^{-}$ ground state was achieved thanks to the purification capabilities of the JYFLTRAP double Penning trap system. The $β$-intensity distributions of both decays have been independently determined. In the analyses the de-excitation of the 1581.6 keV level in $^{96}$Zr, in which conversion electron emission competes with pair production, has been carefully considered and found to have significant impact on the $β$-detector efficiency, influencing the $β$-intensity distribution obtained. Our results for $^{96\text{gs}}$Y (0$^+$) confirm the large ground state to ground state $β$-intensity probability, although a slightly larger value than reported in previous studies was obtained, amounting to $96.6_{-2.1}^{+0.3}\%$ of the total $β$ intensity. Given that the decay of $^{96\text{gs}}$Y is the second most important contributor to the reactor antineutrino spectrum between 5 and 7 MeV, the impact of the present results on reactor antineutrino summation calculations has been evaluated. In the decay of $^{96\text{m}}$Y (8$^{+}$), previously undetected $β$ intensity in transitions to states above 6 MeV has been observed. This shows the importance of total absorption $γ$-ray spectroscopy measurements of $β$ decays with highly fragmented de-excitation patterns. $^{96\text{m}}$Y (8$^{+}$) is a major contributor to reactor decay heat in uranium-plutonium and thorium-uranium fuels around 10 s after fission pulses, and the newly measured average $β$ and $γ$ energies differ significantly from the previous values in evaluated databases (...)

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arXiv2022

Beta decay of the very neutron-deficient $^{60}$Ge and $^{62}$Ge nuclei

We report here the results of a study of the $β$ decay of the proton-rich Ge isotopes, $^{60}$Ge and $^{62}$Ge, produced in an experiment at the RIKEN Nishina Center. We have improved our knowledge of the half-lives of $^{62}$Ge (73.5(1) ms), $^{60}$Ge (25.0(3) ms) and its daughter nucleus, $^{60}$Ga (69.4(2) ms). We measured individual $β$-delayed proton and $γ$ emissions and their related branching ratios. Decay schemes and absolute Fermi and Gamow-Teller transition strengths have been determined. The mass excesses of the nuclei under study have been deduced. A total $β$-delayed proton-emission branching ratio of 67(3)% has been obtained for $^{60}$Ge. New information has been obtained on the energy levels populated in $^{60}$Ga and on the 1/2$^-$ excited state in the $βp$ daughter $^{59}$Zn. We extracted a ground state to ground state feeding of 85.3(3)% for the decay of $^{62}$Ge. Eight new $γ$ lines have been added to the de-excitation of levels populated in the $^{62}$Ga daughter.

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arXiv2021

Measurement of the neutron flux at the Canfranc Underground Laboratory with HENSA

We have performed a long-term measurement of the neutron flux with the High Efficiency Neutron Spectrometry Array HENSA in the Hall A of the Canfranc Underground Laboratory. The Hall A measurement campaign lasted from October 2019 to March 2021, demonstrating an excellent stability of the HENSA setup. Preliminary results on the neutron flux from this campaign are presented for the first time. In Phase 1 (113 live days) a total neutron flux of 1.66(2) $\times$10$^{-5}$ cm$^{-2}$ s$^{-1}$ is obtained. Our results are in good agreement with those from our previous shorter measurement where a reduced experimental setup was employed.

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arXiv2021

Development of a Reference Database for Beta-Delayed Neutron Emission

Beta-delayed neutron emission is important for nuclear structure and astrophysics as well as for reactor applications. Significant advances in nuclear experimental techniques in the past two decades have led to a wealth of new measurements that remain to be incorporated in the databases. We report on a coordinated effort to compile and evaluate all the available beta-delayed neutron emission data. The different measurement techniques have been assessed and the data have been compared with semi-microscopic and microscopic-macroscopic models. The new microscopic database has been tested against aggregate total delayed neutron yields, time-dependent group parameters in 6-and 8-group re-presentation, and aggregate delayed neutron spectra. New recommendations of macroscopic delayed-neutron data for fissile materials of interest to applications are also presented. The new Reference Database for Beta-Delayed Neutron Emission Data is available online at: http://www-nds.iaea.org/beta-delayed-neutron/database.html.

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arXiv2021

Shape changes in the mirror nuclei $^{70}$Kr and $^{70}$Se

We studied the proton-rich $T_z=-1$ nucleus $^{70}$Kr through inelastic scattering at intermediate energies in order to extract the reduced transition probability, $B(E2;\;0^+ \rightarrow 2^+)$. Comparison with the other members of the $A=70$ isospin triplet, $^{70}$Br and $^{70}$Se, studied in the same experiment, shows a $3σ$ deviation from the expected linearity of the electromagnetic matrix elements as a function of $T_z$. At present, no established nuclear structure theory can describe this observed deviation quantitatively. This is the first violation of isospin symmetry at this level observed in the transition matrix elements. A heuristic approach may explain the anomaly by a shape change between the mirror nuclei $^{70}$Kr and $^{70}$Se contrary to the model predictions.

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arXiv2020

On the $β$-decay of $^{186}$Hg

The Gamow-Teller strength distribution of the decay of $^{186}$Hg into $^{186}$Au has been determined for the first time using the total absorption gamma spectroscopy technique and has been compared with theoretical QRPA calculations using the SLy4 Skyrme force. The measured Gamow-Teller strength distribution and the half-life are described by mixing oblate and prolate configurations independently in the parent and daughter nuclei. The best description of the experimental beta strength is obtained with dominantly prolate components for both parent $^{186}$Hg and daughter $^{186}$Au. The approach also allowed us to determine an upper limit of the oblate component in the parent state. The complexity of the analysis required the development of a new approach in the analysis of the X-ray gated total absorption spectrum.

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arXiv2020

Masses of short-lived $^{49}Sc$, $^{50}Sc$, $^{70}As$, $^{73}Br$ and stable $^{196}Hg$ nuclides

Mass measurements of $^{49,50}$Sc, $^{70}$As, $^{73}$Br and $^{196}$Hg nuclides produced at CERN's radioactive-ion beam facility ISOLDE are presented. The measurements were performed at the ISOLTRAP mass spectrometer by use of the multi-reflection time-of-flight and the Penning-trap mass spectrometry techniques. The new results agree well with previously known literature values. The mass accuracy for all cases has been improved.

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arXiv2020

Manifestation of the Berry phase in the atomic nucleus $^{213}$Pb

The neutron-rich $^{213}$Pb isotope was produced in the fragmentation of a primary 1 GeV $A$ $^{238}$U beam, separated in FRS in mass and atomic number, and then implanted for isomer decay $γ$-ray spectroscopy with the RISING setup at GSI. A newly observed isomer and its measured decay properties indicate that states in $^{213}$Pb are characterized by the seniority quantum number that counts the nucleons not in pairs coupled to angular momentum $J=0$. The conservation of seniority is a consequence of the Berry phase associated with particle-hole conjugation, which becomes gauge invariant and therefore observable in semi-magic nuclei where nucleons half-fill the valence shell. The $γ$-ray spectroscopic observables in $^{213}$Pb are thus found to be driven by two mechanisms, particle-hole conjugation and seniority conservation, which are intertwined through the Berry phase.

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arXiv2020

Beta-decay studies for applied and basic nuclear physics

In this review we will present the results of recent beta-decay studies using the total absorption technique that cover topics of interest for applications, nuclear structure and astrophysics. The decays studied were selected primarily because they have a large impact on the prediction of a) the decay heat in reactors, important for the safety of present and future reactors and b) the reactor electron antineutrino spectrum, of interest for particle/nuclear physics and reactor monitoring. For these studies the total absorption technique was chosen, since it is the only method that allows one to obtain beta decay probabilities free from a systematic error called the Pandemonium effect. The measurements presented and discussed here were performed mainly at the IGISOL facility of the University of Jyvaskyla (Finland) using isotopically pure beams provided by the JYFLTRAP Penning trap. Examples are presented to show that the results of our measurements on selected nuclei have had a large impact on predictions of both the decay heat and the anti-neutrino spectrum from reactors. Some of the cases involve beta delayed neutron emission thus one can study the competition between gamma- and neutron-emission from states above the neutron separation energy. The gamma-to-neutron emission ratios can be used to constrain neutron capture (n,gamma)cross sections for unstable nuclei of interest in astrophysics. The information obtained from the measurements can also be used to test nuclear model predictions of half-lives and Pn values for decays of interest in astrophysical network calculations. These comparisons also provide insights into aspects of nuclear structure in particular regions of the nuclear chart.

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arXiv2020

Shape coexistence revealed in the $N=Z$ isotope $^{72}$Kr through inelastic scattering

The $N=Z=36$ nucleus $^{72}$Kr has been studied by inelastic scattering at intermediate energies. Two targets, $^{9}$Be and $^{197}$Au, were used to extract the nuclear deformation length, $δ_\text{N}$, and the reduced $E2$ transition probability, $B(E2)$. The previously unknown non-yrast $2^+$ and $4^+$ states as well as a new candidate for the octupole $3^-$ state have been observed in the scattering on the Be target and placed in the level scheme based on $γ-γ$ coincidences. The second $2^+$ state was also observed in the scattering on the Au target and the $B(E2;\;2^+_2 \rightarrow 0^+_1)$ value could be determined for the first time. Analyzing the results in terms of a two-band mixing model shows clear evidence for a oblate-prolate shape coexistence and can be explained by a shape change from an oblate ground state to prolate deformed yrast band from the first $2^+$ state. This interpretation is corroborated by beyond mean field calculations using the Gogny D1S interaction.

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arXiv2020

Determination of Beta Decay Ground State Feeding of Nuclei of Importance for Reactor Applications

In $β$-decay studies the determination of the decay probability to the ground state of the daughter nucleus often suffers from large systematic errors. The difficulty of the measurement is related to the absence of associated delayed $γ$-ray emission. In this work we revisit the $4πγ-β$ method proposed by Greenwood and collaborators in the 1990s, which has the potential to overcome some of the experimental difficulties. Our interest is driven by the need to determine accurately the $β$-intensity distributions of fission products that contribute significantly to the reactor decay heat and to the antineutrinos emitted by reactors. A number of such decays have large ground state branches. The method is relevant for nuclear structure studies as well. Pertinent formulae are revised and extended to the special case of $β$-delayed neutron emitters, and the robustness of the method is demonstrated with synthetic data. We apply it to a number of measured decays that serve as test cases and discuss the features of the method. Finally, we obtain ground state feeding intensities with reduced uncertainty for four relevant decays that will allow future improvements in antineutrino spectrum and decay heat calculations using the summation method.

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arXiv2019

Total absorption $γ$-ray spectroscopy of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb

The decays of the $β$-delayed neutron emitters $^{137}$I and $^{95}$Rb have been studied with the total absorption $γ$-ray spectroscopy technique. The purity of the beams provided by the JYFLTRAP Penning trap at the ion guide isotope separator on-line facility in Jyväskylä allowed us to carry out a campaign of isotopically pure measurements with the decay total absorption $γ$-ray spectrometer, a segmented detector composed of eighteen NaI(Tl) modules. The contamination coming from the interaction of neutrons with the spectrometer has been carefully studied, and we have tested the use of time differences between prompt $γ$-rays and delayed neutron interactions to eliminate this source of contamination. Due to the sensitivity of our spectrometer, we have found a significant amount of $β$-intensity to states above the neutron separation energy that de-excite by $γ$-rays, comparable to the neutron emission probability. The competition between $γ$ de-excitation and neutron emission has been compared with Hauser-Feshbach calculations, and it can be understood as a nuclear structure effect. In addition, we have studied the impact of the $β$-intensity distributions determined in this work on reactor decay heat and reactor antineutrino spectrum summation calculations. The robustness of our results is demonstrated by a thorough study of uncertainties, and with the reproduction of the spectra of the individual modules and the module-multiplicity gated spectra. This work represents the state-of-the-art of our analysis methodology for segmented total absorption spectrometers.

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arXiv2019

Study of multi-neutron emission in the $β$-decay of $^{11}$Li

The kinematics of two-neutron emission following the $β$-decay of $^{11}$Li was investigated for the first time by detecting the two neutrons in coincidence and by measuring their angle and energy. An array of liquid-scintillator neutron detectors was used to reject cosmic-ray and $γ$-ray backgrounds by pulse-shape discrimination. Cross-talk events in which two detectors are fired by a single neutron were rejected using a filter tested on the $β$-1n emitter $^9$Li. A large cross-talk rejection rate is obtained ($> 95 \%$) over most of the energy range of interest. Application to $^{11}$Li data leads to a significant number of events interpreted as $β$-2n decay. A discrete neutron line at $\approx$ 2 MeV indicates sequential two-neutron emission, possibly from the unbound state at 10.6 MeV excitation energy in $^{11}$Be.

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arXiv2019

Discovery of $^{68}$Br in secondary reactions of radioactive beams

The proton-rich isotope 68Br was discovered in secondary fragmentation reactions of fast radioactive beams. Proton-rich secondary beams of 70,71,72Kr and 70Br, produced at the RIKEN Nishina Center and identified by the BigRIPS fragment separator, impinged on a secondary 9Be target. Unambiguous particle identification behind the secondary target was achieved with the ZeroDegree spectrometer. Based on the expected direct production cross sections from neighboring isotopes, the lifetime of the ground or long-lived isomeric state of 68Br was estimated. The results suggest that secondary fragmentation reactions, where relatively few nucleons are removed from the projectile, offer an alternative way to search for new isotopes, as these reactions populate preferentially low-lying states.

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arXiv2019

Updated Summation Model: An Improved Agreement with the Daya Bay Antineutrino Fluxes

A new summation method model of the reactor antineutrino energy spectrum is presented. It is updated with the most recent evaluated decay databases and with our Total Absorption Gamma-ray Spectroscopy measurements performed during the last decade. For the first time the spectral measurements from the Daya Bay experiment are compared with the detected antineutrino energy spectrum computed with the updated summation method without any renormalisation. The results exhibit a better agreement than is obtained with the Huber-Mueller model in the 2 to 5 MeV range, the region which dominates the detected flux. An unexpected systematic trend is found that the detected antineutrino flux computed with the summation model decreases with the inclusion of more Pandemonium free data. The detected flux obtained now lies only 1.9% above that detected in the Daya Bay experiment, a value that may be reduced with forthcoming new Pandemonium free data leaving less and less room to the reactor anomaly. Eventually, the new predictions of individual antineutrino spectra for the $^{235}$U, $^{239}$Pu, $^{241}$Pu and $^{238}$U are used to compute the dependence of the reactor antineutrino spectral shape on the fission fractions.

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arXiv2019

Total absorption $γ$-ray spectroscopy of niobium isomers

The $β$ intensity distributions of the decays of $^{100\text{gs},100\text{m}}$Nb and $^{102\text{gs},102\text{m}}$Nb have been determined using the Total Absorption $γ$-Ray Spectroscopy technique. The JYFLTRAP double Penning trap system was employed to disentangle the isomeric states involved, lying very close in energy, in a campaign of challenging measurements performed with the Decay Total Absorption $γ$-ray Spectrometer at the Ion Guide Isotope Separator On-Line facility in Jyväskylä. The low-spin isomeric state of each niobium case was populated through the decay of the zirconium parent, that was treated as a contaminant. We have applied a method to extract this contamination, and additionally we have obtained $β$ intensity distributions for these zirconium decays. The $β$-strength distributions evaluated with these results were compared with calculations in quasiparticle random-phase approximation, suggesting a prolate configuration for the ground states of $^{100,102}$Zr. The footprint of the Pandemonium effect was found when comparing our results for the analyses of the niobium isotopes with previous decay data. The $β$-intensities of the decay of $^{102\text{m}}$Nb were obtained for the first time. A careful evaluation of the uncertainties was carried out, and the consistency of our results was validated taking advantage of the segmentation of our spectrometer. The final results were used as input in reactor summation calculations. A large impact on antineutrino spectrum calculations was already reported and here we detail the significant impact on decay heat calculations.

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