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A. E. Stuchbery

Publications and source records attributed to A. E. Stuchbery.

At least 19 recordsLinked to original sources

Resolving anomalous collectivity in the $4_1^+$ to $2_1^+$ transition of $^{58}$Fe

The low-excitation states of atomic nuclei in the region around the $N = Z = 28$ shell closure are generally well described by the shell model. Most experimental observables in the iron isotopes $^{56}$Fe, $^{58}$Fe, and $^{60}$Fe ($Z = 26$; $N=30$, $32$, $34$) support a shell-model description. However, the lifetimes of the $4_1^+$ state in $^{58}$Fe in the literature result in a reduced transition strength that deviates markedly from shell-model predictions. There are three independent measurements, all in agreement and all based on the Doppler Shift Attenuation Method (DSAM) or Doppler-Broadened Line Shape method (DBLS). In this work, Coulomb-excitation measurements were performed on $^{56}$Fe and $^{58}$Fe beams to determine the ratios $B(E2; 4_1^+ \to 2_1^+)/B(E2; 2_1^+ \to 0_1^+)$. Thus, $B(E2; 4_1^+ \to 2_1^+)$ is determined relative to the known $B(E2; 2_1^+ \to 0_1^+)$ values. For $^{56}$Fe, $B(E2; 4_1^+ \to 2_1^+) = 23(4)$ W.u., agreeing with the adopted value. However, for $^{58}$Fe, the $B(E2; 4_1^+ \to 2_1^+)$ values obtained (for the various combinations of matrix element signs that could not be firmly established) are all significantly lower than the value derived from the previous lifetime measurements, and are in accord with shell-model calculations. The 1978 DSAM measurement of Bolotin et al., Nucl. Phys. A 311, 75 (1978), has been re-examined. The discrepancy between that measurement and the Coulomb-excitation measurement can be ascribed to the Lindhard-Scharff-Schiøtt (LSS) electronic stopping powers adopted for the DSAM analysis, which considerably overestimate contemporary values. Evidently, lifetime measurements from that era that are based on LSS stopping powers should be used with caution. The revised lifetime data, incorporating current stopping powers, are compared with shell-model calculations.

nucl-ex

Measurement of the cosmic muon flux at the Stawell Underground Physics Laboratory

We report the first measurement of the underground cosmic muon flux at the Stawell Underground Physics Laboratory. The measurement uses eight EJ200 plastic scintillator panels, equipped with Hamamatsu R13089 PMT pairs at the ends, which are the primary components of the muon veto system for the upcoming SABRE South experiment. The measured muon flux is f = (6.33 +/- 0.04_stat +/- 0.35_sys) x 10^{-8} [s^{-1} cm^{-2}]. This measurement is in excellent agreement with simulations, with a relative uncertainty an order of magnitude smaller than the modelling uncertainty.

hep-ex

Electromagnetic moments of ground and excited states calculated in heavy odd-N open-shell nuclei

Within nuclear DFT, we calculated spectroscopic magnetic dipole and electric quadrupole moments for various quasiparticle configurations of odd-$N$, even-$Z$, $83\leq{}N\leq125$ nuclei ranging from gadolinium to osmium. By tagging the blocked quasiparticles with single-particle states of the semi-magic dysprosium isotope, we efficiently computed 22 prolate and 22 oblate states for each of the 154 nuclei and tracked them across the entire major neutron shell. We compared this extensive set of theoretical results with experimental data for 82 states in the region. Breaking rotational, time-reversal, and signature symmetries, we aligned the intrinsic angular momenta along the axis of axial symmetry, thereby enabling full shape- and spin-self-consistent polarizations. The spectroscopic moments were then obtained by restoring rotational symmetry. We conducted a detailed analysis of the pattern of agreement and disagreement between theory and experiment in individual nuclei. For the magnetic dipole moments, agreement with the data varies and is characterized by an overall average and RMS deviation of 0.11 $μ_N$ and 0.35 $μ_N$, respectively. For the electric quadrupole moments, a good corresponding agreement of 0.16 b and 0.29 b was observed.

nucl-th

Coulomb excitation of $^{124}$Te: Emerging collectivity and persisting seniority structure in the $6_1^+$ level

The low-lying energy spectra of even-even tellurium isotopes near midshell have long been interpreted as `textbook' examples of vibrational collective motion. However, in many cases electric-quadrupole observables, which are a particularly sensitive probe of collectivity, remain undetermined. Coulomb-excitation measurements were performed to measure transition strengths connecting the ground and low-excitation states in $^{124}$Te. This isotope lies at a transitional point between collective structure near the neutron midshell and seniority structures near the $N=82$ shell. A transition strength, $B(E2; 6_1^+ \to 4_1^+)$, of 27(9)~W.u. was measured for the $6^+_1\rightarrow4^+_1$ transition for the first time in this nucleus; this value is significantly below that expected for a spherical vibrator, as well as other collective models. We examine the transition strengths in $^{124}$Te and its neighbors by comparison with large-basis shell-model calculations and by comparison with General Collective Model (GCM) fits. A GCM description of $^{120}$Te agrees with experimental $E2$ transition strengths, but no comparable description of $^{124}$Te is possible with the GCM. In contrast, there is remarkably good agreement between the $B(E2; 6_1^+ \to 4_1^+)$ values and shell-model calculations for $^{124-134}$Te. It appears that, despite approaching midshell, $^{124}$Te retains a seniority structure for the $6^+_1$ level, i.e. a significant $π0g_{7/2}^2$ contribution. This persistence of the shell structure at the $6^+_1$ state is in contrast to the $B(E2)$ values of the lower-excitation $2^+_1$ and $4^+_1$ states in $^{124}$Te, and neighboring $^{120}$Te and $^{122}$Te, for which the collectivity becomes enhanced as more neutrons are removed from $N=82$.

nucl-ex

Photomultiplier Requirements and Pre-Calibration for the SABRE South Liquid Scintillator Veto

We present a study of the oil-proof base Hamamatsu R5912 photomultiplier tubes that will be used in the SABRE South linear-alkylbenzene liquid scintillator veto. SABRE South is a dark matter direct detection experiment at the Stawell Underground Physics Laboratory, aiming to test the DAMA/LIBRA dark matter annual modulation signal. We discuss the requirements of the liquid scintillator system and its photomultipliers, outline the methods and analysis used for the characterisation measurements, and results from initial tests. We discuss the impact of these measurements on the performance of the active veto system and explore analysis methods to allow for low threshold operation. Finally, we include results from a small scale liquid scintillator detector prototype used to assess the future performance of pulse shape discrimination in the liquid scintillator veto, and how well accommodated it is by the R5912 PMTs.

physics.ins-det

Universal Effective Charges in the $sd$ and $fp$ Shells

The 247-keV state in $^{54}$Sc, populated in the $β$ decay of $^{54}$Ca, is reported here as a nanosecond isomer with a half-life of 26.0(22) ns. The state is interpreted as the $1^+$ member of the $πf_{7/2}\otimesνf_{5/2}$ spin-coupled multiplet, which decays to the $3^+,πf_{7/2} \otimes νp_{1/2}$ ground state. The new half-life corresponds to a pure $E2$ transition with a strength of 1.93(16) W.u., providing the most precise, unambiguous $B(E2)$ value in the neutron-rich $fp$ region to date for a nucleus with valence protons above $Z=20$. Notably, it is roughly four times larger than the $B(E2; 1/2^{-} \rightarrow 5/2^{-})$ value in $^{55}$Ca. The results, as compared to semi-empirical and ab initio shell-model calculations, indicate (1) a weak $N=34$ sub-shell gap relative to $N = 32$, (2) a large $E2$ enhancement in Sc as compared to Ca due to $1p-1h$ proton excitations across $Z=28$, and (3) empirical effective proton and neutron charges, $e_π$ = 1.30(8)$e$ and $e_ν$ = 0.452(7)$e$, respectively, that are in contrast to reports of $e_π\approx 1.1-1.15e$ and $e_ν\approx 0.6-0.8e$ for $fp$-shell nuclei near $N = Z$. We demonstrate that these reports are erroneous and that, in fact, a universal set of effective charges can be used across the $sd$ and $fp$ shells.

nucl-ex

Characterisation of Hamamatsu R11065-20 PMTs for use in the SABRE South NaI(Tl) Crystal Detectors

The SABRE Experiment is a direct detection dark matter experiment using a target composed of multiple NaI(Tl) crystals. The experiment aims to be an independent check of the DAMA/LIBRA results with a detector in the Northern (Laboratori Nazionali Del Gran Sasso, LNGS) and Southern (Stawell Underground Physics Laboratory, SUPL) hemispheres. The SABRE South photomultiplier tubes (PMTs) will be used near the low energy noise threshold and require a detailed calibration of their performance and contributions to the background in the NaI(Tl) dark matter search, prior to installation. We present the development of the pre-calibration procedures for the R11065-20 Hamamatsu PMTs. These PMTs are directly coupled to the NaI(Tl) crystals within the SABRE South experiment. In this paper we present methodologies to characterise the gain, dark rate, and timing properties of the PMTs. We develop a method for in-situ calibration without a light injection source. Additionally we explore the application of machine learning techniques using a Boosted Decision Tree (BDT) trained on the response of single PMTs to understand the information available for background rejection. Finally, we briefly present the simulation tool used to generate digitised PMT data from optical Monte Carlo simulations.

physics.ins-det

The SABRE South Technical Design Report Executive Summary

In this technical design report (TDR) executive summary we describe the SABRE South detector to be built at the Stawell Underground Physics Laboratory (SUPL). The SABRE South detector is designed to test the long-standing DAMA/LIBRA signal of an annually modulating rate consistent with dark matter by using the same target material. Located in the Southern Hemisphere, the detector is uniquely positioned to disentangle modulating seasonal effects. SABRE South uses seven ultra-high purity NaI(Tl) crystals (with a total target mass of either 35 kg or 50 kg), hermetically sealed in copper enclosures that are suspended within a liquid scintillator active veto. High quantum efficiency and low background Hamamatsu R11065 photomultiplier tubes are directly coupled to both ends of the crystal, and enclosed with the crystal in an oxygen free copper enclosure. The active veto system consists of 11.6 kL of linear alkylbenzene (LAB) doped with a mixture of fluorophores and contained in a steel vessel, which is instrumented with at least 18 Hamamatsu R5912 photomultipliers. The active veto tags key radiogenic backgrounds intrinsic to the crystals, such as ${^{40}}$K, and is expected to suppress the total background by 27% in the 1-6 keV region of interest. In addition to the liquid scintillator veto, a muon veto is positioned above the detector shielding. This muon veto consists of eight EJ-200 scintillator modules, with Hamamatsu R13089 photomultipliers coupled to both ends. With an expected total background of 0.72 cpd/kg/keV, SABRE South can test the DAMA/LIBRA signal with 5$σ$ discovery or 3$σ$ exclusion after two years of data taking.

physics.ins-det

The DAMA/LIBRA signal: an induced modulation effect?

The persistence of the DAMA/LIBRA (DAMA) modulation over the past two decades has been a source of great contention within the dark matter community. The DAMA collaboration reports a persistent, modulating event rate within their setup of NaI(Tl) scintillating crystals at the INFN Laboratori Nazionali del Gran Sasso (LNGS) underground laboratory. A recent work alluded that this signal could have arisen due to an analysis artefact, caused by DAMA not accounting for time variation of decaying background radioisotopes in their analysis procedure. In this work, we examine in detail this 'induced modulation' effect, arguing that a number of aspects of the DAMA signal are incompatible with an induced modulation arising from decays of background isotopes over the lifetime of the experiment. Using a toy model of the DAMA/LIBRA experiment, we explore the induced modulation effect under different variations of the activities of the relevant isotopes - namely, $^3$H and $^{210}$Pb - highlighting the various inconsistencies between the resultant toy datasets and the DAMA signal. We stress the importance of the SABRE experiment, whose goal is to unambiguously test for the presence of such a modulating signal in an experiment using the same target material and comparable levels of background.

hep-ex

Suppressed Electric Quadrupole Collectivity in $^{49}$Ti

Single-step Coulomb excitation of $^{46,48,49,50}$Ti is presented. A complete set of $E2$ matrix elements for the quintuplet of states in $^{49}$Ti, centered on the $2^+$ core excitation, was measured for the first time. A total of nine $E2$ matrix elements are reported, four of which were previously unknown. $^{49}_{22}$Ti$_{27}$ shows a $20\%$ quenching in electric quadrupole transition strength as compared to its semi-magic $^{50}_{22}$Ti$_{28}$ neighbour. This $20\%$ quenching, while empirically unprecedented, can be explained with a remarkably simple two-state mixing model, which is also consistent with other ground-state properties such as the magnetic dipole moment and electric quadrupole moment. A connection to nucleon transfer data and the quenching of single-particle strength is also demonstrated. The simplicity of the $^{49}$Ti-$^{50}$Ti pair (i.e., approximate single-$j$ $0f_{7/2}$ valence space and isolation of yrast states from non-yrast states) provides a unique opportunity to disentangle otherwise competing effects in the ground-state properties of atomic nuclei, the emergence of collectivity, and the role of proton-neutron interactions.

nucl-ex

Shape polarization in the tin isotopes near $N=60$ from precision $g$-factor measurements on short-lived $11/2^-$ isomers

The $g$ factors of $11/2^-$ isomers in semimagic $^{109}$Sn and $^{111}$Sn (isomeric lifetimes $τ= 2.9(3)$ ns and $τ= 14.4(7)$ ns, respectively) were measured by an extension of the Time Differential Perturbed Angular Distribution technique, which uses \LaBr detectors and the hyperfine fields of a gadolinium host to achieve precise measurements in a new regime of short-lived isomers. The results, $g(11/2^-; {^{109}\textrm{Sn}}) = -0.186(8)$ and $g(11/2^-; {^{111}\textrm{Sn}}) = -0.214(4)$, are significantly lower in magnitude than those of the $11/2^-$ isomers in the heavier isotopes and depart from the value expected for a near pure neutron $h_{11/2}$ configuration. Broken-symmetry density functional theory calculations applied to the sequence of $11/2^-$ states reproduce the magnitude and location of this deviation. The $g(11/2^-)$ values are affected by shape core polarization; the odd $0h_{11/2}$ neutron couples to $J^π=2^+,4^+,6^+...$ configurations in the weakly-deformed effective core, causing a decrease in the $g$-factor magnitudes.

nucl-ex

Simulation and background characterisation of the SABRE South experiment

SABRE (Sodium iodide with Active Background REjection) is a direct detection dark matter experiment based on arrays of radio-pure NaI(Tl) crystals. The experiment aims at achieving an ultra-low background rate and its primary goal is to confirm or refute the results from the DAMA/LIBRA experiment. The SABRE Proof-of-Principle phase was carried out in 2020-2021 at the Gran Sasso National Laboratory (LNGS), in Italy. The next phase consists of two full-scale experiments: SABRE South at the Stawell Underground Physics Laboratory, in Australia, and SABRE North at LNGS. This paper focuses on SABRE South and presents a detailed simulation of the detector, which is used to characterise the background for dark matter searches including DAMA/LIBRA-like modulation. We estimate an overall background of 0.72 cpd/kg/keV$_{ee}$ in the energy range 1$-$6 keV$_{ee}$ primarily due to radioactive contamination in the crystals. Given this level of background and considering that the SABRE South has a target mass of 50 kg, we expect to exclude (confirm) DAMA/LIBRA modulation at $4~(5)σ$ within 2.5 years of data taking.

physics.ins-det

Microsecond Isomer at the N=20 Island of Shape Inversion Observed at FRIB

Excited-state spectroscopy from the first Facility for Rare Isotope Beams (FRIB) experiment is reported. A 24(2)-$μ$s isomer was observed with the FRIB Decay Station initiator (FDSi) through a cascade of 224- and 401-keV $γ$ rays in coincidence with $^{32}\textrm{Na}$ nuclei. This is the only known microsecond isomer ($1{\text{ }μ\text{s}}\leq T_{1/2} < 1\text{ ms}$) in the region. This nucleus is at the heart of the $N=20$ island of shape inversion and is at the crossroads of spherical shell-model, deformed shell-model, and ab initio theories. It can be represented as the coupling of a proton hole and neutron particle to $^{32}\textrm{Mg}$, $^{32}\textrm{Mg}+π^{-1} + ν^{+1}$. This odd-odd coupling and isomer formation provides a sensitive measure of the underlying shape degrees of freedom of $^{32}\textrm{Mg}$, where the onset of spherical-to-deformed shape inversion begins with a low-lying deformed $2^+$ state at 885 keV and a low-lying shape-coexisting $0_2^+$ state at 1058 keV. We suggest two possible explanations for the 625-keV isomer in $^{32}$Na: a $6^-$ spherical shape isomer that decays by $E2$ or a $0^+$ deformed spin isomer that decays by $M2$. The present results and calculations are most consistent with the latter, indicating that the low-lying states are dominated by deformation.

nucl-ex

Direct measurement of hexacontatetrapole, $\textbf{E6}$ γ decay from $^{\textbf{53m}}$Fe

The only proposed observation of a discrete, hexacontatetrapole ($E6$) transition in nature occurs from the T$_{1/2}$ = 2.54(2)-minute decay of $^{53m}$Fe. However, there are conflicting claims concerning its $γ$-decay branching ratio, and a rigorous interrogation of $γ$-ray sum contributions is lacking. Experiments performed at the Australian Heavy Ion Accelerator Facility were used to study the decay of $^{53m}$Fe. For the first time, sum-coincidence contributions to the weak $E6$ and $M5$ decay branches have been firmly quantified using complementary experimental and computational methods. Agreement across the different approaches confirms the existence of the real $E6$ transition; the $M5$ branching ratio and transition rate have also been revised. Shell model calculations performed in the full $pf$ model space suggest that the effective proton charge for high-multipole, $E4$ and $E6$, transitions is quenched to approximately two-thirds of the collective $E2$ value. Correlations between nucleons may offer an explanation of this unexpected phenomenon, which is in stark contrast to the collective nature of lower-multipole, electric transitions observed in atomic nuclei.

nucl-ex

E2 Rotational Invariants of $0^+_1$ and $2^+_1$ states for $^{106}$Cd: the Emergence of Collective Rotation

The collective structure of $^{106}$Cd is elucidated by multi-step Coulomb excitation of a 3.849 MeV/$A$ beam of $^{106}$Cd on a 1.1 mg/cm$^2$ $^{208}$Pb target using GRETINA-CHICO2 at ATLAS. Fourteen $E2$ matrix elements were obtained. The nucleus $^{106}$Cd is a prime example of emergent collectivity that possesses a simple structure: it is free of complexity caused by shape coexistence and has a small, but collectively active number of valence nucleons. This work follows in a long and currently active quest to answer the fundamental question of the origin of nuclear collectivity and deformation, notably in the cadmium isotopes. The results are discussed in terms of phenomenological models, the shell model, and Kumar-Cline sums of $E2$ matrix elements. The ${\langle 0_2^+ ||E2||2_1^+ \rangle}$ matrix element is determined for the first time, providing a total, converged measure of the electric quadrupole strength, $\langle Q^2 \rangle$, of the first-excited $2_1^+$ level relative to the $0_1^+$ ground state, which does not show an increase as expected of harmonic and anharmonic vibrations. Strong evidence for triaxial shapes in weakly collective nuclei is indicated; collective vibrations are excluded. This is contrary to the only other cadmium result of this kind in $^{114}$Cd by C. Fahlander et al., Nucl. Phys. A485, 327 (1988), which is complicated by low-lying shape coexistence near midshell.

nucl-ex

CLARION2-TRINITY: a Compton-suppressed HPGe and GAGG:Ce-Si-Si array for absolute cross-section measurements with heavy ions

The design and performance of a new Compton-suppressed HPGe and charged-particle array, CLARION2-TRINITY, are described. The TRINITY charged-particle array is comprised of 64 Cerium-doped Gadolinium Aluminium Gallium Garnet (GAGG:Ce) crystals configured into five rings spanning 7-54 degrees, and two annular silicon detectors that can shadow or extend the angular coverage to backward angles with minimal $γ$-ray attenuation. GAGG:Ce is a non-hygroscopic, bright, and relatively fast scintillator with a light distribution well matched to SiPMs. Count rates up to 40 kHz per crystal are sustainable. Fundamental characteristics of GAGG:Ce are measured and presented, including light- and heavy-ion particle identification (PID) capability, pulse-height defects, radiation hardness, and emission spectra. The CLARION2 array consists of up to 16 Compton-suppressed HPGe Clover detectors ($\approx4\%$ efficiency at 1 MeV) configured into four rings (eight HPGe crystal rings) using a non-Archimedean geometry that suppresses back-to-back coincident 511-keV gamma rays. The entire array is instrumented with 100- and 500-MHz (14 bit) waveform digitizers which enable triggerless operation, pulse-shape discrimination, fast timing, and pileup correction. Finally, two examples of experimental data taken during the commissioning of the CLARION2-TRINITY system are given: a PID spectrum from $^{16}$O + $^{18}$O fusion-evaporation, and PID and Doppler-corrected $γ$-ray spectra from $^{48}$Ti + $^{12}$C Coulomb excitation.

physics.ins-det

Hyperfine fields at $^{66}$Ga, $^{67,69}$Ge implanted into iron and gadolinium hosts at 6 K, and applications to g-factor measurements

Isomers in $^{66}$Ga, $^{67}$Ge, and $^{69}$Ge were recoil-implanted into ferromagnetic hosts of iron and gadolinium at $\approx 6$~K, and the hyperfine magnetic fields were determined by Time Differential Perturbed Angular Distribution (TDPAD) measurements. The hyperfine field strengths at $\approx 6$~K are compared to the results of previous higher-temperature measurements and the amplitudes of the $R(t)$ functions are compared to empirical expectations. The results show that gadolinium can be a suitable host for high-precision in-beam $g$-factor measurements. The results of new $g$-factor measurements for isomers in $^{66}$Ga and $^{67}$Ge are $g(^{66}$Ga$,7^{-}) = +0.126(4)$, supporting a $[π_{f5/2} \otimes νg_{9/2}]_{7^-}$ configuration assignment, and $g(^{67}$Ge$,\frac{9}{2}^{+})=-0.1932(22)$, derived from a new measurement of the ratio $g(^{67}\mathrm{Ge})/g(^{69}\mathrm{Ge}) = 0.869(9)$. These values are in agreement with previous results. The $R(t)$ amplitudes indicate that the nuclear alignment produced in the isomeric states was significantly lower than the empirically expected $σ/I \approx 0.35$.

nucl-ex

Pulse Shape Discrimination of low-energy nuclear and electron recoils for improved particle identification in NaI:Tl

The scintillation mechanism in NaI:Tl crystals produces different pulse shapes that are dependent on the incoming particle type. The time distribution of scintillation light from nuclear recoil events decays faster than for electron recoil events and this difference can be categorised using various Pulse Shape Discrimination (PSD) techniques. In this study, we measured nuclear and electron recoils in a NaI:Tl crystal, with electron equivalent energies between 2 and 40 keV. We report on a new PSD approach, based on an event-type likelihood; this outperforms the charge-weighted mean-time, which is the conventional metric for PSD in NaI:Tl. Furthermore, we show that a linear combination of the two methods improves the discrimination power at these energies.

physics.ins-det