arXiv subjects

A. E. Stuchbery

Publications and source records attributed to A. E. Stuchbery.

At least 37 records · Page 2Linked to original sources

arXiv2022

Electric monopole transition from the superdeformed band in $^{40}$Ca

The electric monopole ($E0$) transition strength $ρ^2$ for the transition connecting the third 0$^+$ level, a "superdeformed" band head, to the "spherical" 0$^+$ ground state in doubly magic $^{40}$Ca has been determined via $e^+e^-$ pair-conversion spectroscopy. The measured value, $ρ^2(E0; 0^+_3 \to 0^+_1)~=~2.3(5)\times10^{-3}$, is the smallest $ρ^2(E0; 0^+ \to 0^+)$ found in $A<50$ nuclei. In contrast, the $E0$ transition strength to the ground state observed from the second 0$^+$ state, a band head of "normal" deformation, is an order of magnitude larger, $ρ^2(E0; 0^+_2 \to 0^+_1)~=~25.9(16)\times~10^{-3}$, which shows significant mixing between these two states. Large-Scale Shell Model (LSSM) calculations were performed to understand the microscopic structure of the excited states, and the configuration mixing between them; experimental $ρ^2$ values in $^{40}$Ca and neighboring isotopes were well reproduced by the LSSM calculations. The unusually small $ρ^2(E0; 0^+_3 \to 0^+_1)$ value is due to destructive interference in the mixing of shape-coexisting structures, which are based on several different multiparticle-multihole excitations. This observation goes beyond the usual treatment of $E0$ strengths, where two-state shape mixing cannot result in destructive interference.

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arXiv2021

Quenching factor measurements of sodium nuclear recoils in NaI:Tl determined by spectrum fitting

We have performed measurements of sodium nuclear recoils in NaI:Tl crystals, following scattering by neutrons produced in a $^{7}$Li(p,n)$^{7}$Be reaction. Understanding the light output from such recoils, which is reduced relative to electrons of equivalent energy by the quenching factor, is critical to interpret dark matter experiments that search for nuclear scattering interactions. We have developed a spectrum-fitting methodology to extract the quenching factor from our measurements, and report quenching factors for nuclear recoil energies between 36 and 401 keV. Our results agree with other recent quenching factor measurements that use quasi-monoenergetic neutron sources. The new method will be applied in the future to the NaI:Tl crystals used in the SABRE experiment.

physics.ins-det↗

arXiv2021

Characterization of SABRE crystal NaI-33 with direct underground counting

Ultra-pure NaI(Tl) crystals are the key element for a model-independent verification of the long standing DAMA result and a powerful means to search for the annual modulation signature of dark matter interactions. The SABRE collaboration has been developing cutting-edge techniques for the reduction of intrinsic backgrounds over several years. In this paper we report the first characterization of a 3.4 kg crystal, named NaI-33, performed in an underground passive shielding setup at LNGS. NaI-33 has a record low $^{39}$K contamination of 4.3$\pm$0.2 ppb as determined by mass spectrometry. We measured a light yield of 11.1$\pm$0.2 photoelectrons/keV and an energy resolution of 13.2% (FWHM/E) at 59.5 keV. We evaluated the activities of $^{226}$Ra and $^{228}$Th inside the crystal to be $5.9\pm0.6 μ$Bq/kg and $1.6\pm0.3 μ$Bq/kg, respectively, which would indicate a contamination from $^{238}$U and $^{232}$Th at part-per-trillion level. We measured an activity of 0.51$\pm$0.02 mBq/kg due to $^{210}$Pb out of equilibrium and a $α$ quenching factor of 0.63$\pm$0.01 at 5304 keV. We illustrate the analyses techniques developed to reject electronic noise in the lower part of the energy spectrum. A cut-based strategy and a multivariate approach indicated a rate, attributed to the intrinsic radioactivity of the crystal, of $\sim$1 count/day/kg/keV in the [5-20] keV region.

physics.ins-det↗

arXiv2020

The radiative width of the Hoyle state from $γ$-ray spectroscopy

The cascading 3.21 MeV and 4.44 MeV electric quadrupole transitions have been observed from the Hoyle state at 7.65 MeV excitation energy in $^{12}$C, excited by the $^{12}$C(p,p$^{\prime}$) reaction at 10.7 MeV proton energy. From the proton-$γ$-$γ$ triple coincidence data, a value of ${Γ_{\rm rad}}/Γ=6.2(6) \times 10^{-4}$ was obtained for the radiative branching ratio. Using our results, together with ${Γ_π^{E0}}/Γ$ from Eriksen et al., Phys. Rev. C 102, 024320 and the currently adopted $Γ_π(E0)$ values, the radiative width of the Hoyle state is determined as $Γ_{\rm rad}=5.1(6) \times 10^{-3}$ eV. This value is about 34% higher than the currently adopted value and will impact on models of stellar evolution and nucleosynthesis.

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arXiv2020

Improved precision on the experimental E0 decay branching ratio of the Hoyle state

Stellar carbon synthesis occurs exclusively via the $3α$ process, in which three $α$ particles fuse to form $^{12}$C in the excited Hoyle state, followed by electromagnetic decay to the ground state. The Hoyle state is above the $α$ threshold, and the rate of stellar carbon production depends on the radiative width of this state. The radiative width cannot be measured directly, and must instead be deduced by combining three separately measured quantities. One of these quantities is the $E0$ decay branching ratio of the Hoyle state, and the current $10$\% uncertainty on the radiative width stems mainly from the uncertainty on this ratio. The $E0$ branching ratio was deduced from a series of pair conversion measurements of the $E0$ and $E2$ transitions depopulating the $0^+_2$ Hoyle state and $2^+_1$ state in $^{12}$C, respectively. The excited states were populated by the $^{12}$C$(p,p^\prime)$ reaction at 10.5 MeV beam energy, and the pairs were detected with the electron-positron pair spectrometer, Super-e, at the Australian National University. The deduced branching ratio required knowledge of the proton population of the two states, as well as the alignment of the $2^+_1$ state in the reaction. For this purpose, proton scattering and $γ$-ray angular distribution experiments were also performed. An $E0$ branching ratio of $Γ^{E0}_π/Γ=8.2(5)\times10^{-6}$ was deduced in the current work, and an adopted value of $Γ^{E0}_π/Γ=7.6(4)\times10^{-6}$ is recommended based on a weighted average of previous literature values and the new result. The new recommended value for the $E0$ branching ratio is about 14% larger than the previous adopted value of $Γ^{E0}_π/Γ=6.7(6)\times10^{-6}$, while the uncertainty has been reduced from 9% to 5%.

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arXiv2020

Emerging nuclear collectivity in $^{124-130}$Te

The emergence of nuclear collectivity near doubly-magic $^{132}$Sn was explored along the stable, even-even $^{124-130}$Te isotopes. Preliminary measurements of the $B(E2;4^{+}_{1}\rightarrow2^{+}_{1})$ transition strengths are reported from Coulomb excitation experiments primarily aimed at measuring the $g$ factors of the $4^{+}_{1}$ states. Isotopically enriched Te targets were excited by 198-205 MeV $^{58}$Ni beams. A comparison of transition strengths obtained is made to large-scale shell-model calculations with successes and limitations discussed.

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arXiv2019

Early signal of emerging nuclear collectivity in neutron-rich $^{129}$Sb

Radioactive $^{129}$Sb, which can be treated as a proton plus semi-magic $^{128}$Sn core within the particle-core coupling scheme, was studied by Coulomb excitation. Reduced electric quadrupole transition probabilities, $B(E2)$, for the $2^+$ $\times$ $πg_{7/2}$ multiplet members and candidate $πd_{5/2}$ state were measured. The results indicate that the total electric quadrupole strength of $^{129}$Sb is a factor of 1.39(11) larger than the $^{128}$Sn core, which is in stark contrast to the expectations of the empirically successful particle-core coupling scheme. Shell-model calculations performed with two different sets of nucleon-nucleon interactions suggest that this enhanced collectivity is due to constructive quadrupole coherence in the wavefunctions stemming from the proton-neutron residual interactions, where adding one nucleon to a core near a double-shell closure can have a pronounced effect. The enhanced electric quadrupole strength is an early signal of the emerging nuclear collectivity that becomes dominant away from the shell closure.

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arXiv2019

$E0$ transition strength in stable Ni isotopes

Excited states in $^{58,60,62}$Ni were populated via inelastic proton scattering at the Australian National University as well as via inelastic neutron scattering at the University of Kentucky Accelerator Laboratory. The Super-e electron spectrometer and the CAESAR Compton-suppressed HPGe array were used in complementary experiments to measure conversion coefficients and $δ(E2/M1)$ mixing ratios, respectively, for a number of $2^+ \rightarrow 2^+$ transitions. The data obtained were combined with lifetimes and branching ratios to determine $E0$, $M1$, and $E2$ transition strengths between $2^+$ states. The $E0$ transition strengths between $0^+$ states were measured using internal conversion electron spectroscopy and compare well to previous results from internal pair formation spectroscopy. The $E0$ transition strengths between the lowest-lying $2^+$ states were found to be consistently large for the isotopes studied.

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arXiv2019

Table of electronic factors for E0 electron and electron-positron pair conversion transitions

A new tabulation of electronic factors is reported for electron conversion for elements of Z from 5 to 126 and electronic factors for electron-positron pair conversion for elements of even Z from 4 to 100. The electronic factors for electron conversion, $Ω_{CE}$(E0), were calculated using a modified version of the CATAR program developed by Pauli and Raff with a relativistic-Hartree-Fock-Slater approach (Pauli and Raff, 1975). The electronic factors for electron-positron pair conversion, $Ω_{IPF}$(E0), were calculated using the model developed by Wilkinson (1969). The data tables presented here cover all atomic shells up to R2 and transition energies from 1 keV to 6000 keV and from 1100 keV to 8000 keV for pair conversion. A comparison with previous electronic factor tabulations is presented. Ratios of experimental Ω(E0) values for 83 E0 transitions in 8$\leq$Z$\leq$98 are compared to this tabulation. Two examples of how to use the tabulation to extract E0 strengths are also included.

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arXiv2019

Apparatus for in-beam hyperfine interactions and $g$-factor measurements: design and operation

The design and operation of apparatus for measurements of in-beam hyperfine interactions and nuclear excited-state $g$ factors is described. This apparatus enables a magnetic field of about 0.1 tesla to be applied to the target and the target temperature to be set between $\sim 4$ K and room temperature. Design concepts are developed mainly in terms of transient-field $g$-factor measurements following Coulomb excitation by the implantation perturbed angular correlation (IMPAC) technique. The formalism for perturbed angular correlations is outlined and a figure of merit for optimizing these measurements is derived to inform design. Particle detection is based on the use of silicon photodiodes of rectangular shape. The particle-$γ$ angular correlation formalism for this case is described. The experimental program to date includes temperature-dependent studies of hyperfine fields, transient-field $g$-factor measurements, and time-dependent perturbed angular distribution (TDPAD) studies.

physics.ins-det↗

arXiv2019

First-excited state $g$ factors in the stable, even Ge and Se isotopes

Transient-field $g$-factor measurements in inverse kinematics were performed for the first-excited states of the stable, even isotopes of Ge and Se. The $g$ factors of $^{74}$Ge and $^{74}$Se were measured simultaneously using a cocktail beam, which eliminates most possible sources of systematic error in a relative $g$-factor measurement. The results are $g(^{74}{\rm Se})/g(^{74}{\rm Ge})=1.34(7)$, $g(^{70}{\rm Ge})/g(^{74}{\rm Ge}) = 1.16(15)$, $g(^{72}{\rm Ge})/g(^{74}{\rm Ge})=0.92(13)$, $g(^{76}{\rm Ge})/g(^{74}{\rm Ge})=0.88(5)$, $g(^{76}{\rm Se})/g(^{74}{\rm Se})=0.96(7)$, $g(^{78}{\rm Se})/g(^{74}{\rm Se})=0.82(5)$, $g(^{80}{\rm Se})/g(^{74}{\rm Se})=0.99(7)$ and $g(^{82}{\rm Se})/g(^{74}{\rm Se})=1.19(6)$. The measured $g$-factor ratios are in agreement with ratios from previous measurements, despite considerable variation in previous reported absolute values. The absolute values of the $g$ factors remain uncertain, however the Rutgers parametrization was used to set the transient-field strength and then compare the experimental $g$ factors with shell-model calculations based on the JUN45 and jj44b interactions. Modest agreement was found between experiment and theory for both interactions. The shell model calculations indicate that the $g(2^+_1)$ values and trends are determined largely by the balance of the spin carried by orbital motion of the protons.

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arXiv2019

High-resolution conversion electron spectroscopy of the 125I electron-capture decay

The conversion electrons from the decay of the 35.5-keV excited state of 125Te following the electron capture decay of 125I have been investigated at high resolution using an electrostatic spectrometer. The penetration parameter lambda = -1.2(6) and mixing ratio |delta| = 0.015(2) were deduced by fitting to literature values and present data. The shake probability of the conversion electrons is estimated to be 0.5, more than two times larger than the predicted value of 0.2.

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arXiv2019

Spectroscopy and excited-state $g$~factors in weakly collective ${^{111}}$Cd: confronting collective and microscopic models

The even cadmium isotopes near the neutron midshell have long been considered good examples of vibrational nuclei. However, the vibrational nature of these nuclei has been questioned based on E2 transition rates that are not consistent with vibrational excitations. In the neighbouring odd-mass nuclei, the g factors of the low-excitation collective states have been shown to be more consistent with a deformed rotational core than a vibrational core. Beyond the comparison of vibrational versus rotational models, recent advances in computational power have made shell-model calculations feasible for Cd isotopes, which may give insights into the emergence and nature of collectivity in the Cd isotopes. Collective excitations in the A ~ 100 region were studied through magnetic moments and electromagnetic transitions in 111Cd. The spectroscopy of 111Cd has been studied following Coulomb excitation. Angular correlation measurements, transient-field g-factor measurements and lifetime measurements by the Doppler-broadened line shape method were performed. The structure of the nucleus was explored in relation to particle-vibration versus particle-rotor interpretations. Large-scale shell-model calculations were performed with the SR88MHJM Hamiltonian. Excited-state g factors have been measured, spin assignments examined and lifetimes determined. Attention was given to the reported $5/2^{+}$ 753-keV and $3/2^{+}$ 755-keV states. The $3/2^{+}$ 755-keV level was not observed; evidence is presented that the reported $3/2^+$ state was a misidentification of the $5/2^{+}$ 753-keV state. It is shown that the g factors and level structure of 111Cd are not readily explained by the particle-vibration model. A particle-rotor approach has both successes and limitations. The shell-model approach successfully reproduces much of the known low-excitation structure in 111Cd.

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arXiv2019

Emerging collectivity from the nuclear structure of $^{132}$Xe: Inelastic neutron scattering studies and shell-model calculations

Inelastic neutron scattering was used to study the low-lying nuclear structure of $^{132}$Xe. A comprehensive level scheme is presented, as well as new level lifetimes, multipole mixing ratios, branching ratios, and transition probabilities. Comparisons of these data as well as previously measured $E2$ strengths and $g$ factors are made with new shell-model calculations for $^{132,134,136}$Xe to explore the emergence of collectivity in the Xe isotopes with $N$ < 82 near the closed shell.

nucl-ex↗

arXiv2018

The SABRE project and the SABRE PoP

SABRE aims to directly measure the annual modulation of the dark matter interaction rate with NaI(Tl) crystals. A modulation compatible with the standard hypothesis in which our Galaxy is embedded in a dark matter halo has been measured by the DAMA experiment in the same target material. Other direct detection experiments, using different target materials, seem to exclude the interpretation of such modulation in the simplest scenario of WIMP-nucleon elastic scattering. The SABRE experiment aims to carry out an independent search with sufficient sensitivity to confirm or refute the DAMA claim. The SABRE concept and goal is to obtain a background rate of the order of 0.1 cpd/kg/keVee in the energy region of interest. This challenging goal is achievable by operating high-purity crystals inside a liquid scintillator veto for active background rejection. In addition, twin detectors will be located in the northern and southern hemispheres to identify possible contributions to the modulation from seasonal or site-related effects. The SABRE project includes an initial Proof-of-Principle phase at LNGS (Italy), to assess the radio-purity of the crystals and the efficiency of the liquid scintillator veto. This paper describes the general concept of SABRE and the expected sensitivity to WIMP annual modulation.

physics.ins-det↗

arXiv2018

Monte Carlo simulation of the SABRE PoP background

SABRE (Sodium-iodide with Active Background REjection) is a direct dark matter search experiment based on an array of radio-pure NaI(Tl) crystals surrounded by a liquid scintillator veto. Twin SABRE experiments in the Northern and Southern Hemispheres will differentiate a dark matter signal from seasonal and local effects. The experiment is currently in a Proof-of-Principle (PoP) phase, whose goal is to demonstrate that the background rate is low enough to carry out an independent search for a dark matter signal, with sufficient sensitivity to confirm or refute the DAMA result during the following full-scale experimental phase. The impact of background radiation from the detector materials and the experimental site needs to be carefully investigated, including both intrinsic and cosmogenically activated radioactivity. Based on the best knowledge of the most relevant sources of background, we have performed a detailed Monte Carlo study evaluating the expected background in the dark matter search spectral region. The simulation model described in this paper guides the design of the full-scale experiment and will be fundamental for the interpretation of the measured background and hence for the extraction of a possible dark matter signal.

physics.ins-det↗

arXiv2018

Influence of host matrices on krypton electron binding energies and KLL Auger transition energies

The low-energy electron spectra emitted in the radioactive decay of the $^{83}$Rb and $^{83}$Sr isotopes were measured with a combined electrostatic electron spectrometer. Radioactive sources used were prepared by ion implantation of $^{83}$Sr into a high purity polycrystalline platinum foil at 30 keV and by vacuum-evaporation deposition of $^{83}$ Rb on the same type of foil. From the measured conversion electron spectra, the electron binding energies (referenced to the Fermi level) for the K, L$_1$ , L$_2$ , L$_3$ , M$_1$ , M$_2$, and M$_3$ shell/subshells of krypton in the platinum host were determined to be 14 316.4(12), 1 914.3(9), 1 720.3(9), 1 667.6(9), 281.5(9), 209.6(13), and 201.2(15) eV, respectively, and those for the evaporated layer were observed to be lower by 0.7(1) eV. For both host matrices, values of 2.3(2), 4.6(2), 1.7(2), 1.3(2), and 3.2(3) eV were obtained for the krypton K, L$_1$ , L$_2$ , L$_3$ , and M$_1$ natural atomic level widths, respectively. The absolute energies of 10 838.5(9) and 10 839.5(10) eV were measured for the KL$_2$L$_3$ ($^{1}$D$_2$) Auger transition in krypton implanted in Pt and generated in the evaporated rubidium layer, respectively. A value of 601.0(8) eV was measured for the energy difference of the KL$_2$L$_3$ ($^{1}$D$_2$) transitions in Rb and Kr in the Pt host. Multiconfiguration Dirac-Fock calculations of the krypton KLL transition energies and intensities were also performed.

physics.atom-ph↗

arXiv2018

Search for environmental effects on the KLL Auger spectrum of rubidium generated in radioactive decay

The KLL Auger spectrum of rubidium following the electron capture decay of $^{83}$Sr and $^{85}$Sr isotopes was experimentally studied in detail for the first time using one $^{83}$Sr source and three $^{85}$Sr sources in different host matrices. Energies, relative intensities, and natural widths of all the nine well-resolved basic spectrum components were determined and compared with both predictions and experimental data for krypton. Results of our multiconfiguration Dirac-Fock calculations demonstrated an influence of the "atomic structure effect" on absolute energies of the KLL transitions following the creation of initial vacancies by the electron capture decay. Environmental effects on the KLL Auger spectrum were distinctly observed only for the absolute transition energies.

physics.atom-ph↗