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A. Leonhardt

Publications and source records attributed to A. Leonhardt.

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Position Reconstruction in the DEAP-3600 Dark Matter Search Experiment

In the DEAP-3600 dark matter search experiment, precise reconstruction of the positions of scattering events in liquid argon is key for background rejection and defining a fiducial volume that enhances dark matter candidate events identification. This paper describes three distinct position reconstruction algorithms employed by DEAP-3600, leveraging the spatial and temporal information provided by photomultipliers surrounding a spherical liquid argon vessel. Two of these methods are maximum-likelihood algorithms: the first uses the spatial distribution of detected photoelectrons, while the second incorporates timing information from the detected scintillation light. Additionally, a machine learning approach based on the pattern of photoelectron counts across the photomultipliers is explored.

physics.ins-det

Demonstration of the light collection stability of a PEN-based wavelength shifting reflector in a tonne scale liquid argon detector

Liquid argon detectors rely on wavelength shifters for efficient detection of scintillation light. The current standard is tetraphenyl butadiene (TPB), but it is challenging to instrument on a large scale. Poly(ethylene 2,6-naphthalate) (PEN), a polyester easily manufactured as thin sheets, could simplify the coverage of large surfaces with wavelength shifters. Previous measurements have shown that commercial grades of PEN have approximately 50% light conversion efficiency relative to TPB. Encouraged by these results, we conducted a large-scale measurement using $4~m^2$ combined PEN and specular reflector foils in a two-tonne liquid argon dewar to assess its stability over approximately two weeks. This test is crucial for validating PEN as a viable substitute for TPB. The setup used for the measurement of the stability of PEN as a wavelength shifter is described, together with the first results, showing no evidence of performance deterioration over a period of 12 days.

physics.ins-det

A novel cryogenic VUV spectrofluorometer for the characterization of wavelength shifters

We present a novel cryogenic VUV spectrofluorometer designed for the characterization of wavelength shifters (WLS) crucial for experiments based on liquid argon (LAr) scintillation light detection. Wavelength shifters like 1,1,4,4-tetraphenyl-1,3-butadiene (TPB) or polyethylene naphthalate (PEN) are used in these experiments to shift the VUV scintillation light to the visible region. Precise knowledge of the optical properties of the WLS at liquid argon's temperature (87 K) and LAr scintillation wavelength (128 nm) is necessary to model and understand the detector response. The cryogenic VUV spectrofluorometer was commissioned to measure the emission spectra and relative wavelength shifting efficiency (WLSE) of samples between 300 K and 87 K for VUV (128 nm to 190 nm) and UV (310 nm) excitation. New mitigation techniques for surface effects on cold WLS were established. As part of this work, the TPB-based wavelength shifting reflector (WLSR) featured in the neutrinoless double-beta decay experiment LEGEND-200 was characterized. The wavelength shifting efficiency was observed to increase by (54 +/- 5)% from room temperature (RT) to 87 K. PEN installed in LEGEND-200 was also characterized and a first measurement of the relative wavelength shifting efficiency and emission spectrum at RT and 87 K is presented. The WLSE of amorphous PEN was found to be enhanced by at least (37 +/- 4)% for excitation with 128 nm and by (52 +/- 3)% for UV excitation at 87 K compared to RT.

physics.ins-det

Precision Measurement of the Specific Activity of $^{39}$Ar in Atmospheric Argon with the DEAP-3600 Detector

The specific activity of the beta decay of $^{39}$Ar in atmospheric argon is measured using the DEAP-3600 detector. DEAP-3600, located 2 km underground at SNOLAB, uses a total of (3269 $\pm$ 24) kg of liquid argon distilled from the atmosphere to search for dark matter. This detector with very low background uses pulseshape discrimination to differentiate between nuclear recoils and electron recoils and is well-suited to measure the decay of $^{39}$Ar. With 167 live-days of data, the measured specific activity at the time of atmospheric extraction is [0.964 $\pm$ 0.001 (stat) $\pm$ 0.024 (sys)] Bq/kg$_{\rm atmAr}$ which is consistent with results from other experiments. A cross-check analysis using different event selection criteria provides a consistent result.

physics.ins-det

Optical properties of low background PEN structural components for the LEGEND-200 experiment

Polyethylene Naphthalate (PEN) plastic scintillator has been identified as potential self-vetoing structural material in low-background physics experiments. Scintillating components have been produced radio-pure from PEN using injection compression molding technology. These low-background PEN components will be used as active holders to mount the Germanium detectors in the \legend-$200$ neutrinoless double beta decay experiment. In this paper we present the measurement of the optical properties of these PEN components. Thus, the emission spectrum, time constant, attenuation and bulk absorption length as well as light output and light yield are reported. In addition, the surface of these PEN components has been characterized and an estimation of the surface roughness is presented. Moreover, the light output of the final \legend-$200$ detector holders has been measured and is reported. These measurements were used to estimate the self-vetoing efficiency of these holders.

physics.ins-det

Development and characterization of a slow wavelength shifting coating for background rejection in liquid argon detectors

We describe a technique, applicable to liquid-argon-based dark matter detectors, allowing for discrimination of alpha-decays in detector regions with incomplete light collection from nuclear-recoil-like events. Nuclear recoils and alpha events preferentially excite the liquid argon (LAr) singlet state, which has a decay time of ~6 ns. The wavelength-shifter TPB, which is typically applied to the inside of the active detector volume to make the LAr scintillation photons visible, has a short re-emission time that preserves the LAr scintillation timing. We developed a wavelength-shifting polymeric film - pyrene-doped polystyrene - for the DEAP-3600 detector and describe the production method and characterization. At liquid argon temperature, the film's re-emission timing is dominated by a modified exponential decay with time constant of 279(14) ns and has a wavelength-shifting efficiency of 46.4(2.9) % relative to TPB, measured at room temperature. By coating the detector neck (a region outside the active volume where the scintillation light collection efficiency is low) with this film, the visible energy and the scintillation pulse shape of alpha events in the neck region are modified, and we predict that through pulse shape discrimination, the coating will afford a suppression factor of O($10^{5}$) against these events.

physics.ins-det

First direct detection constraints on Planck-scale mass dark matter with multiple-scatter signatures using the DEAP-3600 detector

Dark matter particles with Planck-scale mass ($\simeq10^{19}\text{GeV}/c^2$) arise in well-motivated theories and could be produced by several cosmological mechanisms. Using a blind analysis of data collected over a 813 d live time with DEAP-3600, a 3.3 t single-phase liquid argon-based dark matter experiment at SNOLAB, a search for supermassive dark matter was performed, looking for multiple-scatter signals. No candidate signal events were observed, leading to the first direct detection constraints on Planck-scale mass dark matter. Leading limits constrain dark matter masses between $8.3\times10^{6}$ and $1.2\times10^{19} \text{GeV}/c^2$, and cross sections for scattering on $^{40}$Ar between $1.0\times10^{-23}$ and $2.4\times10^{-18} \text{cm}^2$. These are used to constrain two composite dark matter models.

astro-ph.CO

Direct comparison of PEN and TPB wavelength shifters in a liquid argon detector

A large number of particle detectors employ liquid argon as their target material owing to its high scintillation yield and its ability to drift ionization charge over large distances. Scintillation light from argon is peaked at 128 nm and a wavelength shifter is required for its efficient detection. In this work, we directly compare the light yield achieved in two identical liquid argon chambers, one of which is equipped with PolyEthylene Naphthalate (PEN) and the other with TetraPhenyl Butadiene (TPB) wavelength shifter. Both chambers are lined with enhanced specular reflectors and instrumented with SiPMs with a coverage fraction of approximately 1%, which represents a geometry comparable to the future large scale detectors. We measured the light yield of the PEN chamber to be 39.4$\pm$0.4(stat)$\pm$1.9(syst)% of the yield of the TPB chamber. Using a Monte Carlo simulation this result is used to extract the wavelength shifting efficiency of PEN relative to TPB equal to 47.2$\pm$5.7%. This result paves the way for the use of easily available PEN foils as a wavelength shifter, which can substantially simplify the construction of future liquid argon detectors.

physics.ins-det

Development of very-thick transparent GEMs with wavelength-shifting capability for noble element TPCs

A new concept for the simultaneous detection of primary and secondary scintillation in time projection chambers is proposed. Its core element is a type of very-thick GEM structure supplied with transparent electrodes and machined from a polyethylene naphthalate plate, a natural wavelength-shifter. Such a device has good prospects for scalability and, by virtue of its genuine optical properties, it can improve on the light collection efficiency, energy threshold and resolution of conventional micropattern gas detectors. This, together with the intrinsic radiopurity of its constituting elements, offers advantages for noble gas and liquid based time projection chambers, used for dark matter searches and neutrino experiments. Production, optical and electrical characterization, and first measurements performed with the new device are reported.

physics.ins-det

Pulseshape discrimination against low-energy Ar-39 beta decays in liquid argon with 4.5 tonne-years of DEAP-3600 data

The DEAP-3600 detector searches for the scintillation signal from dark matter particles scattering on a 3.3 tonne liquid argon target. The largest background comes from $^{39}$Ar beta decays and is suppressed using pulseshape discrimination (PSD). We use two types of PSD algorithm: the prompt-fraction, which considers the fraction of the scintillation signal in a narrow and a wide time window around the event peak, and the log-likelihood-ratio, which compares the observed photon arrival times to a signal and a background model. We furthermore use two algorithms to determine the number of photons detected at a given time: (1) simply dividing the charge of each PMT pulse by the charge of a single photoelectron, and (2) a likelihood analysis that considers the probability to detect a certain number of photons at a given time, based on a model for the scintillation pulseshape and for afterpulsing in the light detectors. The prompt-fraction performs approximately as well as the log-likelihood-ratio PSD algorithm if the photon detection times are not biased by detector effects. We explain this result using a model for the information carried by scintillation photons as a function of the time when they are detected.

physics.ins-det

Investigation of the surface properties of different highly aligned N-MWCNT carpets

We investigated the physicochemical surface properties of different highly aligned nitrogen-doped multi-walled carbon nanotube (N-MWCNT) carpets, synthesized using toluene/pyrazine, toluene/benzylamine and acetonitrile via a sublimation-based chemical vapor deposition (SCVD) method at 760°C. The surfaces of the N-MWCNT carpets synthesized using toluene/pyrazine and toluene/benzylamine were very hydrophobic. In contrast, we observed a complete wetting of the N-MWCNT carpets synthesized using acetonitrile. The difference in the wetting behavior of these N-MWCNT carpets is the main focus in this study and was not investigated before. Here, we show that not only the presence or concentration of nitrogen inside the carbon lattice, but especially it's kind of incorporation have an important influence on the surface polarity.

cond-mat.mes-hall

Quantitative magnetic force microscopy on permalloy dots using an iron filled carbon nanotube probe

We have characterized a new Magnetic Force Microscopy (MFM) probe based on an iron filled carbon nanotube (FeCNT) using MFM imaging on permalloy (Py) disks saturated in a high magnetic field perpendicular to the disk plane. The experimental data are accurately modeled by describing the FeCNT probe as having a single magnetic monopole at its tip whose effective magnetic charge is determined by the diameter of the iron wire enclosed in the carbon nanotube and its saturation magnetization 4 πM_s ~ 2.2 x 10^4 G. A magnetic monopole probe enables quantitative measurements of the magnetic field gradient close to the sample surface. The lateral resolution is defined by the diameter of the iron wire ~15 nm and the probe-sample separation. As a demonstration, the magnetic field gradients close to the surface of a Py dot in domain and vortex states were imaged.

cond-mat.mes-hall

Investigation of electric conditions in the vicinity of carbon nanotubes grown in a DC plasma sheath

Carbon nanotubes (CNTs - long tubular carbon nanostructures) belong to the best electron field emitting materials. Based on the experimentally determined electron density in the dual hot filament/DC plasma deposition system the electric field close to the substrate and ion energy flux were calculated. The dependences of electric characteristics close to the nanotube tips on various geometric and plasma parameters were numerically investigated. Taking into account the field enhancement in the vicinity of the CNTs tips the force acting on them was determined. The reliability of numeric computations was tested on a model of conductive sphere placed in a homogeneous electric field, for which theoretical predictions concerning electric forces and field emission currents can be derived.

physics.plasm-ph