arXiv subjects

A. Fujimori

Publications and source records attributed to A. Fujimori.

At least 199 records · Page 11Linked to original sources

arXiv2002

Chemical potential shift in La(1-x)Sr(x)MnO(3): Photoemission test of the phase separation scenario

We have studied the chemical potential shift in La(1-x)Sr(x)MnO(3) as a function of doped hole concentration by core-level x-ray photoemission. The shift is monotonous, which means that there is no electronic phase separation on a macroscopic scale, whereas it is consistent with the nano-meter scale cluster formation induced by chemical disorder. Comparison of the observed shift with the shift deduced from the electronic specific heat indicates that hole doping in La(1-x)Sr(x)MnO(3) is well described by the rigid-band picture. In particular no mass enhancement toward the metal-insulator boundary was implied by the chemical potential shift, consistent with the electronic specific heat data.

cond-mat.str-el↗

arXiv2002

Crossover in the nature of the metallic phases in the perovskite-type RNiO_3

We have measured the photoemission spectra of Nd$_{1-x}$Sm$_{x}$NiO$_{3}$, where the metal-insulator transition and the Néel ordering occur at the same temperature for $x \lesssim 0.4$ and the metal-insulator transition temperature ($T_{MI}$) is higher than the Néel temperature for $x \gtrsim 0.4$. For $x \le 0.4$, the spectral intensity at the Fermi level is high in the metallic phase above $T_{MI}$ and gradually decreases with cooling in the insulating phase below $T_{MI}$ while for $x > 0.4$ it shows a pseudogap-like behavior above $T_{MI}$ and further diminishes below $T_{MI}$. The results clearly establish that there is a sharp change in the nature of the electronic correlations in the middle ($x \sim 0.4$) of the metallic phase of the $R$NiO$_3$ system.

cond-mat.str-el↗

arXiv2002

Chemical potential shift in lightly-doped to overdoped Bi$_2$Sr$_2$Ca$_{1-x}${\it R}$_{x}$Cu$_2$O$_{8+y}$ ({\it R} = Pr, Er)

We have studied the chemical potential shift in the high-temperature superconductor Bi$_2$Sr$_2$Ca$_{1-x}${\it R}$_{x}$Cu$_2$O$_{8+y}$ ({\it R} = Pr, Er), where the hole concentration is varied from 0.025 to 0.17 per Cu, by precise measurements of core-level photoemission spectra. The result shows that the shift becomes slow in the underdoped region as in the case of La$_{2-x}$Sr$_{x}$CuO$_{4}$ (LSCO) but the effect is much weaker than in LSCO. The observed shift in the present system can be relatively well explained by numerical results on the doped two-dimensional Hubbard model, and suggests that the change of the electronic structure induced by hole doping is less influenced by stripe fluctuations than in LSCO.

cond-mat.supr-con↗

arXiv2002

Electronic structure of In$_{1-x}$Mn$_x$As studied by photoemission spectroscopy: Comparison with Ga$_{1-x}$Mn$_x$As

We have investigated the electronic structure of the $p$-type diluted magnetic semiconductor In$_{1-x}$Mn$_x$As by photoemission spectroscopy. The Mn 3$d$ partial density of states is found to be basically similar to that of Ga$_{1-x}$Mn$_x$As. However, the impurity-band like states near the top of the valence band have not been observed by angle-resolved photoemission spectroscopy unlike Ga$_{1-x}$Mn$_x$As. This difference would explain the difference in transport, magnetic and optical properties of In$_{1-x}$Mn$_x$As and Ga$_{1-x}$Mn$_x$As. The different electronic structures are attributed to the weaker Mn 3$d$ - As 4$p$ hybridization in In$_{1-x}$Mn$_x$As than in Ga$_{1-x}$Mn$_x$As.

cond-mat.mtrl-sci↗

arXiv2001

Doping dependent evolution of the electronic structure of La2-xSrxCuO4 in the superconducting and metallic phases

The electronic structure of the La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) system has been studied by angle-resolved photoemission spectroscopy (ARPES). We report on the evolution of the Fermi surface, the superconducting gap and the band dispersion around the extended saddle point $k=(π,0)$ with hole doping in the superconducting and metallic phases. As hole concentration $x$ decreases, the flat band at $(π,0)$ moves from above the Fermi level ($E_F$) for $x>0.2$ to below $E_F$ for $x<0.2$, and is further lowered down to $x=0.05$. From the leading-edge shift of ARPES spectra, the magnitude of the superconducting gap around $(π,0)$ is found to monotonically increase as $x$ decreases from $x=0.30$ down to $x=0.05$ even though $T_c$ decreases in the underdoped region, and the superconducting gap appears to smoothly evolve into the normal-state gap at $x=0.05$. It is shown that the energy scales characterizing these low-energy structures have similar doping dependences. For the heavily overdoped sample ($x=0.30$), the band dispersion and the ARPES spectral lineshape are analyzed using a simple phenomenological self-energy form, and the electronic effective mass enhancement factor $m^*/m_b \simeq 2$ has been found. As the hole concentration decreases, an incoherent component that cannot be described within the simple self-energy analysis grows intense in the high-energy tail of the ARPES peak. Some unusual features of the electronic structure observed for the underdoped region ($x \lesssim 0.10$) are consistent with the numerical works on the stripe model.

cond-mat.supr-con↗

arXiv2001

Evidence for ubiquitous strong electron-phonon coupling in high-temperature superconductors

Coupling between electrons and phonons (lattice vibrations) drives the formation of the electron pairs responsible for conventional superconductivity. The lack of direct evidence for electron-phonon coupling in the electron dynamics of the high transition temperature superconductors has driven an intensive search for an alternative mechanism. A coupling of an electron with a phonon would result in an abrupt change of its velocity and scattering rate near the phonon energy. Here we use angle resolved photoemission spectroscopy to probe electron dynamics -velocity and scattering rate- for three different families of copper oxide superconductors. We see in all of these materials an abrupt change of electron velocity at 50-80meV, which we cannot explain by any known process other than to invoke coupling with the phonons associated with the movement of the oxygen atoms. This suggests that electron-phonon coupling strongly influences the electron dynamics in the high-temperature superconductors, and must therefore be included in any microscopic theory of superconductivity.

cond-mat.supr-con↗

arXiv2001

Chemical Potential Shift in Nd$_{2-x}$Ce$_{x}$CuO$_{4}$: Contrasting Behaviors of the Electron- and Hole-Doped Cuprates

We have studied the chemical potential shift in the electron-doped superconductor Nd$_{2-x}$Ce$_{x}$CuO$_{4}$ by precise measurements of core-level photoemission spectra. The result shows that the chemical potential monotonously increases with electron doping, quite differently from La$_{2-x}$Sr$_{x}$CuO$_{4}$, where the shift is suppressed in the underdoped region. If the suppression of the shift in La$_{2-x}$Sr$_{x}$CuO$_{4}$ is attributed to strong stripe fluctuations, the monotonous increase of the chemical potential is consistent with the absence of stripe fluctuations in Nd$_{2-x}$Ce$_{x}$CuO$_{4}$. The chemical potential jump between Nd$_{2}$CuO$_{4}$ and La$_{2}$CuO$_{4}$ is found to be much smaller than the optical band gaps.

cond-mat.supr-con↗

arXiv2001

Photoemission study of the skutterudite compounds Co(Sb$_{1-x}$Te$_{x}$)$_3$ and RhSb$_3$

We have studied the electronic structure of the skutterudite compounds Co(Sb$_{1-x}$Te$_{x}$)$_3$ (x= 0, 0.02, 0.04) by photoemission spectroscopy. Valence-band spectra revealed that Sb 5p states are dominant near the Fermi level and are hybridized with Co 3d states just below it. The spectra of {\it p}-type CoSb$_3$ are well reproduced by the band-structure calculation, which suggests that the effect of electron correlations is not strong in CoSb$_3$. When Te is substituted for Sb and n-type carriers are doped into CoSb$_3$, the spectra are shifted to higher binding energies as predicted by the rigid-band model. From this shift and the free-electron model for the conduction and valence bands, we have estimated the band gap of CoSb$_3$ to be 0.03-0.04 eV, which is consistent with the result of transport measurements. Photoemission spectra of RhSb$_3$ have also been measured and revealed similarities to and differences from those of CoSb$_3$.

cond-mat.mtrl-sci↗

arXiv2001

Electron-Like Fermi Surface and Remnant (pi,0) Feature in Overdoped La1.78Sr0.22CuO4

We have performed an angle-resolved photoemission study of overdoped La1.78Sr0.22CuO4, and have observed sharp nodal quasiparticle peaks in the second Brillouin zone that are comparable to data from Bi2Sr2CaCu2O8+d. The data analysis using energy distribution curves, momentum distribution curves and intensity maps all show evidence of an electron-like Fermi surface, which is well explained by band structure calculations. Evidence for many-body effects are also found in the substantial spectral weight remaining below the Fermi level around (pi,0), where the band is predicted to lie above EF.

cond-mat.supr-con↗

arXiv2000

Fermi surface, pseudogaps and dynamical stripes in La2-xSrxCuO4

Doping dependence of the electronic structure of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) has been systematically studied in a series of photoemission measurements. The unusual spectral features in the underdoped regime are attributed to the formation of dynamical stripes and the opening of large and small pseudogaps.

cond-mat.supr-con↗

arXiv2000

Electronic Structure of the Chevrel-Phase Compounds Sn$_{x}$Mo$_{6}$Se$_{7.5}$: Photoemission Spectroscopy and Band-structure Calculations

We have studied the electronic structure of two Chevrel-phase compounds, Mo$_6$Se$_{7.5}$ and Sn$_{1.2}$Mo$_6$Se$_{7.5}$, by combining photoemission spectroscopy and band-structure calculations. Core-level spectra taken with x-ray photoemission spectroscopy show systematic core-level shifts, which do not obey a simple rigid-band model. The inverse photoemission spectra imply the existence of an energy gap located $\sim 1$ eV above the Fermi level, which is a characteristic feature of the electronic structure of the Chevrel compounds. Quantitative comparison between the photoemission spectra and the band-structure calculations have been made. While good agreement between theory and experiment in the wide energy range was obtained as already reported in previous studies, we found that the high density of states near the Fermi level predicted theoretically due to the Van Hove singularity is considerably reduced in the experimental spectra taken with higher energy resolution than in the previous reports. Possible origins are proposed to explain this observation.

cond-mat.str-el↗

arXiv2000

Angle-resolved photoemission study of insulating and metallic Cu-O chains in PrBa$_2$Cu$_3$O$_7$ and PrBa$_2$Cu$_4$O$_8$

We compare the angle-resolved photoemission spectra of the hole-doped Cu-O chains in PrBa$_2$Cu$_3$O$_7$ (Pr123) and in PrBa$_2$Cu$_4$O$_8$ (Pr124). While, in Pr123, a dispersive feature from the chain takes a band maximum at $k_b$ (momentum along the chain) $\sim$ $π/4$ and loses its spectral weight around the Fermi level, it reaches the Fermi level at $k_b$ $\sim$ $π/4$ in Pr124. Although the chains in Pr123 and Pr124 are approximately 1/4-filled, they show contrasting behaviors: While the chains in Pr123 have an instability to charge ordering, those in Pr124 avoid it and show an interesting spectral feature of a metallic coupled-chain system.

cond-mat.str-el↗

arXiv2000

Photoemission in the system of linear chains : application to PrBa$_2$Cu$_3$O$_7$ and La$_{\rm 2-x-y}$Nd$_{\rm y}$Sr$_{\rm x}$CuO$_4$

Photoemission in the system of linear charged chains has been studied with the dipole matrix incorporated, from which its dependencies on the photoelectron momentum (${\bf k}$), photon polarization ($\hat{\bf E}$), and photon energy ($ω$) can be explored. The used model is the three-dimensional array of noninteracting chains, which is so simple as to allow an analytic approach. Motivations of the study are for the doped CuO$_3$ chain in PrBa$_2$Cu$_3$O$_7$ and the doped static stripe phase in La$_{\rm 2-x-y}$Nd$_{\rm y}$Sr$_{\rm x}$CuO$_4$. The one-dimensional dispersion exhibiting spin-charge separation and its dependence on the momentum perpendicular to the chain and its $\hat{\bf E}$-dependency as well are discussed in PrBa$_2$Cu$_3$O$_7$. For La$_{\rm 2-x-y}$Nd$_{\rm y}$Sr$_{\rm x}$CuO$_4$, the anomalous spectral distribution formed by two sets of stripes perpendicular to each other is investigated. The geometric effects led to by the dipole transition matrix including the interference of photocurrents from different chains are found to change the simple one-dimensional feature drastically. We find these changes are consistent with experiment for the chain system PrBa$_2$Cu$_3$O$_7$, but less satisfactory for the stripe phase in La$_{\rm 2-x-y}$Nd$_{\rm y}$Sr$_{\rm x}$CuO$_4$. This means that in the stripe phase much two-dimensional characters still exist unlike the chain system.

cond-mat.mtrl-sci↗

arXiv2000

Electronic structure of the strongly hybridized ferromagnet CeFe2

We report on results from high-energy spectroscopic measurements on CeFe2, a system of particular interest due to its anomalous ferromagnetism with an unusually low Curie temperature and small magnetization compared to the other rare earth-iron Laves phase compounds. Our experimental results indicate very strong hybridization of the Ce 4f states with the delocalized band states, mainly the Fe 3d states. In the interpretation and analysis of our measured spectra, we have made use of two different theoretical approaches: The first one is based on the Anderson impurity model, with surface contributions explicitly taken into account. The second method consists of band-structure calculations for bulk CeFe2. The analysis based on the Anderson impurity model gives calculated spectra in good agreement with the whole range of measured spectra, and reveals that the Ce 4f -- Fe 3d hybridization is considerably reduced at the surface, resulting in even stronger hybridization in the bulk than previously thought. The band-structure calculations are ab initio full-potential linear muffin-tin orbital calculations within the local-spin-density approximation of the density functional. The Ce 4f electrons were treated as itinerant band electrons. Interestingly, the Ce 4f partial density of states obtained from the band-structure calculations also agree well with the experimental spectra concerning both the 4f peak position and the 4f bandwidth, if the surface effects are properly taken into account. In addition, results, notably the partial spin magnetic moments, from the band-structure calculations are discussed in some detail and compared to experimental findings and earlier calculations.

cond-mat.mtrl-sci↗

arXiv2000

Dual Nature of the Electronic Structure of the Stripe Phase

High resolution angle-resolved photoemission measurements have been carried out on (La_1.4-xNd_0.6Sr_x)CuO_4, a model system with static stripes, and (La_1.85Sr_0.15)CuO_4, a high temperature superconductor (T_c=40K) with dynamic stripes. In addition to the straight segments near (pi, 0) and (0, pi) antinodal regions, we have identified the existence of nodal spectral weight and its associated Fermi surface in the electronic structure of both systems. The ARPES spectra in the nodal region show well-defined Fermi cut-off, indicating a metallic character of this charge-ordered state. This observation of nodal spectral weight, together with the straight segments near antinodal regions, reveals dual nature of the electronic structure of the stripes due to the competition of order and disorder.

cond-mat.supr-con↗

arXiv2000

Electronic Structure of La2-xSrxCuO4 in the Vicinity of the Superconductor-Insulator Transition

We report on the result of angle-resolved photoemission (ARPES) study of La$_{2-x}$Sr$_x$CuO$_4$ (LSCO) from an optimally doped superconductor ($x=0.15$) to an antiferromagnetic insulator ($x=0$). Near the superconductor-insulator transition (SIT) $x\sim 0.05$, spectral weight is transferred with hole doping between two coexisting components, suggesting a microscopic inhomogeneity of the doped-hole distribution. For the underdoped LSCO ($x\leq 0.12$), the dispersive band crossing the Fermi level becomes invisible in the $(0,0)-(π,π)$ direction unlike Bi$_2$Sr$_2$CaCu$_2$O$_{8+y}$. These observations may be reconciled with the evolution of holes in the insulator into fluctuating stripes in the superconductor.

cond-mat.supr-con↗

arXiv2000

Fermi Surface and Band Dispersion in La2-xSrxCuO4

Using angle-resolved photoemission spectroscopy (ARPES), we have observed the band structure, Fermi surface and their doping dependences in La2-xSrxCuO4. The results reveal that the Fermi surface undergoes a dramatic change: it is hole-like and centered at k=(pi,pi) in underdoped (x = 0.1) and optimally doped (x = 0.15) samples as in other cuprates while it is electron-like and centered at (0,0) in heavily overdoped (x = 0.3) ones. The peak in the ARPES spectra near (pi/2,pi/2) is broad and weak unlike in other cuprates. In the underdoped and optimally doped samples, a superconducting gap (Delta = 10 - 15 meV) is observed on the Fermi surface near (pi,0).

cond-mat.supr-con↗

arXiv1999

Photoemission Spectral Weight Transfer and Mass Renormalization in the Fermi-Liquid System La$_{1-x}$Sr$_x$TiO$_{3+y/2}$

We have performed a photoemission study of La$_{1-x}$Sr$_x$TiO$_{3+y/2}$ near the filling-control metal-insulator transition (MIT) as a function of hole doping. Mass renormalization deduced from the spectral weight and the width of the quasi-particle band around the chemical potential $μ$ is compared with that deduced from the electronic specific heat. The result implies that, near the MIT, band narrowing occurs strongly in the vicinity of $μ$. Spectral weight transfer occurs from the coherent to the incoherent parts upon antiferromagnetic ordering, which we associate with the partial gap opening at $μ$.

cond-mat.str-el↗