arXiv subjects

A. Imamoglu

Publications and source records attributed to A. Imamoglu.

At least 19 recordsLinked to original sources

arXiv2024

Cavity-Driven Attractive Interactions in Quantum Materials

Many-body phenomena in quantum materials emerge from the interplay among a broad continuum of electronic states, and controlling these interactions is critical for engineering novel phases. One promising approach exploits fluctuations of the vacuum electromagnetic field confined within optical cavities to tailor electronic properties. Here, we demonstrate that cavity photons can mediate attractive interactions in a tunable van der Waals material and reorganize a continuum of electron-hole transitions into an exciton-like state. We introduce a broadband, sub-wavelength time-domain microscope that integrates exfoliated, dual-gated two-dimensional quantum materials into a terahertz cavity. This approach enables the first-ever measurement of the field-tunable bandgap of bilayer graphene at terahertz frequencies while revealing ultrastrong coupling with a vacuum Rabi frequency exceeding $\Omega_{Rabi}/\omega\approx 40\%$ of the bare photon energy. Crucially, we identify a novel cavity-induced resonance emerging from the interband continuum that resembles Coulomb-bound excitons and remains stable across a broad temperature range. By uniting longstanding theoretical predictions with advanced experimental techniques, our findings open new avenues for designing and probing unique light-matter states and realizing hybrid correlated phases in quantum materials.

cond-mat.mtrl-sci↗

arXiv2020

Spin Reversal of a Quantum Hall Ferromagnet at a Landau Level Crossing

When Landau levels (LLs) become degenerate near the Fermi energy in the quantum Hall regime, interaction effects can drastically modify the electronic ground state. We study the quantum Hall ferromagnet formed in a two-dimensional hole gas around the LL filling factor $\nu=1$ in the vicinity of a LL crossing in the heave-hole valence band. Cavity spectroscopy in the strong-coupling regime allows us to optically extract the two-dimensional hole gas' spin polarization. By analyzing this polarization as a function of hole density and magnetic field, we observe a spin flip of the ferromagnet. Furthermore, the depolarization away from $\nu=1$ accelerates close to the LL crossing. This is indicative of an increase in the size of Skyrmion excitations as the effective Zeeman energy vanishes at the LL crossing.

cond-mat.str-el↗

arXiv2018

Shubnikov-de Haas oscillations in optical conductivity of monolayer MoSe$_2$

We report polarization-resolved resonant reflection spectroscopy of a charge-tunable atomically-thin valley semiconductor hosting tightly bound excitons coupled to a dilute system of fully spin- and valley-polarized holes in the presence of a strong magnetic field. We find that exciton-hole interactions manifest themselves in hole-density dependent, Shubnikov-de Haas-like oscillations in the energy and line broadening of the excitonic resonances. These oscillations are evidenced to be precisely correlated with the occupation of Landau levels, thus demonstrating that strong interactions between the excitons and Landau-quantized itinerant carriers enable optical investigation of quantum-Hall physics in transition metal dichalcogenides.

cond-mat.mes-hall↗

arXiv2015

Trion-polaritons : How strong coupling to a cavity changes the orbital and spin properties of trions

The elementary optical excitations of a two-dimensional electron system strongly coupled to a microcavity are trion-polaritons. Using a variational approach, we demonstrate that the competition between Coulomb interaction and light-matter coupling plays a crucial role in determining the lowest-energy orbital and spin properties of trion-polaritons. When the light-matter interaction exceeds the bare trion binding, singlet and triplet trion states are mixed due to a cavity-mediated spin-orbit effect, which in turn results in a strong increase of the outer electron Bohr radius. In this strong cavity coupling regime, the trion-polariton consists of an exciton-polariton surrounded by a weakly bound electron and is reminiscent of a coherent Rydberg excitation.

cond-mat.mes-hall↗

arXiv2013

Nonequilibrium dynamics in an optical transition from a neutral quantum dot to a correlated many-body state

We investigate the effect of many-body interactions on the optical absorption spectrum of a charge-tunable quantum dot coupled to a degenerate electron gas. A constructive Fano interference between an indirect path, associated with an intra dot exciton generation followed by tunneling, and a direct path, associated with the ionization of a valence-band quantum dot electron, ensures the visibility of the ensuing Fermi-edge singularity despite weak absorption strength. We find good agreement between experiment and renormalization group theory, but only when we generalize the Anderson impurity model to include a static hole and a dynamic dot-electron scattering potential. The latter highlights the fact that an optically active dot acts as a tunable quantum impurity, enabling the investigation of a new dynamic regime of Fermi-edge physics.

cond-mat.mes-hall↗

arXiv2013

Proposed Rabi-Kondo Correlated State in a Laser-Driven Semiconductor Quantum Dot

Spin exchange between a single-electron charged quantum dot and itinerant electrons leads to an emergence of Kondo correlations. When the quantum dot is driven resonantly by weak laser light, the resulting emission spectrum allows for a direct probe of these correlations. In the opposite limit of vanishing exchange interaction and strong laser drive, the quantum dot exhibits coherent oscillations between the single-spin and optically excited states. Here, we show that the interplay between strong exchange and non-perturbative laser coupling leads to the formation of a new nonequilibrium quantum-correlated state, characterized by the emergence of a laser-induced secondary spin screening cloud, and examine the implications for the emission spectrum.

cond-mat.str-el↗

arXiv2013

Quantum Teleportation from a Propagating Photon to a Solid-State Spin Qubit

The realization of a quantum interface between a propagating photon used for transmission of quantum information, and a stationary qubit used for storage and manipulation, has long been an outstanding goal in quantum information science. A method for implementing such an interface between dissimilar qubits is quantum teleportation, which has attracted considerable interest not only as a versatile quantum-state-transfer method but also as a quantum computational primitive. Here, we experimentally demonstrate transfer of quantum information carried by a photonic qubit to a quantum dot spin qubit using quantum teleportation. In our experiment, a single photon in a superposition state of two colors -- a photonic qubit is generated using selective resonant excitation of a neutral quantum dot. We achieve an unprecedented degree of indistinguishability of single photons from different quantum dots by using local electric and magnetic field control. To teleport a photonic qubit, we generate an entangled spin-photon state in a second quantum dot located 5 meters away from the first and interfere the photons from the two dots in a Hong-Ou-Mandel set-up. A coincidence detection at the output of the interferometer heralds successful teleportation, which we verify by measuring the resulting spin state after its coherence time is prolonged by an optical spin-echo pulse sequence. The demonstration of successful inter-conversion of photonic and semiconductor spin qubits constitute a major step towards the realization of on-chip quantum networks based on semiconductor nano-structures.

quant-ph↗

arXiv2013

Topology by dissipation

Topological states of fermionic matter can be induced by means of a suitably engineered dissipative dynamics. Dissipation then does not occur as a perturbation, but rather as the main resource for many-body dynamics, providing a targeted cooling into a topological phase starting from an arbitrary initial state. We explore the concept of topological order in this setting, developing and applying a general theoretical framework based on the system density matrix which replaces the wave function appropriate for the discussion of Hamiltonian ground-state physics. We identify key analogies and differences to the more conventional Hamiltonian scenario. Differences mainly arise from the fact that the properties of the spectrum and of the state of the system are not as tightly related as in a Hamiltonian context. We provide a symmetry-based topological classification of bulk steady states and identify the classes that are achievable by means of quasi-local dissipative processes driving into superfluid paired states. We also explore the fate of the bulk-edge correspondence in the dissipative setting, and demonstrate the emergence of Majorana edge modes. We illustrate our findings in one- and two-dimensional models that are experimentally realistic in the context of cold atoms.

quant-ph↗

arXiv2012

Cavity quantum electrodynamics with charge-controlled quantum dots coupled to a fiber Fabry-Perot cavity

We demonstrate non-perturbative coupling between a single self-assembled InGaAs quantum dot and an external fiber-mirror based microcavity. Our results extend the previous realizations of tunable microcavities while ensuring spatial and spectral overlap between the cavity-mode and the emitter by simultaneously allowing for deterministic charge control of the quantum dots. Using resonant spectroscopy, we show that the coupled quantum dot cavity system is at the onset of strong coupling, with a cooperativity parameter of 2. Our results constitute a milestone towards the realization of a high efficiency solid-state spin-photon interface.

cond-mat.mes-hall↗

arXiv2012

Exciton-assisted optomechanics with suspended carbon nanotubes

We propose a framework for inducing strong optomechanical effects in a suspended carbon nanotube based on deformation potential exciton-phonon coupling. The excitons are confined using an inhomogeneous axial electric field which generates optically active quantum dots with a level spacing in the milli-electronvolt range and a characteristic size in the 10-nanometer range. A transverse field induces a tunable parametric coupling between the quantum dot and the flexural modes of the nanotube mediated by electron-phonon interactions. We derive the corresponding excitonic deformation potentials and show that this interaction enables efficient optical ground-state cooling of the fundamental mode and could allow us to realise the strong and ultra-strong coupling regimes of the Jaynes-Cummings and Rabi models.

cond-mat.mes-hall↗

arXiv2012

Majorana-Like Modes of Light in a One-Dimensional Array of Nonlinear Cavities

The search for Majorana fermions in p-wave paired fermionic systems has recently moved to the forefront of condensed-matter research. Here we propose an alternative route and show theoretically that Majorana-like modes can be realized and probed in a driven-dissipative system of strongly correlated photons consisting of a chain of tunnel-coupled cavities, where p-wave pairing effectively arises from the interplay between strong on-site interactions and two-photon parametric driving. The nonlocal nature of these exotic modes could be demonstrated through cross-correlation measurements carried out at the ends of the chain---revealing a strong photon bunching signature---and their non-Abelian properties could be simulated through tunnel-braid operations.

cond-mat.quant-gas↗

arXiv2012

Majorana Modes in Driven-Dissipative Atomic Superfluids With Zero Chern Number

We investigate dissipation-induced p-wave paired states of fermions in two dimensions and show the existence of spatially separated Majorana zero modes in a phase with vanishing Chern number. We construct an explicit and natural model of a dissipative vortex that traps a single of these modes, and establish its topological origin by mapping the problem to a chiral one-dimensional wire where we observe a non-equilibrium topological phase transition characterized by an abrupt change of a topological invariant (winding number). We show that the existence of a single Majorana zero mode in the vortex core is intimately tied to the dissipative nature of our model. Engineered dissipation opens up possibilities for experimentally realizing such states with no Hamiltonian counterpart.

cond-mat.quant-gas↗

arXiv2012

Decoherence-avoiding spin qubits in optically active quantum dot molecules

In semiconductors, the T2* coherence time of a single confined spin is limited either by the fluctuating magnetic environment (via the hyperfine interaction), or by charge fluctuations (via the spin-orbit interaction). We demonstrate that both limitations can be overcome simultaneously by using two exchange-coupled electron spins that realize a single decoherence-avoiding qubit. Using coherent population trapping, we generate a coherent superposition of the singlet and triplet states of an optically active quantum-dot molecule, and show that the corresponding T2* may exceed 200 nanoseconds.

cond-mat.mes-hall↗

arXiv2011

Dynamic nuclear spin polarization in resonant laser spectroscopy of a quantum dot

Resonant optical excitation of lowest-energy excitonic transitions in self-assembled quantum dots lead to nuclear spin polarization that is qualitatively different from the well known optical orientation phenomena. By carrying out a comprehensive set of experiments, we demonstrate that nuclear spin polarization manifests itself in quantum dots subjected to finite external magnetic field as locking of the higher energy Zeeman transition to the driving laser field, as well as the avoidance of the resonance condition for the lower energy Zeeman branch. We interpret our findings on the basis of dynamic nuclear spin polarization originating from non-collinear hyperfine interaction and find an excellent agreement between the experimental results and the theoretical model.

cond-mat.mes-hall↗

arXiv2010

A coupled quantum dot laser amplifier: Raman transitions between spin singlet and triplet states

A holy grail of photonics research is the realization of a laser that uses a single quantum emitter as the gain medium. Such a device would exhibit a plethora of new features, including lasing without a well-defined threshold and output intensity fluctuations that remain below the shot-noise limit. While single-atom lasers have been demonstrated, compact devices capable of continuous-wave operation require monolithic structures involving a solid-state quantum emitter. Here, we report the observation of steady-state laser amplification in Raman transitions between the lowest-energy entangled spin states of a quantum-dot molecule. Absorption and resonance fluorescence experiments demonstrate that the singlet and triplet states have electric-dipole coupling to a common optically excited state. Fast spin relaxation ensures population inversion on the triplet transition when the singlet transition is driven resonantly. By embedding the quantum-dot molecule in a cavity of modest quality factor, a solid-state single-emitter laser could be realized.

cond-mat.mes-hall↗

arXiv2010

Observation of heavy-hole hyperfine interaction in quantum dots

We measure the strength and the sign of hyperfine interaction of a heavy-hole with nuclear spins in single self-assembled quantum dots. Our experiments utilize the locking of a quantum dot resonance to an incident laser frequency to generate nuclear spin polarization. By monitoring the resulting Overhauser shift of optical transitions that are split either by electron or exciton Zeeman energy with respect to the locked transition using resonance fluorescence, we find that the ratio of the heavy-hole and electron hyperfine interactions is -0.09 +/- 0.02 in two QDs. Since hyperfine interactions constitute the principal decoherence source for spin qubits, we expect our results to be important for efforts aimed at using heavy-hole spins in solid-state quantum information processing. The novel spectroscopic technique we develop also brings new insights to the nuclear-spin mediated locking mechanism in quantum dots.

cond-mat.mes-hall↗

arXiv2010

Signatures of the super fluid-insulator phase transition in laser driven dissipative nonlinear cavity arrays

We analyze the non-equilibrium dynamics of a gas of interacting photons in an array of coupled dissipative nonlinear cavities driven by a pulsed external coherent field. Using a mean-field approach, we show that the system exhibits a phase transition from a Mott-insulator-like to a superfluid regime. For a given single-photon nonlinearity, the critical value of the photon tunneling rate at which the phase transition occurs increases with the increasing photon loss rate. We checked the robustness of the transition by showing its insensitivity to the initial state prepared by the the pulsed excitation. We find that the second-order coherence of cavity emission can be used to determine the phase diagram of an optical many-body system without the need for thermalization.

cond-mat.str-el↗

arXiv2010

Quantum-dot-spin single-photon interface

Using background-free detection of spin-state-dependent resonance fluorescence from a single-electron charged quantum dot with an efficiency of 0:1%, we realize a single spin-photon interface where the detection of a scattered photon with 300 picosecond time resolution projects the quantum dot spin to a definite spin eigenstate with fidelity exceeding 99%. The bunching of resonantly scattered photons reveals information about electron spin dynamics. High-fidelity fast spin-state initialization heralded by a single photon enables the realization of quantum information processing tasks such as non-deterministic distant spin entanglement. Given that we could suppress the measurement back-action to well below the natural spin-flip rate, realization of a quantum non-demolition measurement of a single spin could be achieved by increasing the fluorescence collection efficiency by a factor exceeding 20 using a photonic nanostructure.

cond-mat.mes-hall↗