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A. Amo

Publications and source records attributed to A. Amo.

49 records · Page 3Linked to original sources

Spin rings in bi-stable planar semiconductor microcavities

A unique feature of exciton-polaritons, inherited from their mixed light-matter origin, is the strongly spin-dependent polariton-polariton interaction, which has been predicted to result in the formation of spin rings in real space [Shelykh et al., Phys. Rev. Lett. 100, 116401 (2008)]. Here we experimentally demonstrate the spin bi-stability of exciton-polaritons in an InGaAs-based semiconductor microcavity under resonant optical pumping. We observe the formation of spin rings whose size can be finely controlled in a spatial scale down to the micrometer range, much smaller than the spot size. We additionally evaluate the sign and magnitude of the antiparallel polariton spin interaction constant.

cond-mat.mes-hall↗

Collective dynamics of excitons and polaritons in semiconductor nanostructures

Time resolved photoluminescence is a powerful technique to study the collective dynamics of excitons and polaritons in semiconductor nanostructures. We present a two excitation pulses technique to induce the ultrafast and controlled quenching of the exciton emission in a quantum well. The depth of the dip is given by the magnitude of the warming of the carriers induced by the arrival of a laser pulse when an exciton population is already present in the sample. We use this technique to study the relaxation mechanisms of polaritons in semiconductor microcavities, which are of great importance to enhance the conditions for their condensation under non-resonant excitation. We also explore the dynamics of polariton fluids resonantly created in the lower polariton branch in a triggered optical parametric oscillator configuration, showing evidence of polariton superfluidity, and opening up the way to the real-time study of quantum fluids.

cond-mat.mes-hall↗

Dynamics of formation and decay of coherence in a polariton condensate

We study the dynamics of formation and decay of a condensate of microcavity polaritons. We investigate the relationship between the number of particles, the emission's linewidth and its degree of linear polarization which serves as the order parameter. Tracking the condensate's formation, we show that, even when interactions are negligible, coherence is not determined only by occupation of the ground state. As a result of the competition between the coherent and thermal fractions of the condensate, the highest coherence is obtained some time after the particle number has reached its maximum.

cond-mat.mes-hall↗

Exciton-polariton condensation in a natural two dimensional trap

Bose Einstein condensation of exciton-polaritons has recently been reported in homogeneous structures only affected by random in-plane fluctuations. We have taken advantage of the ubiquitous defects in semiconductor microcavities to reveal the spontaneous dynamical condensation of polaritons in the quantised levels of a trap. We observe condensation in several quantized states, taking their snapshots in real and reciprocal space. We show also the effect of particle interactions for high occupations numbers, revealed by a change in the confined wave function toward the Thomas Fermi profile.

cond-mat.mes-hall↗

Anisotropic Optical Spin Hall Effect in Semiconductor Microcavities

Propagating, directionally dependent, polarized spin-currents are created in an anisotropic planar semiconductor microcavity, via Rayleigh scattering of optically injected polaritons in the optical spin Hall regime. The influence of anisotropy results in the suppression or enhancement of the pseudospin precession of polaritons scattered into different directions. This is exploited to create intense spin currents by excitation on top of localized defects. A theoretical model considering the influence of the total effective magnetic field on the polariton pseudospin quantitatively reproduces the experimental observations.

cond-mat.mes-hall↗

All-Optical Ultrafast Control and Read-Out of a Single Negatively Charged Self-Assembled InAs Quantum Dot

We demonstrate the all-optical ultrafast manipulation and read-out of optical transitions in a single negatively charged self-assembled InAs quantum dot, an important step towards ultrafast control of the resident spin. Experiments performed at zero magnetic field show the excitation and decay of the trion (negatively charged exciton) as well as Rabi oscillations between the electron and trion states. Application of a DC magnetic field perpendicular to the growth axis of the dot enables observation of a complex quantum beat structure produced by independent precession of the ground state electron and the excited state heavy hole spins.

cond-mat.mes-hall↗

Observation of Superfluidity of Polaritons in Semiconductor Microcavities

One of the most striking manifestations of quantum coherence in interacting boson systems is superfluidity. Exciton-polaritons in semiconductor microcavities are two-dimensional composite bosons predicted to behave as particular quantum fluids. We report the observation of superfluid motion of polaritons created by a laser in a semiconductor microcavity. Superfluidity is investigated in terms of the Landau criterion and manifests itself as the suppression of scattering from defects when the flow velocity is slower than the speed of sound in the fluid. On the other hand, a Cerenkov-like wake pattern is clearly observed when the flow velocity exceeds the speed of sound. The experimental findings are in excellent quantitative agreement with the predictions based on a generalized Gross-Pitaevskii theory, showing that polaritons in microcavities constitute a very rich system for exploring the physics of non-equilibrium quantum fluids.

cond-mat.mtrl-sci↗

Quantum-fluid dynamics of microcavity polaritons

Semiconductor microcavities offer a unique system to investigate the physics of weakly interacting bosons. Their elementary excitations, polaritons--a mixture of excitons and photons--behave, in the low density limit, as bosons that can undergo a phase transition to a regime characterised by long range coherence. Condensates of polaritons have been advocated as candidates for superfluidity; and the formation of vortices as well as elementary excitations with a linear dispersion are actively sought after. In this work, we have created and set in motion a macroscopically degenerate state of polaritons and let it collide with a variety of defects present in the sample. Our experiments show striking manifestations of a coherent light-matter packet that displays features of a superfluid, although one of a highly unusual character as it involves an out-of-equilibrium dissipative system where it travels at ultra-fast velocity of the order of 1% the speed of light. Our main results are the observation of i) a linear polariton dispersion accompanied with diffusion-less motion, ii) flow without resistance when crossing an obstacle, iii) suppression of Rayleigh scattering and iv) splitting into two fluids when the size of the obstacle is comparable with the size of the wavepacket. This work opens the way to the investigation of new phenomenology of out-of-equilibrium condensates.

cond-mat.mes-hall↗

Observation of long-lived polariton states in semiconductor microcavities across the parametric threshold

The excitation spectrum around the pump-only stationary state of a polariton optical parametric oscillator (OPO) in semiconductor microcavities is investigated by time-resolved photoluminescence. The response to a weak pulsed perturbation in the vicinity of the idler mode is directly related to the lifetime of the elementary excitations. A dramatic increase of the lifetime is observed for a pump intensity approaching and exceeding the OPO threshold. The observations can be explained in terms of a critical slowing down of the dynamics upon approaching the threshold and the following onset of the soft Goldstone mode.

cond-mat.other↗

Pauli blockade of the electron spin flip in bulk GaAs

By means of time-resolved optical orientation under strong optical pumping, the k-dependence of the electron spin-flip time (t_sf) in undoped GaAs is experimentally determined. t_sf monotonically decreases by more than one order of magnitude when the electron kinetic energy varies from 2 to 30 meV. At the high excitation densities and low temperatures of the reported experiments the main spin-flip mechanism of the conduction band electrons is the Bir-Aronov-Pikus. By means of Monte-Carlo simulations we evidence that phase-space filling effects result in the blocking of the spin flip, yielding an increase of t_sf with excitation density. These effects obtain values of t_sf up to 30 ns at k=0, the longest reported spin-relaxation time in undoped GaAs in the absence of a magnetic field.

cond-mat.mes-hall↗

Optical Anisotropy and Pinning of the Linear Polarization of Light in Semiconductor Microcavities

We report a strong experimental evidence of the optical anisotropy in a CdTe-based microcavity: the polarization of light is pinned to one of the crystallographic axes independently on the polarization of the excitation. The polarization degree depends strongly on the excitation power, reaching almost 100 % in the stimulated regime. The relaxation time of the polarization is about 1 ns. We argue that all this is an effect of a splitting of the polariton doublet at k=0. We consider different sources for the splitting and conclude that the most likely one is optical birefringence in the mirrors and/or the cavity.

cond-mat.mtrl-sci↗

Interplay of the exciton and electron-hole plasma recombination on the photoluminescence dynamics in bulk GaAs

We present a systematic study of the exciton/electron-hole plasma photoluminescence dynamics in bulk GaAs for various lattice temperatures and excitation densities. The competition between the exciton and electron-hole pair recombination dominates the onset of the luminescence. We show that the metal-to-insulator transition, induced by temperature and/or excitation density, can be directly monitored by the carrier dynamics and the time-resolved spectral characteristics of the light emission. The dependence on carrier density of the photoluminescence rise time is strongly modified around a lattice temperature of 49 K, corresponding to the exciton binding energy (4.2 meV). In a similar way, the rise-time dependence on lattice temperature undergoes a relatively abrupt change at an excitation density of 120-180x10^15 cm^-3, which is about five times greater than the calculated Mott density in GaAs taking into account many body corrections.

cond-mat.mtrl-sci↗

Influence of Trapping on the Exciton Dynamics of Al_xGa_1-xAs Films

We present a systematic study on the exciton relaxation in high purity AlGaAs epilayers. The time for the excitonic photoluminescence to reach its maximum intensity (t_max) shows a non-monotonic dependence on excitation density which is attributed to a competition between exciton localization and carrier-carrier scattering. A phenomenological four level model fully describes the influence of exciton localization on t_max. This localization effect is enhanced by the increase of the Al content in the alloy and disappears when localization is hindered by rising the lattice temperature above the exciton trapping energy.

cond-mat.mtrl-sci↗