arXiv subjects

A. S. Moskalenko

Publications and source records attributed to A. S. Moskalenko.

17 recordsLinked to original sources

arXiv2022

Back action in quantum electro-optic sampling of electromagnetic vacuum fluctuations

The influence of measurement back action on electro-optic sampling of electromagnetic quantum fluctuations is investigated. Based on a cascaded treatment of the nonlinear interaction between a near-infrared coherent probe and the mid-infrared vacuum, we account for the generated electric-field contributions that lead to detectable back action. Specifically, we theoretically address two realistic setups, exploiting one or two probe beams for the nonlinear interaction with the quantum vacuum, respectively. The setup parameters at which back action starts to considerably contaminate the measured noise profiles are determined. Due to the vacuum fluctuations entering at the beam splitter, the shot noise of two incoming probe pulses in different channels is uncorrelated. This leads to the absence of the base-level shot noise in the correlation, while further contributions due to nonlinear shot-noise enhancement are still present. Ultimately, the regime in which electro-optic sampling of quantum fields can be considered as effectively back-action free is found.

quant-ph↗

arXiv2018

Spectra of ultrabroadband squeezed pulses and the finite-time Unruh-Davies effect

We study spectral properties of quantum radiation of ultimately short duration. In particular, we introduce a continuous multimode squeezing operator for the description of subcycle pulses of entangled photons generated by a coherent-field driving in a thin nonlinear crystal with second order susceptibility. We find the ultrabroadband spectra of the emitted quantum radiation perturbatively in the strength of the driving field. These spectra can be related to the spectra expected in an Unruh-Davies experiment with a finite time of acceleration. In the time domain, we describe the corresponding behavior of the normally ordered electric field variance.

quant-ph↗

arXiv2018

Negative dynamic conductivity of a current driven array of graphene nanoribbons

We consider a periodic array of graphene nanoribbons under the action of a strong dc electric field $E_0$ and an external electromagnetic excitation with the frequency $ω$ and the lateral wave vector $q$. Solving the quasi-classical Boltzmann kinetic equation and calculating the surface dynamic conductivity $σ_{2D}(q,ω,E_0)$ and the absorption coefficient of such a system we show that the real part of the conductivity and the absorption coefficient may become negative under certain conditions. Physically this corresponds to the amplification of the electromagnetic waves at the expense of the energy of the direct current source. The results are discussed in connection with experiments on the surface acoustic waves and on the Smith-Purcell-type graphene-based terahertz emitter.

cond-mat.mes-hall↗

arXiv2016

Angle-resolved time delay in photoemission of neon

We investigate theoretically the relative time delay of photoelectrons originating from the different subshells (2s and 2p) of neon. This quantity was measured via attosecond streaking and studied theoretically by Schultze et al. [Science 328, 1658 (2010)]. A substantial discrepancy was found between the measured and the calculated values of the relative time delay. Several theoretical studies has been put forward to resolve this issue, e.g. by including correlation effects. In the present paper we explore the directional dependence of the photoelectron emission and the consequences for the inferred time delay. Our quantum mechanical calculations for an electron subject to laser fields and an effective single particle potential show that the time delay is indeed strongly angular dependent. Compared to strict forward emission we find that accounting for emission within a cone of 45 deg aperture, leads to a substantially increase of the relative time delay.

physics.atom-ph↗

arXiv2013

Radiative damping and synchronization in a graphene-based terahertz emitter

We investigate the collective electron dynamics in a recently proposed graphene-based terahertz emitter under the influence of the radiative damping effect, which is included self-consistently in a molecular dynamics approach. We show that under appropriate conditions synchronization of the dynamics of single electrons takes place, leading to a rise of the oscillating component of the charge current. The synchronization time depends dramatically on the applied dc electric field and electron scattering rate, and is roughly inversely proportional to the radiative damping rate that is determined by the carrier concentration and the geometrical parameters of the device. The emission spectra in the synchronized state, determined by the oscillating current component, are analyzed. The effective generation of higher harmonics for large values of the radiative damping strength is demonstrated.

cond-mat.mes-hall↗

arXiv2013

Photovoltaic effect of light carrying orbital angular momentum on a semiconducting stripe

We investigate the influence of a light beam carrying an orbital angular momentum on the current density of an electron wave packet in a semiconductor stripe. It is shown that due to the photo-induced torque the electron density can be deflected to one of the stripe sides. The direction of the deflection is controlled by the direction of the light orbital momentum. In addition the net current density can be enhanced. This is a photovoltaic effect that can be registered by measuring the generated voltage drop across the stripe and/or the current increase.

physics.optics↗

arXiv2012

Attosecond tracking of light absorption and refraction in fullerenes

The collective response of matter is ubiquitous and widely exploited, e.g. in plasmonic, optical and electronic devices. Here we trace on an attosecond time scale the birth of collective excitations in a finite system and find distinct new features in this regime. Combining quantum chemical computation with quantum kinetic methods we calculate the time-dependent light absorption and refraction in fullerene that serve as indicators for the emergence of collective modes. We explain the numerically calculated novel transient features by an analytical model and point out the relevance for ultra-fast photonic and electronic applications. A scheme is proposed to measure the predicted effects via the emergent attosecond metrology.

physics.atm-clus↗

arXiv2011

Photo-induced spin filtering in a double quantum dot

We investigate the spin-resolved electron dynamics in a double quantum dot driven by ultrafast asymmetric electromagnetic pulses. Using a analytical model we show that applying an appropriate pulse sequence allows to control coherently the spin degree of freedom on the femtosecond time scale. It can be achieved that the spin-up state is localized in a selected quantum dot while the spin-down state remains in the other dot. We show that this photo-induced spin-dependent separation can be maintained for a desired period of time.

cond-mat.mes-hall↗

arXiv2010

Direct bandgap optical transitions in Si nanocrystals

The effect of quantum confinement on the direct bandgap of spherical Si nanocrystals has been modelled theoretically. We conclude that the energy of the direct bandgap at the $Γ$-point decreases with size reduction: quantum confinement enhances radiative recombination across the direct bandgap and introduces its "red" shift for smaller grains. We postulate to identify the frequently reported efficient blue emission (F-band) from Si nanocrystals with this zero-phonon recombination. In a dedicated experiment, we confirm the "red" shift of the F-band, supporting the proposed identification.

cond-mat.mtrl-sci↗

arXiv2009

Light-induced valley currents and magnetization in graphene rings

We study the non-equilibrium dynamics in a mesoscopic graphene ring excited by picoseconds shaped electromagnetic pulses. We predict an ultrafast buildup of charge polarization, currents and orbital magnetization. Applying the light pulses identified here, non-equilibrium valley currents are generated in a graphene ring threaded by a stationary magnetic flux. We predict a finite graphene ring magnetization even for a vanishing charge current; the magnetization emerges due to the light-induced difference of the valley populations.

cond-mat.mes-hall↗

arXiv2008

Energy transfer processes in Er-doped SiO2 sensitized with Si nanocrystals

We present a high-resolution photoluminescence study of Er-doped SiO2 sensitized with Si nanocrystals (Si NCs). Emission bands originating from recombination of excitons confined in Si NCs and of internal transitions within the 4f-electron core of Er3+ ions, and a band centered at lambda = 1200nm have been identified. Their kinetics have been investigated in detail. Based on these measurements, we present a comprehensive model for energy transfer mechanisms responsible for light generation in this system. A unique picture of energy flow between subsystems of Er3+ and Si NCs is developed, yielding truly microscopic information on the sensitization effect and its limitations. In particular, we show that most of the Er3+ ions available in the system are participating in the energy exchange. The long standing problem of apparent loss of optical activity of majority of Er dopants upon sensitization with Si NCs is clarified and assigned to appearance of a very efficient energy exchange mechanism between Si NCs and Er3+ ions. Application potential of SiO2:Er sensitized by Si NCs is discussed in view of the newly acquired microscopic insight.

cond-mat.mtrl-sci↗

arXiv2008

Carrier relaxation in Si/SiO$_2$ quantum dots

Carrier relaxation due to both optical and nonradiative intraband transitions in silicon quantum dots in SiO$_2$ has been considered. Interaction of confined holes with optical phonons has been studied. The Huang-Rhys factor is calculated for such transitions. The probability of intraband transition of a confined hole emitting several optical phonons is estimated.

cond-mat.mtrl-sci↗

arXiv2008

Polarized light bursts from kicked quantum rings

Non-equilibrium quantum rings emit circular polarized subterahertz radiation with a polarization degree controllable on nano- to picosecond time scales. This we conclude using a theory developed here for the time-dependent detection of the circular polarization of polychromatic radiations, valid for time scales comparable to the reciprocal of characteristic emission frequencies. The theory is applied to driven quantum rings whereby the influence of radiative and non-radiative processes on the properties of the emitted light is incorporated.

quant-ph↗

arXiv2007

Nonequilibrium charge dynamics of light-driven rings threaded by a magnetic flux

We study theoretically the charge polarization and the charge current dynamics of a mesoscopic ring driven by short asymmetric electromagnetic pulses and threaded by an external static magnetic flux. It is shown that the pulse-induced charge polarization and the associated light-emission is controllable by tuning the external magnetic flux. Applying two mutually perpendicular pulses triggers a charge current in the ring. The interplay between this nonequilibrium and the persistent currents is investigated and the conditions under which the pulses stop the persistent current are identified.

cond-mat.mes-hall↗

arXiv2007

Single-particle states in spherical Si/SiO$_2$ quantum dots

We calculate ground and excited electron and hole levels in spherical Si quantum dots inside SiO$_2$ in a multiband effective mass approximation. Luttinger Hamiltonian is used for holes and the strong anisotropy of the conduction electron effective mass in Si is taken into account. As boundary conditions for electron and hole wave functions we use continuity of the wave functions and the velocity density at the boundary of the quantum dots.

cond-mat.mtrl-sci↗

arXiv2006

Revivals, collapses and magnetic-pulse generation in quantum rings

Using a microscopic theory based on the density matrix formalism we investigate quantum revivals and collapses of the charge polarization and charge current dynamics in mesoscopic rings driven by short asymmetric electromagnetic pulses. The collapsed state is utilized for sub-picosecond switching of the current and associated magnetization, enabling thus the generation of pulsed magnetic fields with a tunable time structure and shape asymmetry which provides a new tool to study ultrafast spin-dynamics and ratchet-based effects.

cond-mat.mes-hall↗

arXiv2003

Magnetic field effect on tunnel ionization of deep impurities by terahertz radiation

A suppression of tunnelling ionization of deep impurities in terahertz frequency electric fields by a magnetic field is observed. It is shown that the ionization probability at external magnetic field, B, oriented perpendicular to the electric field of terahertz radiation, E, is substantially smaller than that at B || E. The effect occurs at low temperatures and high magnetic fields.

cond-mat↗