arXiv subjects

A. K. Grover

Publications and source records attributed to A. K. Grover.

35 records · Page 2Linked to original sources

arXiv2008

Sign reversal in the exchange bias and the collapse of hysteresis width across the magnetic compensation temperature in a single crystal of Nd0.75Ho0.25Al2

In the admixed Nd0.75Ho0.25Al2 system, magnetic moments of Nd and Ho occupying the same crystallographic site are antiferromagnetically coupled and the chosen stoichiometry displays a magnetic compensation behavior (Tcomp of about 24 K) in all orientations. In the vicinity of Tcomp, the conduction electron polarization (CEP) assumes the role of a soft ferromagnet exchange coupled to a pseudo-antiferromagnet comprising Nd/Ho moments, resulting in an asymmetry in the hysteretic (M-H) loop, i.e., the notion of an exchange bias field (Hexch). Across Tcomp, the CEP contribution reverses sign, and in consonance, the asymmetry in the M-H loop also undergoes a phase reversal. Interestingly, the width of the M-H loop shows a divergence, followed by a collapse on approaching Tcomp from either end. The observed behavior confirms a long standing prediction based on a phenomenological model for ferrimagnetic systems. The field induced changes across Tcomp leave an imprint of a quasi-phase transition in the heat capacity data. Magneto-resistance (ΔR / R vs T) has an oscillatory response, in which the changes across Tc and Tcomp can be recognized.

cond-mat.str-el↗

arXiv2008

New Samarium and Neodymium based admixed ferromagnets with near zero net magnetization and tunable exchange bias field

Rare earth based intermetallics, SmScGe and NdScGe, are shown to exhibit near zero net magnetization with substitutions of 6 to 9 atomic percent of Nd and 25 atomic percent of Gd, respectively. The notion of magnetic compensation in them is also elucidated by the crossover of zero magnetization axis at low magnetic fields (less than 103 Oe) and field-induced reversal in the orientation of the magnetic moments of the dissimilar rare earth ions at higher magnetic fields. These magnetically ordered materials with no net magnetization and appreciable conduction electron polarization display an attribute of an exchange bias field, which can be tuned. The attractively high magnetic ordering temperatures of about 270 K, underscore the importance of these materials for potential applications in spintronics.

cond-mat.str-el↗

arXiv2008

Flux jumps, Second Magnetization Peak anomaly and the Peak Effect phenomenon in single crystals of $YNi_2B_2C$ and $LuNi_2B_2C$

We present magnetization measurements in single crystals of the tetragonal $YNi_2B_2C$ compound, which exhibit the phenomenon of peak effect as well as the second magnetization peak anomaly for H $>$ 0.5T (H $||$ c). At the lower field (50mT $<$ H $<$ 200mT), we have observed the presence of flux jumps, which seem to relate to a structural change in the local symmetry of the flux line lattice (a first order re-orientation transition across a local field in some parts of the sample, in the range of 100mT to 150mT). These flux jumps are also observed in a single crystal of $LuNi_2B_2C$ for H $||$ c in the field region from 2 mT to 25 mT, which are compatible with the occurrence of a re-orientation transition at a lower field in a cleaner crystal of this compound, as compared to those of $YNi_2B_2C$. Vortex phase diagrams drawn for H $||$ c in $LuNi_2B_2C$ and $YNi_2B_2C$ show that the ordered elastic glass phase spans a larger part of (H, T) space in the former as compared to latter, thereby, reaffirming the difference in the relative purity of the two samples.

cond-mat.supr-con↗

arXiv2008

Anisotropy in spatial order-disorder transformations and the vortex lattice symmetry transition in $YNi_2B_2C$ and $LuNi_2B_2C$

Explorations of the order-disorder transformation in vortex matter in single crystals of tetragonal structured (c/a $\sim$3) borocarbide superconductors, $YNi_2B_2C$ and $LuNi_2B_2C$, reveal that vortex arrays experience different effective pinning in different crystallographic directions. We surmise that correlation exists between the large anisotropy in effective pinning/disorder and the differences in the (local) symmetry transition from rhombohedral to (quasi) square vortex lattice(VL). For field along high symmetry directions, like, c-axis and ab-basal plane, the VL symmetry is close to square and the ordered state spans a large field interval. When the field is turned away from the c-axis towards ab-plane, at intermediate angles, the region of ordered state shrinks, in response to enhancement in effective pinning. At such intermediate angles the symmetry of the VL would be far from ideal triangular or square.

cond-mat.supr-con↗

arXiv2008

Repeated magnetic compensation behaviour in Nd0.75Gd0.25Rh3B2 alloy having hexagonal structure and planar anisotropy

The results of dc and ac magnetization, electrical resistance and heat capacity studies in an admixed rare earth alloy Nd0.75Gd0.25Rh3B2, which is close to the zero magnetization limit, are reported. Novel observations include the two antiferromagnetic like transitions, concomitant repeated/multiple magnetic compensation behaviour and a characteristic oscillatory magnetic response, with temperature dependence of magnetization at low fields crossing the M = 0 axis thrice. The effective coercive field relating to the residual remanence also has an oscillatory response, with two minima located close to two zero-crossover temperatures. The unusual behavior in Nd0.75Gd0.25Rh3B2 is conjectured to arise from its anisotropic hexagonal structure, with planar anisotropy, resulting in a quasi one dimensional electronic structure and the accentuated role of conduction electron polarization near the zero magnetization limit.

cond-mat.str-el↗

arXiv2006

Manifestation of modulation in spatial order of flux line lattice in weakly pinned superconductors : a vibrating sample magnetometer study

We have investigated the healing of transient disordered vortex states injected into a superconducting sample during the field ramping process in isothermal M-H measurements as a prescription to comprehend the modulation in the state of order of the underlying equilibrium vortex state in weakly pinned single crystals of $2H$-NbSe$_2$ (zero field transition temperature, $T_c(0) \sim 6 K$) and Ca$_3$Rh$_4$Sn$_{13}$ ($T_c(0) \sim 8.2 K$), which display order-disorder transition(s). Our results reaffirm the notion that spatial order in the flux line lattice proceeds to the amorphous state in two distinct steps as evidenced by the presence of second magnetization peak (SMP) anomaly and the peak effect (PE) phenomenon. Disordering commencing at the onset field of SMP has a window to heal between its peak field ($H_{smp}^p$) and the onset field ($H_p^{on}$) of the PE. A comparison of the scan rate dependence of magnetization hysteresis widths in two different crystals of $2H$-NbSe$_2$, one of which displays only the PE phenomenon and the other one that displays both SMP and PE anomalies, show that while enhancment in quenched random pinning invokes the occurence of SMP anomaly, it slows down the temporal decay of currents across the PE region.

cond-mat.supr-con↗

arXiv2006

Evolution in the split-peak structure across the Peak Effect region in single crystals of $2H$-NbSe$_2$

We have explored the presence of a two-peak feature spanning the peak effect (PE) region in the ac susceptibility data and the magnetization hysteresis measurements over a wide field-temperature regime in few weakly pinned single crystals of $2H$-NbSe$_2$, which display reentrant characteristic in the PE curve near $T_c$(0). We believe that the two-peak feature evolves into distinct second magnetization peak anomaly well separated from the PE with gradual enhancement in the quenched random pinning.

cond-mat.supr-con↗

arXiv2005

Critical points in the Bragg glass phase of a weakly pinned crystal of Ca$_3$Rh$_4$Sn$_{13}$

New experimental data are presented on the scan rate dependence of the magnetization hysteresis width $ΔM(H)$ ($\propto$ critical current density $J_c(H)$) in isothermal $M-H$ scans in a weakly pinned single crystal of Ca$_3$Rh$_4$Sn$_{13}$, which displays second magnetization peak (SMP) anomaly as distinct from the peak effect (PE). We observe an interesting modulation in the field dependence of a parameter which purports to measure the dynamical annealing of the disordered bundles of vortices injected through the sample edges towards the destined equilibrium vortex state at a given $H$. These data, in conjunction with the earlier observations made while studying the thermomagnetic history dependence in $J_c(H)$ in the tracing of the minor hysteresis loops, imply that the partially disordered state heals towards the more ordered state between the peak field of the SMP anomaly and the onset field of the PE. The vortex phase diagram in the given crystal of Ca$_3$Rh$_4$Sn$_{13}$ has been updated in the context of the notion of the phase coexistence of the ordered and disordered regions between the onset field of the SMP anomaly and the spinodal line located just prior to the irreversibility line. A multi-critical point and a critical point in the ($H,T$) region of the Bragg glass phase have been marked in this phase diagram and the observed behaviour is discussed in the light of recent data on multi-critical point in the vortex phase diagram in a single crystal of Nb.

cond-mat.supr-con↗

arXiv2005

Effect of pinning and driving force on the metastability effects in weakly pinned superconductors and the determination of spinodal line pertaining to order-disorder transition

We explore the effect of varying drive on metastability features exhibited by the vortex matter in single crystals of 2H-NbSe$_2$ and CeRu$_2$ with varying degree of random pinning. An optimal balance between the pinning and driving force is needed to view the metastability effects in typically weakly pinned specimen of low temperature superconductors. As one uses samples with larger pinning in order to differentiate the response of different metastable vortex states, one encounters a new phenomena, viz., the second magnetization peak (SMP) anomaly prior to the PE. Interplay between the path dependence in the critical current density and the non-linearity in the electromagnetic response determine the metastability effects seen in first and the third harmonic response of the ac susceptibility across the temperature regions of the SMP and the PE. The limiting temperature above which metastability effects cease can be conveniently located in the third harmonic data, and the observed behavior can be rationalized within the Beans Critical State model. A vortex phase diagram showing the different vortex phases for a typically weakly pinned specimen has been constructed via the ac susceptibility data in a crystal of 2H-NbSe$_2$ which shows the SMP and the PE anomalies. The phase space of coexisting weaker and stronger pinned regions has been identified. It can be bifurcated into two parts, where the order and disorder dominate, respectively. The former part continuously connects to the reentrant disordered vortex phase pertaining to the small bundle pinning regime, where the vortices are far apart, interaction effects are weak and the polycrystalline form of flux line lattice prevails.

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arXiv2005

Exploring metastability via the third harmonic measurements in single crystals of $2H$-$NbSe_2$ showing anomalous Peak effect

We explore the metastability effects across the order-disorder transition pertaining to the peak effect phenomenonon in critical current density ($J_c$) via the first and the third harmonic ac susceptibility measurements in the weakly pinned single crystals of $2H$-$NbSe_2$. An analysis of our data suggests that an imprint of the limiting (spinodal) temperature above which $J_c$ is path independent can be conveniently located in the third harmonic data ($χ_{3ω}^{\prime}$).

cond-mat.supr-con↗

arXiv2001

Comparison of History Effects in Magnetization in Weakly pinned Crystals of high-$T_c$ and low-T$_c$ Superconductors

A comparison of the history effects in weakly pinned single crystals of a high $T_c$ YBa$_2$Cu$_3$O$_{7 - δ}$ (for H $\parallel$ c) and a low $T_c$ Ca$_3$Rh$_4$Sn$_{13}$, which show anomalous variations in critical current density $J_c(H)$ are presented via tracings of the minor magnetization hysteresis loops using a vibrating sample magnetometer. The sample histories focussed are, (i) the field cooled (FC), (ii) the zero field cooled (ZFC) and (iii) an isothermal reversal of field from the normal state. An understanding of the results in terms of the modulation in the plastic deformation of the elastic vortex solid and supercooling across order-disorder transition is sought.

cond-mat.supr-con↗

arXiv2001

Vortex Phase Diagram of weakly pinned YBa$_2$Cu$_3$O$_{7-δ}$ for H $\parallel$ c

Vortex phase diagram in a weakly pinned crystal of YBCO for H $\parallel$ c is reviewed in the light of a recent elucidation of the process of `inverse melting' in a Bismuth cuprate system and the imaging of an interface between the ordered and the disordered regions across the peak effect in 2H-NbSe$_2$. In the given YBCO crystal, a clear distinction can be made between the second magnetization peak (SMP) and the peak effect (PE) between 65 K and 75 K. The field region between the peak fields of the SMP (H$^m_{smp}$) and the onset fields of the PE (H$^{on}_{pe}$)is not only continuously connected to the Bragg glass phase at lower fields but it is also sandwiched between the higher temperature vortex liquid phase and the lower temperature vortex glass phase. Thus, an ordered vortex state between H$^m_{smp}$ and H$^{on}_{pe}$ can get transformed to the (disordered) vortex liquid state on heating as well as to the (disordered) vortex glass state on cooling, a situation analogous to the thermal melting and the inverse melting phenomenon seen in a Bismuth cuprate.

cond-mat.supr-con↗

arXiv2000

Establishment of a stable vortex state in the peak effect region in a weakly pinned superconductor CeRu_2

We present magnetization data on a weakly pinned CeRu_2 single crystal showing the existence of a stable state of the vortex lattice in the peak effect region. The stable state is achieved by cycling the magnetic field by small amplitude. This stable state is characterized by a unique value of critical current density (J_c), independent of the magnetic history of the sample. The results support the recent model proposed by Ravikumar et al \cite{r39} on the history dependence of the J_c.

cond-mat.supr-con↗

arXiv2000

Disordered Type-II Superconductors: A Universal Phase Diagram for Low-T$_c$ Systems

A universal phase diagram for weakly pinned low-T$_c$ type-II superconductors is revisited and extended with new proposals. The low-temperature ``Bragg glass'' phase is argued to transform first into a disordered, glassy phase upon heating. This glassy phase, a continuation of the high-field equilibrium vortex glass phase, then melts at higher temperatures into a liquid. This proposal provides an explanation for the anomalies observed in the peak effect regime of 2H-NbSe$_2$ and several other low-T$_c$ materials which is independent of the microscopic mechanisms of superconductivity in these systems.

cond-mat.supr-con↗

arXiv2000

Stable and Metastable vortex states and the first order transition across the peak effect region in weakly pinned 2H-NbSe_2

The peak effect in weakly pinned superconductors is accompanied by metastable vortex states. Each metastable vortex configuration is characterized by a different critical current density J_c, which mainly depends on the past thermomagnetic history of the superconductor. A recent model [G. Ravikumar, et al, Phys. Rev. B 61, R6479 (2000)] proposed to explain the history dependent J_c postulates a stable state of vortex lattice with a critical current density J_c^{st}, determined uniquely by the field and temperature. In this paper, we present evidence for the existence of the stable state of the vortex lattice in the peak effect region of 2H-NbSe_2. It is shown that this stable state can be reached from any metastable vortex state by cycling the applied field by a small amplitude. The minor magnetization loops obtained by repeated field cycling allow us to determine the pinning and "equilibrium" properties of the stable state of the vortex lattice at a given field and temperature unambiguously. The data imply the occurence of a first order phase transition from an ordered phase to a disordered vortex phase across the peak effect.

cond-mat.supr-con↗

arXiv2000

Amorphization of Vortex Matter and Reentrant Peak Effect in YBa$_2$Cu$_3$O$_{7-δ}$

The peak effect (PE) has been observed in a twinned crystal of YBa$_2$Cu$_3$O$_{7-δ}$ for H$\parallel$c in the low field range, close to the zero field superconducting transition temperature (T$_c$(0)) . A sharp depinning transition succeeds the peak temperature T$_p$ of the PE. The PE phenomenon broadens and its internal structure smoothens out as the field is increased or decreased beyond the interval between 250 Oe and 1000 Oe. Moreover, the PE could not be observed above 10 kOe and below 20 Oe. The locus of the T$_p$(H) values shows a reentrant characteristic with a nose like feature located at T$_p$(H)/T$_c$(0)$\approx$0.99 and H$\approx$100 Oe (where the FLL constant a$_0$$\approx$penetration depth $λ$). The upper part of the PE curve (0.5 kOe$<$H$<$10 kOe) can be fitted to a melting scenario with the Lindemann number c$_L$$\approx$0.25. The vortex phase diagram near T$_c$(0) determined from the characteristic features of the PE in YBa$_2$Cu$_3$O$_{7-δ}$(H$\parallel$c) bears close resemblance to that in the 2H-NbSe$_2$ system, in which a reentrant PE had been observed earlier.

cond-mat.supr-con↗

arXiv1999

Peak Effect in Ca$_3$Rh$_4$Sn$_{13}$ : Vortex Phase Diagram and Evidences for Stepwise Amorphization of Flux Line Lattice

The Peak Effect (PE) regime in a single crystal of Ca$_3$Rh$_4$Sn$_{13}$ has been investigated in detail via ac susceptibility as well as dc magnetization measurements. The PE region comprises two discontinuous first order like transitions, located near its onset and peak positions and reflects a stepwise fracturing of the flux line lattice (FLL). This scenario can be construed as an alternative to a scheme involving the appearance of Generalized Fulde-Ferrel-Larkin-Ovchinnikov (GFFLO) state as considered in the case of PE phenomenon in isostructural Yb$_3$Rh$_4$Sn$_{13}$ system. The procedure of thermal cycling across the onset position of PE produces an open hysteresis loop, which is consistent with the notion of the fracturing of the FLL. A study of thermomagnetic history dependence of different metastable vortex states shows the path dependence in the critical current density J_c(H,T) over a large part of the (H,T) parameter space. The path dependence in J_c ceases above the peak position of the PE, suggesting a complete amorphization and the loss of long range correlations of the FLL at (T_p, H_p) line. A plausible vortex phase diagram has been illustrated for Ca$_3$Rh$_4$Sn$_{13}$n and phases like an elastic solid, a plastic solid, a pinned amorphous and an unpinned amorphous states have been identified.

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