arXiv subjects

A. Imamoglu

Publications and source records attributed to A. Imamoglu.

At least 37 records · Page 2Linked to original sources

arXiv2009

Anomalous Hanle Effect in Quantum Dots : Evidence for Strong Dynamical Nuclear Polarization in Transverse Magnetic Field

Hanle effect is ubiquitous in the study of spin-related phenomena and has been used to determine spin lifetime, precession and transport in semiconductors. Here, we report an experimental observation of anomalous Hanle effect in individual self-assembled InAs/GaAs quantum dots where we find that a sizeable photo-created electron spin polarization can be maintained in transverse fields as high as 1T until it abruptly collapses. The striking broadening of the Hanle curve by a factor of ~20 and its bistability upon reversal of the magnetic sweep direction points to a novel dynamical nuclear spin polarization mechanism where the effective nuclear magnetic field compensates the transverse applied field. This interpretation is further supported by the measurement of actual electron Zeeman splitting which exhibits an abrupt increase at the Hanle curve collapse. Strong inhomogeneous quadrupolar interactions typical for strained quantum dots are likely to play a key role in polarizing nuclear spins perpendicular to the optically injected spin orientation.

cond-mat.mes-hall↗

arXiv2009

Shedding light on non-equilibrium dynamics of a spin coupled to fermionic reservoir

A single confined spin interacting with a solid-state environment has emerged as one of the fundamental paradigms of mesoscopic physics. In contrast to standard quantum optical systems, decoherence that stems from these interactions can in general not be treated using the Born-Markov approximation at low temperatures. Here we study the non-equilibrium dynamics of a single-spin in a semiconductor quantum dot adjacent to a fermionic reservoir and show how the dynamics can be revealed in detail in an optical absorption experiment. We show that the highly asymmetrical optical absorption lineshape of the resulting Kondo exciton consists of three distinct frequency domains, corresponding to short, intermediate and long times after the initial excitation, which are in turn described by the three fixed points of the single-impurity Anderson Hamiltonian. The zero-temperature power-law singularity dominating the lineshape is linked to dynamically generated Kondo correlations in the photo-excited state. We show that this power-law singularity is tunable with gate voltage and magnetic field, and universal.

cond-mat.str-el↗

arXiv2009

Demagnetization of Quantum Dot Nuclear Spins: Breakdown of the Nuclear Spin Temperature Approach

The physics of interacting nuclear spins arranged in a crystalline lattice is typically described using a thermodynamic framework: a variety of experimental studies in bulk solid-state systems have proven the concept of a spin temperature to be not only correct but also vital for the understanding of experimental observations. Using demagnetization experiments we demonstrate that the mesoscopic nuclear spin ensemble of a quantum dot (QD) can in general not be described by a spin temperature. We associate the observed deviations from a thermal spin state with the presence of strong quadrupolar interactions within the QD that cause significant anharmonicity in the spectrum of the nuclear spins. Strain-induced, inhomogeneous quadrupolar shifts also lead to a complete suppression of angular momentum exchange between the nuclear spin ensemble and its environment, resulting in nuclear spin relaxation times exceeding an hour. Remarkably, the position dependent axes of quadrupolar interactions render magnetic field sweeps inherently non-adiabatic, thereby causing an irreversible loss of nuclear spin polarization.

cond-mat.mes-hall↗

arXiv2009

Confluence of resonant laser excitation and bi-directional quantum dot nuclear spin polarization

Resonant laser scattering along with photon correlation measurements have established the atom-like character of quantum dots. Here, we present measurements which challenge this identification for a wide range of experimental parameters: the absorption lineshapes that we measure at magnetic fields exceeding 1 Tesla indicate that the nuclear spins polarize by an amount that ensures locking of the quantum dot resonances to the incident laser frequency. In contrast to earlier experiments, this nuclear spin polarization is bi-directional, allowing the electron+nuclear spin system to track the changes in laser frequency dynamically on both sides of the quantum dot resonance. Our measurements reveal that the confluence of the laser excitation and nuclear spin polarization suppresses the fluctuations in the resonant absorption signal. A master equation analysis shows narrowing of the nuclear Overhauser field variance, pointing to potential applications in quantum information processing.

cond-mat.mes-hall↗

arXiv2009

Tunable Raman Photons from a Single Quantum Dot

We report the observation of all-optically tunable Raman fluorescence from a single quantum dot. The Raman photons are produced in an optically-driven Lambda-system defined by subjecting the single electron charged quantum dot to a magnetic field in Voigt geometry. Detuning the driving laser from resonance, we tune the frequency of the Raman photons by about 2.5 GHz. The number of scattered photons and the linewdith of the Raman photons are investigated as a function of detuning. The study presented here could form the basis of a new technique for investigating spin-bath interactions in the solid state.

cond-mat.mes-hall↗

arXiv2008

The quantum optical Josephson interferometer

The interplay between coherent tunnel coupling and on-site interactions in dissipation-free bosonic systems has lead to many spectacular observations, ranging from the demonstration of number-phase uncertainty relation to quantum phase transitions. To explore the effect of dissipation and coherent drive on tunnel coupled interacting bosonic systems, we propose a device that is the quantum optical analog of a Josephson interferometer. It consists of two coherently driven linear optical cavities connected via a central cavity with a single-photon nonlinearity. The Josephson-like oscillations in the light emitted from the central cavity as a function of the phase difference between two pumping fields can be suppressed by increasing the strength of the nonlinear coupling. Remarkably, we find that in the limit of ultra-strong interactions in the center-cavity, the coupled system maps on to an effective Jaynes-Cummings system with a nonlinearity determined by the tunnel coupling strength. In the limit of a single nonlinear cavity coupled to two linear waveguides, the degree of photon antibunching from the nonlinear cavity provides an excellent measure of the transition to the nonlinear regime where Josephson oscillations are suppressed.

cond-mat.mes-hall↗

arXiv2008

Spin entanglement using coherent light and cavity-QED

A scheme for probabilistic entanglement generation between two distant single electron doped quantum dots, each placed in a high-Q microcavity, by detecting strong coherent light which has interacted dispersively with both subsystems and experienced Faraday rotation due to the spin selective trion transitions is discussed. In order to assess the applicability of the scheme for distant entanglement generation between atomic qubits proposed by T.D. Ladd et al. [New J. Phys. 8, 184 (2006)] to two distant quantum dots, one needs to understand the limitations imposed by hyperfine interactions of the quantum dot spin with the nuclear spins of the material and by non-identical quantum dots. Feasibility is displayed by calculating the fidelity for Bell state generation analytically within an approximate framework. The fidelity is evaluated for a wide range of parameters and different pulse lengths, yielding a trade-off between signal and decoherence, as well as a set of optimal parameters. Strategies to overcome the effect of non-identical quantum dots on the fidelity are examined and the timescales imposed by the nuclear spins are discussed, showing that efficient entanglement generation is possible with distant quantum dots. In this context, effects due to light hole transitions become important and have to be included. The scheme is discussed for one- as well as for two-sided cavities, where one must be careful with reflected light which carries spin information. The validity of the approximate method is checked by a more elaborate semiclassical simulation which includes trion formation.

quant-ph↗

arXiv2008

Single photon absorption by a single quantum emitter

We show that a three-level lambda quantum emitter with equal spontaneous emission rates on both optically active transitions can absorb an incident light field with a probability approaching unity, provided that the focused light profile matches that of the emitter dipole emission pattern. Even with realistic focusing geometries, our results could find applications in long-distance entanglement of spin qubits.

quant-ph↗

arXiv2007

Strong extinction of a far-field laser beam by a single quantum dot

Through the utilization of index-matched GaAs immersion lens techniques we demonstrate a record extinction (12%) of a far-field focused laser by a single InAs/GaAs quantum dot. This contrast level enables us to report for the first time resonant laser transmission spectroscopy on a single InAs/GaAs quantum dot without the need for phase-sensitive lock-in detection.

cond-mat.other↗

arXiv2007

Dynamics of Quantum Dot Nuclear Spin Polarization Controlled by a Single Electron

We present an experimental study of the dynamics underlying the buildup and decay of dynamical nuclear spin polarization in a single semiconductor quantum dot. Our experiment shows that the nuclei can be polarized on a time scale of a few milliseconds, while their decay dynamics depends drastically on external parameters. We show that a single electron can very efficiently depolarize the nuclear spins and discuss two processes that can cause this depolarization. Conversely, in the absence of a quantum dot electron, the lifetime of nuclear spin polarization is on the time scale of a second, most likely limited by the non-secular terms of the nuclear dipole-dipole interaction. We can further suppress this depolarization rate by 1-2 orders of magnitude by applying an external magnetic field exceeding 1 mT.

physics.optics↗

arXiv2006

Coherent optical manipulation of triplet-singlet states in coupled quantum dots

We show that spin-orbit coupling in a quantum dot molecule allows for coherent manipulation of two electron spin states using Raman transitions. Such two-electron spin states defined by the singlet and triplet states of two exchange coupled quantum dots can have favorable coherence properties. In addition, two of the four metastable ground states in this system can be used as auxiliary states that could facilitate implementation of tasks such as mapping of spin states to that of a single propagating photon. We find that even weak spin-orbit effects -- manifesting themselves as slightly different g-factors for the electron and the hole -- would allow for the coherent Raman coupling of the singlet-triplet states. We also discuss the possibilities for implementing quantum optical techniques for spin preparation and manipulation.

cond-mat.mes-hall↗

arXiv2006

Quantum nature of a strongly-coupled single quantum dot-cavity system

Cavity quantum electrodynamics (QED) studies the interaction between a quantum emitter and a single radiation-field mode. When an atom is in strong coupling with a cavity mode1,2, it is possible to realize key quantum information processing (QIP) tasks, such as controlled coherent coupling and entanglement of distinguishable quantum systems. Realizing these tasks in the solid state is clearly desirable, and coupling semiconductor self-assembled quantum dots (QDs) to monolithic optical cavities is a promising route to this end. However, validating the efficacy of QDs in QIP applications requires confirmation of the quantum nature of the QD-cavity system in the strong coupling regime. Here we find a confirmation by observing quantum correlations in photoluminescence (PL) from a photonic crystal (PC) nanocavity3-5 interacting with one, and only one, QD located precisely at the cavity electric field maximum. When off-resonance, photon emission from the cavity mode and QD excitons is anti-correlated at the level of single quanta, proving that the mode is driven solely by the QD despite an energy mis-match between cavity and excitons. When tuned into resonance, the exciton and photon enter the strong-coupling regime of cavity-QED and the QD lifetime reduces by a factor of 120. The photon stream from the cavity becomes anti-bunched, proving that the coupled exciton/photon system is in the quantum anharmonic regime. Our observations unequivocally show that QIP tasks requiring the quantum nonlinear regime are achievable in the solid state.

quant-ph↗

arXiv2006

Quantum measurement of a mesoscopic spin ensemble

We describe a method for precise estimation of the polarization of a mesoscopic spin ensemble by using its coupling to a single two-level system. Our approach requires a minimal number of measurements on the two-level system for a given measurement precision. We consider the application of this method to the case of nuclear spin ensemble defined by a single electron-charged quantum dot: we show that decreasing the electron spin dephasing due to nuclei and increasing the fidelity of nuclear-spin-based quantum memory could be within the reach of present day experiments.

quant-ph↗

arXiv2006

Nonlinear dynamics of quantum dot nuclear spins

We report manifestly nonlinear dependence of quantum dot nuclear spin polarization on applied magnetic fields. Resonant absorption and emission of circularly polarized radiation pumps the resident quantum dot electron spin, which in turn leads to nuclear spin polarization due to hyperfine interaction. We observe that the resulting Overhauser field exhibits hysteresis as a function of the external magnetic field. This hysteresis is a consequence of the feedback of the Overhauser field on the nuclear spin cooling rate. A semi-classical model describing the coupled nuclear and electron spin dynamics successfully explains the observed hysteresis but leaves open questions for the low field behaviour of the nuclear spin polarization.

cond-mat.mes-hall↗

arXiv2005

Knight Field Enabled Nuclear Spin Polarization in Single Quantum Dots

We demonstrate dynamical nuclear spin polarization in the absence of an external magnetic field, by resonant circularly polarized optical excitation of a single electron or hole charged quantum dot. Optical pumping of the electron spin induces an effective inhomogeneous magnetic (Knight) field that determines the direction along which nuclear spins could polarize and enables nuclear-spin cooling by suppressing depolarization induced by nuclear dipole-dipole interactions. Our observations suggest a new mechanism for spin-polarization where spin exchange with an electron reservoir plays a crucial role. These experiments constitute a first step towards quantum measurement of the Overhauser field.

cond-mat.mes-hall↗

arXiv2005

Voltage-controlled electron-hole interaction in a single quantum dot

The ground state of neutral and negatively charged excitons confined to a single self-assembled InGaAs quantum dot is probed in a direct absorption experiment by high resolution laser spectroscopy. We show how the anisotropic electron-hole exchange interaction depends on the exciton charge and demonstrate how the interaction can be switched on and off with a small dc voltage. Furthermore, we report polarization sensitive analysis of the excitonic interband transition in a single quantum dot as a function of charge with and without magnetic field.

cond-mat.mes-hall↗

arXiv2004

Quantum information processing using localized ensembles of nuclear spins

We describe a technique for quantum information processing based on localized en sembles of nuclear spins. A qubit is identified as the presence or absence of a collective excitation of a mesoscopic ensemble of nuclear spins surrounding a single quantum dot. All single and two-qubit operations can be effected using hyperfine interactions and single-electron spin rotations, hence the proposed scheme avoids gate errors arising from entanglement between spin and orbital degrees of freedom. Ultra-long coherence times of nuclear spins suggest that this scheme could be particularly well suited for applications where long lived memory is essential.

cond-mat.mes-hall↗

arXiv2004

Quantum dot single photon sources: Prospects for applications in linear optics quantum information processing

An optical source that produces single photon pulses on demand has potential applications in linear optics quantum computation, provided that stringent requirements on indistinguishability and collection efficiency of the generated photons are met. We show that these are conflicting requirements for anharmonic emitters that are incoherently pumped via reservoirs. As a model for a coherently pumped single photon source, we consider cavity-assisted spin-flip Raman transitions in a single charged quantum dot embedded in a microcavity. We demonstrate that using such a source, arbitrarily high collection efficiency and indistinguishability of the generated photons can be obtained simultaneously with increased cavity coupling. We analyze the role of errors that arise from distinguishability of the single photon pulses in linear optics quantum gates by relating the gate fidelity to the strength of the two-photon interference dip in photon cross-correlation measurements. We find that performing controlled phase operations with error < 1% requires nano-cavities with Purcell factors F_P >= 40 in the absence of dephasing, without necessitating the strong coupling limit.

quant-ph↗