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A. Shrivastava

Publications and source records attributed to A. Shrivastava.

At least 19 recordsLinked to original sources

Investigation of reaction and $α$ production cross sections with $^9$Be projectile

In order to investigate the contribution of $α$ production in the reaction cross sections, measurements of elastic scattering and inclusive $α$ particle angular distributions have been carried out with the $^9$Be projectile on $^{89}$Y, $^{124}$Sn, $^{159}$Tb, $^{198}$Pt, and $^{209}$Bi targets over a wide angular range at energies near the Coulomb barrier. The measured elastic scattering angular distributions were fitted with optical model calculations, and reaction cross sections were extracted. The same data were also analysed using both global optical model potentials (Global OMP) and microscopic S$\tilde{a}$o Paulo potentials (SPP), to obtain the reaction cross sections. The data available in the literature for $^9$Be projectile includes the elastic scattering angular distributions, $α$ production cross sections, and complete fusion cross sections on these and other targets at several energies are also utilised for comparative studies. The reaction cross section extracted from the three potentials (Best Fit, Global OMP and SPP) are in reasonable agreement for all the targets except for the energies below the barrier where the results from SPP deviate by 30-50 \%. Inclusive $α$ particle production cross sections were also extracted by integrating the $α$ particle angular distributions. The present data and data available from literature of reaction and $α$-particle production cross sections were utilised to make systematic studies. Systematics of reaction and $α$-particle production cross sections revealed their universal behaviour.

nucl-ex

Fusion of $^{7}$Li with $^{205}$Tl at near barrier energies

The complete and incomplete fusion cross sections for the $^{7}$Li+$^{205}$Tl reaction were measured at near barrier energies by online characteristic $γ$ ray detection technique. The complete fusion (CF) cross sections at energies above the Coulomb barrier were found to be suppressed by $\sim$ 26 \% compared to the coupled channel calculations. Reduced fusion cross sections for the present system at energies normalised to the Coulomb barrier were also found to be systematically lower than those with strongly bound projectiles forming a similar compound nucleus. The suppression observed in CF cross sections is found to be commensurate with the measured total incomplete fusion (ICF) cross sections. In the ICF cross sections, t capture is found to be dominant than $α$ capture at all the measured energies. The systematic study of available CF, ICF and total fusion (TF) data with $^7$Li projectile is performed.

nucl-ex

Experimental Evidence of Large Collective Enhancement of Nuclear Level Density and its Significance in Radiative Neutron Capture

The collective enhancement of nuclear level density and its fade out with excitation energy in deformed $^{171}$Yb nucleus has been inferred through an exclusive measurement of neutron spectra.The statistical model analysis of neutron spectra demonstrated a large collective enhancement factor of 40$\pm$3 for the first time, which corroborates with the recent microscopic model predictions but is an anomalous result compared with the measurements in the nearby deformed nuclei. The complete picture of the energy dependent collective enhancement has been obtained by combining with Oslo data below neutron binding energy. The significance of large collective enhancement in radiative neutron capture cross section of astrophysical interest is highlighted.

nucl-ex

An analytical model for electronic noise in a cryogenic bolometer detector readout circuit

This paper presents an analytical model to quantify the measured noise in a cryogenic bolometer readout circuit. The model includes the contributions from the bias resistors and sensor resistors, voltage and current noise of amplifier, and cable capacitance. The model parameters are empirically estimated using frequency domain analysis of the measured noise data of indigenously developed Neutron Transmutation Doped (NTD) Ge sensors. The model is shown to describe noise data for NTD Ge sensors over a wide range of resistances corresponding to temperatures in the range 20 - 70 mK. Relative contributions of different components are discussed and it is shown that the contribution to the overall noise from the differential amplifier at 300 K is the dominant source. It is observed that the amplifier flicker noise is significantly lower than that specified in the amplifier datasheet. The present study also indicates that a desirable value of resistance of NTD sensor (R$_{NTD}$) from noise considerations is $\leq$ 1 G$Ω$ at $sim$ 20 mK.

physics.ins-det

Neutron transfer in $^{9}$Be + $^{159}$Tb system

One neutron stripping cross sections ($σ_{-1n}$) are measured in $^{9}$Be+$^{159}$Tb system in the energy range E$_{cm}$/V$_{B}$ $\sim$ 0.79 - 1.24 using offline gamma counting technique. The CRC model calculations including the ground state and the 2$^{+}$ resonance state of $^{8}$Be, carried out using the FRESCO code, give a reasonable description of the measured data. In addition, comparisons of reduced 1n-stripping cross sections- $σ_{red}$ with $^{9}$Be for different target nuclei (A $\sim$150-200), and $σ_{red}$ for $^{9}$Be, $^{6}$Li with $^{159}$Tb target are presented. While no strong target dependence is observed with $^{9}$Be projectile, $σ_{red}$($^{9}$Be) is significantly larger than that for $^{6}$Li, which is consistent with the Q-value for transfer reactions and breakup threshold energy of projectiles.

nucl-ex

Unraveling the reaction mechanism for large alpha production and incomplete fusion in reactions involving weakly bound stable nuclei

The origin of the large $α$ particle production and incomplete fusion in reactions involving weakly-bound $α$+$x$ cluster nuclei still remains unresolved. While the (two-step) process of breakup followed by capture of the ``free" complementary fragment ($x$) is widely believed to be responsible, a few recent studies suggest the dominant role of (direct) cluster stripping. To achieve an unambiguous experimental discrimination between these two processes, a coincidence measurement between the outgoing $α$ particles and $γ$ rays from the heavy residues has been performed for the $^7$Li($α$+triton)+$^{93}$Nb system. Proper choice of kinematical conditions allowed for the first time a significant population of the region accessible only to the direct triton stripping process and not to breakup followed by the capture of the ``free'' triton (from the three-body continuum). This result, also supported by a cluster-transfer calculation, clearly establishes the dominance of the direct cluster-stripping mechanism in the large alpha production.

nucl-ex

Fusion of 16O+165Ho at deep sub-barrier energies

Fusion cross-sections have been measured for the asymmetric system 16O+165Ho at energies near and deep below the Coulomb barrier with an aim to investigate the occurrence of fusion hindrance for the system. Fusion cross sections down to ~ 700 nb have been measured using the off-beam gamma-ray technique. The fusion cross sections have been compared with the coupled channel calculations. Although the onset of fusion hindrance could not be observed experimentally, an indication of a small deviation of the experimental fusion cross-sections with respect to the calculated cross-sections could be observed at the lowest energy measured. However, the energy onset of fusion hindrance has been obtained from the extrapolation technique and is found to be about 2 MeV below the lowest energy of the present measurement.

nucl-ex

Investigating neutron transfer in the $^{9}$Be + $^{197}$Au system

In this work $\textit{n}$-transfer and incomplete fusion cross sections for $^{9}$Be + $^{197}$Au system are reported over a wide energy range, E$_{c.m.}$ $\approx$ 29-45 MeV. The experiment was carried out using activation technique and off-line gamma counting. The transfer process is found to be the dominant mode as compared to all other reaction channels. Detailed coupled reaction channel (CRC) calculations have been performed for $\textit{n}$-transfer stripping and pickup cross sections. The measured 1$\textit{n}$-stripping cross sections are explained with CRC calculations by including the ground state and the 2$^{+}$ resonance state (E = 3.03 MeV) of $^{8}$Be. The calculations for 1$\textit{n}$-pickup, including only the ground state of $^{10}$Be agree reasonably well with the measured cross sections, while it overpredicts the data at subbarrier energies. For a better insight into the role of projectile structure in the transfer process, a comprehensive analysis of 1$\textit{n}$-stripping reaction has been carried out for various weakly bound projectiles on $^{197}$Au target nucleus. The transfer cross sections scaled with the square of total radius of interacting nuclei show the expected Q-value dependence of 1$\textit{n}$-stripping channel for weakly bound stable projectiles.

nucl-ex

Synchrotron x-ray diffraction studies of the $α\rightleftharpoons β$ structural phase transition in Sn and Sn-Cu

The transformation between the metallic ($β$) and semi-conducting ($α$) allotropes of tin is still not well understood. The phase transition temperature stated in the literature, 286.2 K, seems to be inconsistent with recent calorimetric measurements. In this paper, this intriguing aspect has been explored in Sn and Sn-Cu (alloyed 0.5% Cu by weight) using temperature resolved synchrotron x-ray diffraction measurements performed at the Indus-2 facility. Additionally, the $α\rightleftharpoons β$ Sn transition has been recorded using in-situ heating/cooling experiments in a scanning electron microscope. Based on these measurements, a protocol has been suggested to reduce the formation of $α$-Sn in potentially susceptible systems. This will be useful in experiments like TIN.TIN (The INdia-based TIN detector), which proposes to employ ~100 - 1000 kg of superconducting tin-based detectors to search for neutrinoless double beta decay in the isotope $^{124}$Sn.

cond-mat.mtrl-sci

Large back-angle quasielastic scattering for $^{7}$Li+$^{159}$Tb

Quasielastic scattering excitation function at large backward angle has been measured for the weakly bound system, $^{7}$Li+$^{159}$Tb at energies around the Coulomb barrier. The corresponding quasielastic barrier distribution has been derived from the excitation function, both including and excluding the $α$-particles produced in the reaction. The centroid of the barrier distribution obtained after inclusion of $α$-particles was found to be shifted higher in energy, compared to the distribution excluding the $α$-particles. The quasielastic data, excluding the $α$-particles, have been analyzed in the framework of continuum discretized coupled channel calculations. The quasielastic barrier distribution for $^{7}$Li+$^{159}$Tb, has also been compared with the fusion barrier distribution for the system.

nucl-ex

A Unifying Framework for Formal Theories of Novelty:Framework, Examples and Discussion

Managing inputs that are novel, unknown, or out-of-distribution is critical as an agent moves from the lab to the open world. Novelty-related problems include being tolerant to novel perturbations of the normal input, detecting when the input includes novel items, and adapting to novel inputs. While significant research has been undertaken in these areas, a noticeable gap exists in the lack of a formalized definition of novelty that transcends problem domains. As a team of researchers spanning multiple research groups and different domains, we have seen, first hand, the difficulties that arise from ill-specified novelty problems, as well as inconsistent definitions and terminology. Therefore, we present the first unified framework for formal theories of novelty and use the framework to formally define a family of novelty types. Our framework can be applied across a wide range of domains, from symbolic AI to reinforcement learning, and beyond to open world image recognition. Thus, it can be used to help kick-start new research efforts and accelerate ongoing work on these important novelty-related problems. This extended version of our AAAI 2021 paper included more details and examples in multiple domains.

cs.AI

Evidence for the general dominance of proton shells in low-energy fission

A regular pattern, revealing the leading role of the light-fragment nuclear charge, is found to emerge from a consistent analysis of the experimental information collected recently on low-energy asymmetric fission of neutron-deficient nuclei around lead. The observation is corroborated by a theoretical investigation within a microscopic framework, suggesting the importance of proton configurations driven by quadrupole-octupole correlations. This is in contrast to the earlier theoretical interpretations in terms of dominant neutron shells. The survey of a wider area of the nuclear chart by a semi-empirical approach points to the lack of understanding of the competition between the different underlying macroscopic and microscopic forces in a quantitative manner. Combined with previously identified stabilizing forces, the present finding shows a striking connection between the "old" (actinide) and "new" (pre-actinide) islands of asymmetric fission which could steer the strive for an unified theory of fission.

nucl-th

Nickel Hexacyanoferrate Electrodes for Continuous Cation Intercalation Desalination of Brackish Water

Using porous electrodes containing nickel hexacyanoferrate (NiHCF) nanoparticles, we construct and test a device for capacitive deionization in a two flow-channel device where the intercalation electrodes are in direct contact with an anion-exchange membrane. Upon negatively charging NiHCF, cations intercalate into it and the water in its vicinity is desalinated; at the same time water in the opposing electrode becomes more saline upon positively charging the NiHCF in that electrode. In a cyclic process of charge and discharge, fresh water is continuously produced, alternating between the two channels in sync with the direction of applied current. We present proof-of-principle experiments of this technology for single salt solutions, where we analyze various levels of current and cycle durations. We analyze salt removal rate and energy consumption. In desalination experiments with salt mixtures we find a threefold enhancement for K$^+$ over Na$^+$-adsorption, which shows the potential of NiHCF intercalation electrodes for selective ion separation from mixed ionic solutions.

physics.chem-ph

Competing quasifission and asymmetric fusion-fission in neutron-deficient sub-lead nuclei

To disentangle the role of shell effects and dynamics, fission fragment mass distributions of $^{191}$Au, a nucleus in the newly identified island of mass asymmetric fission in the sub-lead region, have been measured down to excitation energy of $\approx$20 MeV above the fission barrier via two different entrance channels, viz. $^{16}$O+$^{175}$Lu and $^{37}$Cl+$^{154}$Sm reactions. Apart from having signature of the shell effects in both the cases, clear experimental evidence of quasifission has been observed in the mass distributions of the Cl induced reaction, that has also been substantiated by the theoretical calculations. This crucial evidence along with a systematic analysis of available experimental data has revealed that the dynamics in the entrance channel has significant influence on most of the reactions used earlier to explore the persistence of recently discovered mass asymmetry in $β$-delayed fission at low energy in this mass region, ignoring which might lead to ambiguity in interpreting the heavy-ion data.

nucl-ex

Fusion of Borromean nucleus $^{9}$Be with $^{197}$Au target at near barrier energies

To probe the role of the intrinsic structure of the projectile on sub-barrier fusion, measurement of fusion cross sections has been carried out in $^{9}$Be + $^{197}$Au system in the energy range E$_{c.m.}$/V$_B$ $\approx$ 0.82 to 1.16 using off-beam gamma counting method. Measured fusion excitation function has been analyzed in the framework of the coupled-channel approach using CCFULL code. It is observed that the coupled-channel calculations, including couplings to the inelastic state of the target and the first two states of the rotational band built on the ground state of the projectile, provide a very good description of the sub-barrier fusion data. At above barrier energies, the fusion cross section is found to be suppressed by $\approx$ 39(2)\% as compared to the coupled-channel prediction. A comparison of reduced excitation function of $^{9}$Be + $^{197}$Au with other $x$ + $^{197}$Au shows a larger enhancement for $^9$Be in the sub-barrier region amongst Z=2-5 weakly and tightly bound projectiles, which indicates the prominent role of the projectile deformation in addition to the weak binding.

nucl-ex

Interpretation of coincidence data from strip detectors and extraction of absolute cross section using 3-body Monte Carlo simulation method

Accurate knowledge of the response of the detection system is very crucial for unambiguous interpretation of the experimental data. A simulation code has been developed using the Monte Carlo technique involving 3-body kinematics for the analysis of data obtained with segmented large area Si $ΔE-E$ detector telescopes in nuclear reaction measurements. Care was taken in the analysis to maximize the angular coverage and statistics. The emphasis is placed to extract the absolute cross sections of the different reaction processes, for which coincident measurements are unavoidable. The estimated detection efficiency of different coincidence events are found to depend on various parameters, e.g., the relative energy of the breakup fragments, incident beam energy of the projectile, ground state $Q$-value of the reaction, the excitation of the ejectile as well as target like nuclei, mass asymmetry of the breakup fragments, detection threshold, and geometric solid angle of the detection setup. The interpretation of the various observables from the exclusive measurements of breakup and transfer breakup reactions is reported.

physics.ins-det

Particle identification using digital pulse shape discrimination in a nTD silicon detector with a 1 GHz sampling digitizer

In beam test experiments have been carried out for particle identification using digital pulse shape analysis in a 500~$μ$m thick Neutron Transmutation Doped (nTD) silicon detector with an indigenously developed FPGA based 12 bit resolution, 1 GHz sampling digitizer. The nTD Si detector was used in a low-field injection setup to detect light heavy-ions produced in reactions of $\sim$ 5 MeV/A $^{7}$Li and $^{12}$C beams on different targets. Pulse height, rise time and current maximum have been obtained from the digitized charge output of a high bandwidth charge and current sensitive pre-amplifier. Good isotopic separation have been achieved using only the digitized charge output in case of light heavy-ions. The setup can be used for charged particle spectroscopy in nuclear reactions involving light heavy-ions around the Coulomb barrier energies.

physics.ins-det