arXiv subjects

A. K. Grover

Publications and source records attributed to A. K. Grover.

At least 19 recordsLinked to original sources

arXiv2021

Negative differential resistance state in the free-flux-flow regime of driven vortices in a single crystal of 2H-NbS$_2$

Time series measurements in 2H-NbS$_2$ crystal had unravelled a drive induced transition wherein the critical current (Ic) changes from a low to a high Ic jammed vortex state, via a negative differential resistance (NDR) transition. Here, using multiple current (I) - voltage (V) measurement cycles, we explore the statistical nature of observing the NDR transition in the free-flux-flow (FF) regime in a single crystal of 2H-NbS$_2$. The probability of observing the NDR transition always remains finite for a vortex state created with either fast or slow rate of magnetic field. The probability of observing the NDR transition in the FF regime is found to systematically increase with magnetic field (B) in weak collective pinning regime. In the strong pinning regime, the said probability becomes B-independent. We show that the higher Ic state is unique and cannot be accessed via any conventional route. While the I-V curves do not distinguish between zero field cooled (ZFC) and field cooled (FC) modes of preparing the vortex state, the probability for observing an NDR transition has different B-dependences for the vortex matter prepared in the ZFC and FC modes. We find that the NDR occurs in a high dissipation regime, where the flow resistivity is well above the theoretical value expected in the FF regime. We understand our results on the basis of a rapid drop in vortex viscosity at high drives in 2H-NbS$_2$, which triggers a rapid increase in the vortex velocity and reorganization in the moving vortex matter leading to a dynamical unstable vortex flow. This dynamical instability leads to the NDR transition into a high entropy vortex state with high Ic.

cond-mat.supr-con↗

arXiv2015

Unveiling of Bragg glass to vortex glass transition by an ac driving force in a single crystal of Yb3Rh4Sn13

We present here some striking discrepancies in the results of ac and dc magnetization measurements performed in a single crystal of low Tc superconductor, Yb3Rh4Sn13. Fingerprint of a transition from an ordered vortex lattice a la Bragg glass (BG) phase to a partially-disordered vortex glass (VG) like phase gets unearthed under the influence of an ac driving force present inevitably in the isothermal ac susceptibility measurements. In contrast to its well-known effect of improving the state of spatial order in the vortex matter, the ac drive is surprisingly found to promote disorder by assisting the BG to VG transition to occur at a lower field value in this compound. On the other hand, the isothermal dc magnetization (M-H) scans, devoid of such a driving force, do not reveal this transition; they instead yield signature of another order-disorder transition at elevated fields, viz., peak effect (PE), located substantially above the BG to VG transition observed in the isothermal ac susceptibility measurements. Further, the evolution of PE feature with increasing field as observed in isofield ac susceptibility plots indicates emergence of an ordered vortex configuration (BG) from a disordered phase above a certain field, H* (~ 4 kOe). Below H*, the vortex matter created via field-cooling (FC) is found to be better spatially ordered than that prepared in zero field-cooled (ZFC) mode. This is contrary to the usual behavior anticipated near the high-field order-disorder transition (PE) wherein a FC state is supposed to be a supercooled disordered phase and the ZFC state is comparatively better ordered.

cond-mat.supr-con↗

arXiv2015

Paramagnetic magnetization signals and curious metastable behaviour in field-cooled magnetization of a single crystal of superconductor 2H-NbSe2

We present here some newer characteristics pertaining to paramagnetic Meissner effect like response in a single crystal of the low Tc superconducting compound 2H-NbSe2 via a detailed study of effects of perturbation on the field-cooled magnetization response. In the temperature range, where an anomalous paramagnetic magnetization occurs, the field-cooled magnetization response is found to be highly metastable: it displays a curious tendency to switch randomly from a given paramagnetic value to a diamagnetic or to a different paramagnetic value, when the system is perturbed by an impulse of an externally applied ac field. The new facets revealed in a single crystal of 2H-NbSe2 surprisingly bear a marked resemblance with the characteristics of magnetization behaviour anticipated for the giant vortex states with multiple flux quanta predicted to occur in mesoscopic-sized superconducting specimen and possible transitions amongst such states.

cond-mat.supr-con↗

arXiv2014

Evidence of surface superconductivity and multi-quanta vortex states in a weakly-pinned single crystal of Ca3Ir4Sn13

We report here the observation of anomalous paramagnetic signal(s) in the isofield field-cooled cool-down magnetization scans (MFCC(T)) recorded for a single crystal of a low Tc superconductor Ca3Ir4Sn13. Novel features emanating from the MFCC(T) response include an oscillatory magnetization behaviour below Tc and a rich multiplicity (non-uniqueness) in magnetization ranging from diamagnetism to paramagnetism at a given H, T value. The metastability in MFCC(T) has been ascribed to non-unique coexistence of multi-quanta vortex states and single quantum (Abrikosov) vortices. Additionally, the isothermal M(H) scans recorded across a short window of temperature just below Tc show evidence for only the multi-quanta vortex states in the domain of surface superconductivity, with no fingerprint(s) of pinned Abrikosov lattice.

cond-mat.supr-con↗

arXiv2014

Dual role of an ac driving force and the underlying two distinct order-disorder transitions in the vortex phase diagram of Ca3Ir4Sn13

We present distinct demarcation of the Bragg glass (BG) to multi-domain vortex glass (VG) transition line and the eventual amorphization of the VG phase in a weakly pinned single crystal of the superconducting compound Ca3Ir4Sn13 on the basis of comprehension of the different yields about the second magnetization peak (SMP) anomaly in the dc magnetization and the corresponding anomalous feature in the ac susceptibility measurements. The shaking by a small ac magnetic field, inevitably present in the ac susceptibility measurements, is seen to result in contrasting responses in two different portions of the field-temperature (H, T) phase space of the multi-domain VG. In one of the portions, embracing the BG to VG transition across the onset of the SMP anomaly, the ac drive is surprisingly seen to assist the transformation of the well ordered BG phase to a lesser ordered VG phase. The BG phase exists as a superheated state over a small portion of the VG space and this attests to the first order nature of the BG to VG transition.

cond-mat.supr-con↗

arXiv2014

Magnetic compensation phenomenon by Nd doping in spin surplus Sm based ferromagnetic intermetallic SmScGe

The magnetization compensation phenomenon is observed for Sm1-xNdxScGe at x = 0.09 at a temperature near 90 K in a small applied magnetic field, which establishes the spin surplus status of magnetic moment of Sm in the host matrix. We also noted that the sample profiles in QD SQUID magnetometer become asymmetric in some situations indicating significant contributions from multiple moments higher than the dipole moment. We have successfully accounted for them using a fitting procedure involving the higher order magnetic moments.

cond-mat.mtrl-sci↗

arXiv2012

Critical behavior at de-pinning of a driven disordered vortex matter in 2H-NbS2

We report unusual jamming in driven ordered vortex flow in 2H-NbS2. Reinitiating movement in these jammed vortices with a higher driving force, and halting it thereafter once again with a reduction in drive, unfolds a critical behavior centered around the de-pinning threshold via divergences in the lifetimes of transient states, validating the predictions of a recent simulation study, which also pointed out a correspondence between plastic de-pinning in vortex matter and the notion of random organization proposed in the context of sheared colloids undergoing diffusive motion.

cond-mat.supr-con↗

arXiv2011

Magnetization hysteresis and time decay measurements in FeSe$_{0.50}$Te$_{0.50}$ : Evidence for fluctuation in mean free path induced pinning

We present results of magnetic measurements relating to vortex phase diagram in a single crystal of FeSe$_{0.5}$Te$_{0.5}$ which displays second magnetization peak anomaly for $H \parallel c$. The possible role of the crystalline anisotropy on vortex pinning is explored via magnetic torque magnetometry. We present evidence in favor of pinning related to spatial variations of the charge carrier mean free path leading to small bundle vortex pinning by randomly distributed (weak) pinning centers for both $H \parallel c$ and $H \perp c$. This is further corroborated using magnetization data for $H \parallel c$ in a single crystal of FeSe$_{0.35}$Te$_{0.65}$. Dynamical response across second magnetization peak (SMP) anomaly in FeSe$_{0.5}$Te$_{0.5}$ has been compared with that across the well researched phenomenon of peak effect (PE) in a single crystal of CeRu$_2$.

cond-mat.supr-con↗

arXiv2011

Crossover from paramagnetic compressed flux regime to diamagnetic pinned vortex lattice in a single crystal of cubic Ca(3)Rh(4)Sn(13)

We report the observation of positive magnetization on field cooling (PMFC) in low applied magnetic fields (H < 100 Oe) in a single crystal of Ca(3)Rh(4)Sn(13) near its superconducting transition temperature (T(c) approx 8.35 K). For 30 Oe < H < 100 Oe, the PMFC response crosses over to a diamagnetic response as the temperature is lowered below 8 K. For 100 Oe < H < 300 Oe, the diamagnetic response undergoes an unexpected reversal in its field dependence above a characteristic temperature (designated as T*(VL) = 7.9 K), where the field-cooled cool-down magnetization curves intersect. The in-phase and out-of-phase ac susceptibility data confirm the change in the superconducting state across T*(VL). We ascribe the PMFC response to a compression of magnetic flux caused by the nucleation of superconductivity at the surface of the sample. In very low fields (H < 20 Oe), the PMFC response has an interesting oscillatory behaviour which persists up to about 7 K. The oscillatory nature underlines the interplay between competing responses contributing to the magnetization signal in PMFC regime. We believe that the (i) counterintuitive field dependence of the diamagnetic response for H > 100 Oe and above T*(VL) (lasting up to T(c), (ii) the oscillatory character in PMFC response at low fields and (iii) the PMFC peaks near 8.2 K in 30 Oe <= H <= 100 Oe provide support in favour of a theoretical scenario based on the Ginzburg-Landau equations. The scenario predicts the possibility of complex magnetic fluctuations associated with transformation between different metastable giant vortex states prior to transforming into the conventional vortex state as the sample is cooled below T*(VL).

cond-mat.supr-con↗

arXiv2010

Observation of tunable exchange bias in Sr$_2$YbRuO$_6$

The double perovskite compound, Sr$_{2}$YbRuO$_{6}$, displays reversal in the orientation of magnetic moments along with negative magnetization due to an underlying magnetic compensation phenomenon. The exchange bias (EB) field below the compensation temperature could be the usual negative or the positive depending on the initial cooling field. This EB attribute has the potential of getting tuned in a preselected manner, as the positive EB field is seen to crossover from positive to negative value above $T_{\mathrm{comp}}$.

cond-mat.mtrl-sci↗

arXiv2010

Search and identification of repeated magnetic compensation in Nd(1-x)R(x)Al(2) (R = Gd, Tb) series

We undertook investigations in polycrystalline R(x)R'(1-x)Al(2) alloys, in particular, explored the stoichiometries, Nd(0.8)Gd(0.2)Al(2) and Nd(0.8)Tb(0.2)Al(2), to study the magnetic compensation behavior in them in the context of contemporary interest. In these admixed rare-earth (RE) intermetallics, the compensation phenomenon is characterized by a crossover of the M = 0 axis in the low field thermomagnetic response, and a turnaround behavior due to the field-induced reversal in the orientations of the RE moments at high fields. While the characteristic attributes are present in Nd(0.8)Gd(0.2)Al(2), a repeated/multiple magnetic compensation behavior stands observed in Nd(0.8)Tb(0.2)Al(2). The ac susceptibility, the heat capacity and the transport measurements in the latter compound reveal the onset of two quasi-antiferromagnetic transitions one after the other on cooling down from the high temperature end. The two magnetic transitions involving competition between the contributions from nearly balanced weighted averages of moments of Nd{3+} and Tb{3+} ions generate the curious multiple crossings of the M = 0 axis. The results are compared and contrasted with repeated compensation behavior reported earlier in admixed Nd(0.8)Gd(0.2)Rh(3)B(2) alloy.

cond-mat.str-el↗

arXiv2010

Field induced changes across magnetic compensation in Pr(1-x)Gd(x)Al(2) alloys

The magnetic compensation phenomenon has been explored in the Pr(1-x)Gd(x)Al(2) series. The contributions from Pr and Gd moments compensate each other at a specific temperature in the ordered state (below (T(c)). At high fields, the magnetic reorientation (with respect to the external field direction) of the Pr and Gd moments appears as a minimum in the thermomagnetic response. We demonstrate several interesting attributes related with the magnetic reorienation phenomenon, viz., oscillatory behavior of the magneto-resistance, sign change of the anamalous Hall resistivity, fingerprints of field induced changes in the specific heat and ac-susceptibility data.

cond-mat.str-el↗

arXiv2010

Self-magnetic compensation and Exchange Bias in ferromagnetic Samarium systems

For Sm(3+) ions in a vast majority of metallic systems, the following interesting scenario has been conjured up for long, namely, a magnetic lattice of tiny self (spin-orbital) compensated 4f-moments exchange coupled (and phase reversed) to the polarization in the conduction band. We report here the identification of a self-compensation behavior in a variety of ferromagnetic Sm intermetallics via the fingerprint of a shift in the magnetic hysteresis (M-H) loop from the origin. Such an attribute, designated as exchange bias in the context of ferromagnetic/antiferromagnetic multilayers, accords these compounds a potential for niche applications in spintronics. We also present results on magnetic compensation behavior on small Gd doping (2.5 atomic percent) in one of the Sm ferromagnets (viz. SmCu(4)Pd). The doped system responds like a pseudo-ferrimagnet and it displays a characteristic left-shifted linear M-H plot for an antiferromagnet.

cond-mat.mtrl-sci↗

arXiv2009

Giant low frequency velocity fluctuations in a driven vortex lattice

The driven state of a well-ordered flux line lattice in a single crystal of 2H-NbSe2 in the time domain has revealed the presence of substantial fluctuations in velocity, with large and distinct time periods (~ seconds). A superposition of a periodic drive in the driven vortex lattice causes distinct changes in these fluctuations. We propose that prior to onset of the peak effect there exist hithertofore unexplored regime of coherent dynamics, with unexpected behaviour in velocity fluctuations.

cond-mat.supr-con↗

arXiv2008

Anisotropy in vortex phase diagram and the pinning force density in the basal plane of YNi_2B_2C

We present magnetic field dependence of the critical current density from dc-magnetization measurements concerning the anisotropic behavior of flux line lattice (FLL) in a single crystal of YNi_2B_2C. The peak effect (PE) phenomenon is observed for all crystallographic orientations, but the second magnetization peak (SMP) anomaly is observed only for H//a. Our study reveals that the FLL obtained when H//[100] is better ordered within the basal plane. However, the FLL for H// c is found to be even more ordered than that for H//[110]. The perfect square symmetry of the FLL for H//c is perhaps responsible for promoting the realization of the best spatial order of the FLL prior to the onset of PE, indicating a correlation between the crystalline lattice and the FLL. We have also found a change over in the power law governing the decay of the critical current density which is identified as a crossover from weak to weaker pinning regime in the phase diagram.

cond-mat.supr-con↗

arXiv2008

Peak effect phenomena, surface superconductivity and paramagnetic Meissner effect in a spherical single crystal of niobium

We have explored the vortex phase diagram in a spherical single crystal of niobium (T ~ 9.3 K) via isothermal and temperature dependent dc magnetization and ac-susceptibility measurements. The crystal has extremely weak pinning that can be inferred from the reversibility of loops below T_c. However, one can visualize the peak effect (PE) feature in the isothermal M-H loops up to T = 8 K. The PE is also prominent in isothermal ac-susceptibility data for H > 750 Oe. An interesting observation in the present study is the prominent fingerprints of surface superconductivity, starting just above the collapse of pinning at the peak position of the PE and ending at the surface critical field (H_c3). We have also observed the paramagnetic Meissner effect in field-cooled magnetization data recorded at relatively large fields in this crystal. A vortex phase diagram is constructed by marking the peak positions of the PE (H_p), the upper critical field (H_c2) and the surface critical field (H_c3). Unlike a previous report which shows the existence of a multi-critical point in the phase dia-gram of a Nb crystal, where H_p, H_c2 and H_c3 lines meet, we do not observe a multi-critical point in our weak pinning crystal.

cond-mat.supr-con↗

arXiv2008

Thermo-magnetic history effects in the vortex state of YNi_2B_2C superconductor

The nature of five-quadrant magnetic isotherms for is different from that for in a single crystal of YNi2B2C, pointing towards an anisotropic behaviour of the flux line lattice (FLL). For, a well defined peak effect (PE) and second magnetization peak (SMP) can be observed and the loop is open prior to the PE. However, for, the loop is closed and one can observe only the PE. We have investigated the history dependence of magnetization hysteresis data for by recording minor hysteresis loops. The observed history dependence in across different anomalous regions are rationalized on the basis of su-perheating/supercooling of the vortex matter across the first-order-like phase transition and possible additional effects due to annealing of the disordered vortex bundles to the underlying equilibrium state.

cond-mat.supr-con↗

arXiv2008

Exchange bias and its phase reversal in the zero magnetization admixed rare earth intermetallics

Exchange bias effect is an important attribute in several device applications. Traditionally, it is discussed as a form of exchange anisotropy at the interface between the ferromagnetic/antiferromagnetic layers of two distinct systems. We report here on the magnetically ordered alloys possessing the feature of unidirectional anisotropy, which reverses its sign across a characteristic temperature. These are admixed rare earth intermetallics, comprising two dissimilar rare earth (RE) ions, belonging to the two different halves of the 4f-series and imbibing the notion of ferromagnetic coupling between the spins of all 4f-rare earth ions and that of the conduction electrons. Magnetic moments of dissimilar RE ions in such admixed alloys, however, get antiferromagnetically coupled and they display magnetic compensation feature such that the field induced reversal in the orientation of the magnetic moments of dissimilar rare earth ions happens across the compensation temperature (Tcomp). Above a threshold field, the conduction electron polarization also reverses its sign across Tcomp, this is argued to correlate with the observed phase reversal in the exchange bias field.

cond-mat.str-el↗