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A. Mueller

Publications and source records attributed to A. Mueller.

44 records · Page 3Linked to original sources
arXiv2001

Band structure of MoS_2, MoSe_2, and alpha-MoTe_2: Angle-resolved photoelectron spectroscopy and ab-initio calculations

In this work the complete valence-band structure of the molybdenum dichalcogenides MoS_2, MoSe_2, and alpha-MoTe_2 is presented and discussed in comparison. The valence bands have been studied using both angle-resolved photoelectron spectroscopy (ARPES) with synchrotron radiation, as well as, ab-initio band-structure calculations. The ARPES measurements have been carried out in the constant-final-state (CFS) mode. The results of the calculations show in general very good agreement with the experimentally determined valence-band structures allowing for a clear identification of the observed features. The dispersion of the valence bands as a function of the perpendicular component k_perp of the wave vector reveals a decreasing three-dimensional character from MoS_2 to alpha-MoTe_2 which is attributed to an increasing interlayer distance in the three compounds. The effect of this k_perp dispersion on the determination of the exact dispersion of the individual states as a function of k_parallel is discussed. By performing ARPES in the CFS mode the k_parallel-component for off-normal emission spectra can be determined. The corresponding k_perp-value is obtained from the symmetry of the spectra along the GammaA, KH, and ML line, respectively.

cond-mat.mtrl-sci↗
arXiv2001

Storage ring measurement of the C IV recombination rate coefficient

The low energy C IV dielectronic recombination (DR) rate coefficient associated with 2s-2p Delta n=0 excitations of this lithiumlike ion has been measured with high energy-resolution at the heavy-ion storage-ring TSR of the Max-Planck-Institut fuer Kernphysik in Heidelberg, Germany. The experimental procedure and especially the experimental detection probabilities for the high Rydberg states produced by the recombination of this ion are discussed in detail. From the experimental data a Maxwellian plasma rate coefficient is derived with 15% systematic uncertainty and parameterized for ready use in plasma modeling codes. Our experimental result especially benchmarks the plasma rate coefficient below 10000 K where DR occurs predominantly via C III (1s2 2p 4l) intermediate states and where existing theories differ by orders of magnitude. Furthermore, we find that the total dielectronic and radiative C IV recombination can be represented by the incoherent sum of our DR rate coefficient and the RR rate coefficient of Pequignot et al. (1991, Astron. Astrophys., 251, 680).

astro-ph↗
arXiv2000

Radiative recombination of bare Bi83+: Experiment versus theory

Electron-ion recombination of completely stripped Bi83+ was investigated at the Experimental Storage Ring (ESR) of the GSI in Darmstadt. It was the first experiment of this kind with a bare ion heavier than argon. Absolute recombination rate coefficients have been measured for relative energies between ions and electrons from 0 up to about 125 eV. In the energy range from 15 meV to 125 eV a very good agreement is found between the experimental result and theory for radiative recombination (RR). However, below 15 meV the experimental rate increasingly exceeds the RR calculation and at Erel = 0 eV it is a factor of 5.2 above the expected value. For further investigation of this enhancement phenomenon the electron density in the interaction region was set to 1.6E6/cm3, 3.2E6/cm3 and 4.7E6/cm3. This variation had no significant influence on the recombination rate. An additional variation of the magnetic guiding field of the electrons from 70 mT to 150 mT in steps of 1 mT resulted in periodic oscillations of the rate which are accompanied by considerable changes of the transverse electron temperature.

physics.atom-ph↗
arXiv1999

Dielectronic Recombination of Ground-State and Metastable Li+ Ions

Dielectronic recombination has been investigated for Delta-n = 1 resonances of ground-state Li+(1s^2) and for Delta-n = 0 resonances of metastable Li+(1s2s ^3S). The ground-state spectrum shows three prominent transitions between 53 and 64 eV, while the metastable spectrum exhibits many transitions with energies < 3.2 eV. Reasonably good agreement of R-matrix, LS coupling calculations with the measured recombination rate coefficient is obtained. The time dependence of the recombination rate yields a radiative lifetime of 52.2 +- 5.0 s for the 2 ^3S level of Li+.

physics.atom-ph↗
arXiv1999

Dielectronic Recombination in Photoionized Gas. II. Laboratory Measurements for Fe XVIII and Fe XIX

In photoionized gases with cosmic abundances, dielectronic recombination (DR) proceeds primarily via nlj --> nl'j' core excitations (Dn=0 DR). We have measured the resonance strengths and energies for Fe XVIII to Fe XVII and Fe XIX to Fe XVIII Dn=0 DR. Using our measurements, we have calculated the Fe XVIII and Fe XIX Dn=0 DR DR rate coefficients. Significant discrepancies exist between our inferred rates and those of published calculations. These calculations overestimate the DR rates by factors of ~2 or underestimate it by factors of ~2 to orders of magnitude, but none are in good agreement with our results. Almost all published DR rates for modeling cosmic plasmas are computed using the same theoretical techniques as the above-mentioned calculations. Hence, our measurements call into question all theoretical Dn=0 DR rates used for ionization balance calculations of cosmic plasmas. At temperatures where the Fe XVIII and Fe XIX fractional abundances are predicted to peak in photoionized gases of cosmic abundances, the theoretical rates underestimate the Fe XVIII DR rate by a factor of ~2 and overestimate the Fe XIX DR rate by a factor of ~1.6. We have carried out new multiconfiguration Dirac-Fock and multiconfiguration Breit-Pauli calculations which agree with our measured resonance strengths and rate coefficients to within typically better than <~30%. We provide a fit to our inferred rate coefficients for use in plasma modeling. Using our DR measurements, we infer a factor of ~2 error in the Fe XX through Fe XXIV Dn=0 DR rates. We investigate the effects of this estimated error for the well-known thermal instability of photoionized gas. We find that errors in these rates cannot remove the instability, but they do dramatically affect the range in parameter space over which it forms.

astro-ph↗
arXiv1998

Confinement potential in dual Monopole Nambu-Jona-Lasinio model with dual Dirac strings

Interquark confinement potential is calculated in the dual Monopole Nambu-Jona-Lasinio model with dual Dirac strings as a functional of a dual Dirac string length. The calculation is carried out by the explicit integration over quantum fluctuations of a dual-vector field (monopole-antimonopole collective excitation) around the Abrikosov flux line and string shape fluctuations. The contribution of the scalar field (monopole-antimonopole collective excitation) exchange is taken into account in the tree approximation due to the London limit regime.

hep-th↗
arXiv1998

Quantum and string shape fluctuations in the dual Monopole Nambu-Jona-Lasinio model with dual Dirac strings

The magnetic monopole condensate is calculated in the dual Monopole Nambu-Jona-Lasinio model with dual Dirac strings suggested in Refs.[1,2] as a functional of the dual Dirac string shape. The calculation is carried out in the tree approximation in the scalar monopole-antimonopole collective excitation field. The integration over quantum fluctuations of the dual-vector monopole-antimonopole collective excitation field around the Abrikosov flux line and string shape fluctuations are performed explicitly. We claim that there are important contributions of quantum and string shape fluctuations to the magnetic monopole condensate.

hep-th↗