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A. Shrivastava

Publications and source records attributed to A. Shrivastava.

35 records · Page 2Linked to original sources

Investigation of complete and incomplete fusion in $^{7}$Li+$^{124}$Sn reaction around Coulomb barrier energies

The complete and incomplete fusion cross sections for $^{7}$Li+$^{124}$Sn reaction were measured using online and offline characteristic $γ$-ray detection techniques. The complete fusion (CF) cross sections at energies above the Coulomb barrier were found to be suppressed by $\sim$ 26 \% compared to the coupled channel calculations. This suppression observed in complete fusion cross sections is found to be commensurate with the measured total incomplete fusion (ICF) cross sections. There is a distinct feature observed in the ICF cross sections, i.e., $\textit{t}$-capture is found to be dominant than $α$-capture at all the measured energies. A simultaneous explanation of complete, incomplete and total fusion (TF) data was also obtained from the calculations based on Continuum Discretized Coupled Channel method with short range imaginary potentials. The cross section ratios of CF/TF and ICF/TF obtained from the data as well as the calculations showed the dominance of ICF at below barrier energies and CF at above barrier energies.

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Probing transfer to unbound states of the ejectile with weakly bound 7Li on 93Nb

The two-step process of transfer followed by breakup is explored by measuring a rather complete set of exclusive data for reaction channels populating states in the ejectile continua of the $^7$Li+$^{93}$Nb system at energies close to the Coulomb barrier. The cross sections for $α+α$ events from one proton pickup were found to be smaller than those for $α+d$ events from one neutron stripping and $α+t$ events from direct breakup of $^7$Li. Coupled channels Born approximation and continuum discretized coupled channels calculations describe the data well and support the conclusion that the $α+d$ and $α+α$ events are produced by direct transfer to unbound states of the ejectile.

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No influence of a N=126 Neutron Shell Closure in Fission Fragment Mass Distributions

Mass distributions of the fragments in the fission of $^{206}$Po and the N=126 neutron shell closed nucleus $^{210}$Po have been measured. No significant deviation of mass distributions has been found between $^{206}$Po and $^{210}$Po, indicating the absence of shell correction at the saddle point in both the nuclei, contrary to the reported angular anisotropy and pre-scission neutron multiplicity results. This new result provides benchmark data to test the new fission dynamical models to study the effect of shell correction on the potential energy surface at saddle point.

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Characterization of the scission point from fission-fragment velocities

The isotopic-yield distributions and kinematic properties of fragments produced in transfer-induced fission of 240Pu and fusion-induced fission of 250Cf, with 9 MeV and 45 MeV of excitation energy respectively, were measured in inverse kinematics with the spectrometer VAMOS. The kinematic properties of identified fission fragments allow to derive properties of the scission configuration such as the distance between fragments, the total kinetic energy, the neutron multiplicity, the total excitation energy, and, for the first time, the proton- and neutron-number sharing during the emergence of the fragments. These properties of the scission point are studied as functions of the fragment atomic number. The correlation between these observables, gathered in one single experiment and for two different fissioning systems at different excitation energies, give valuable information for the understanding and modeling of the fission process.

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Radiation Background Studies for 0$νββ$ decay in $^{124}$Sn

Radiation background studies pertaining to $0νββ$ decay in $^{124}$Sn have been carried out. A TiLES setup has been installed at TIFR for this purpose. Neutron-induced background is studied in the TIN.TIN detector materials using fast neutron activation technique. The neutron flux ($E_n\leq15$ MeV) resulting from SF and ($α, n$) interactions for the rock in the INO cavern is estimated using MC simulations. A two layer composite shield of borated paraffin (20 cm) + Pb (5 cm) is proposed for the reduction of neutron flux.

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Characterization of neutron transmutation doped (NTD) Ge for low temperature sensor development

Development of NTD Ge sensors has been initiated for low temperature (mK) thermometry in The India-based Tin detector (TIN.TIN). NTD Ge sensors are prepared by thermal neutron irradiation of device grade Ge samples at Dhruva reactor, BARC, Mumbai. Detailed measurements have been carried out in irradiated samples for estimating the carrier concentration and fast neutron induced defects. The Positron Annihilation Lifetime Spectroscopy (PALS) measurements indicated monovacancy type defects for all irradiated samples, while Channeling studies employing RBS with 2 MeV alpha particles, revealed no significant defects in the samples exposed to fast neutron fluence of $\sim 4\times10^{16}/cm^2$. Both PALS and Channeling studies have shown that vacuum annealing at 600 $^\circ$C for $\sim2$ hours is sufficient to recover the damage in the irradiated samples, thereby making them suitable for the sensor development.

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Study of Radioactive Impurities in Neutron Transmutation Doped Germanium

A program to develop low temperature (mK) sensors with neutron transmutation doped Ge for rare event studies with a cryogenic bolometer has been initiated. For this purpose, semiconductor grade Ge wafers are irradiated with thermal neutron flux from Dhruva reactor at BARC, Mumbai. Spectroscopic studies of irradiated samples have revealed that the environment of the capsule used for irradiating the sample leads to significant levels of $^{65}$Zn, $^{110}$Ag and $^{182}$Ta impurities, which can be reduced by chemical etching of approximately $\sim50 μ$m thick surface layer. From measurements of the etched samples in the low background counting setup, activity due to trace impurities of $^{123}$Sb in bulk Ge is estimated to be $\sim$ 1 Bq/gm after irradiation. These estimates indicate that in order to use the NTD Ge sensors for rare event studies, a cool down period of $\sim$ 2 years would be necessary to reduce the radioactive background to $\le$ 1 mBq/gm.

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Study of neutron-induced background and its effect on the search of 0$νββ$ decay in $\rm^{124}Sn$

Neutron-induced background has been studied in various components of the TIN.TIN detector, which is under development for the search of Neutrinoless Double Beta Decay in $\rm^{124}Sn$. Fast neutron flux $\sim10^{6}~n~cm^{-2}s^{-1}$ covering a broad energy range ($ \sim0.1$ to $ \sim18$~MeV) was generated using $^{9}Be(p,n)^{9}B$ reaction. In addition, reactions with quasi-monoenergetic neutrons were also studied using $^{7}Li(p,n)^{7}Be$ reaction. Among the different cryogenic support structures studied, Teflon is found to be preferable compared to Torlon as there is no high energy gamma background ($E_γ>$ 1 MeV). Contribution of neutron-induced reactions in $\rm ^{nat, 124} $Sn from other Sn isotopes (A = 112 -- 122) in the energy region of interest, namely, around the $Q_{ββ}$ of $\rm^{124}Sn$ ($E \sim$ 2.293 MeV), is also investigated.

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Electromagnetic transition from the 4$^+$ to 2$^+$ resonance in $^8$Be measured via the radiative capture in $^4$He+$^4$He

An earlier measurement on the 4$^+$ to 2$^+$ radiative transition in $^8$Be provided the first electromagnetic signature of its dumbbell-like shape. However, the large uncertainty in the measured cross section does not allow a stringent test of nuclear structure models. The present paper reports a more elaborate and precise measurement for this transition, via the radiative capture in the $^4$He+$^4$He reaction, improving the accuracy by about a factor of three. The {\it ab initio} calculations of the radiative transition strength with improved three-nucleon forces are also presented. The experimental results are compared with the predictions of the alpha cluster model and {\it ab initio} calculations.

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Isotopic Yield Distributions of Transfer- and Fusion-Induced Fission from 238U+12C Reactions in Inverse Kinematics

A novel method to access the complete identification in atomic number Z and mass A of fragments produced in low-energy fission of actinides is presented. This method, based on the use of multi- nucleon transfer and fusion reactions in inverse kinematics, is applied in this work to reactions between a 238U beam and a 12C target to produce and induce fission of moderately excited actinides. The fission fragments are detected and fully identified with the VAMOS spectrometer of GANIL, allowing the measurement of fragment yields of several hundreds of isotopes in a range between A ~ 80 and ~ 160, and from Z ~ 30 to ~ 64. For the first time, complete isotopic yield distributions of fragments from well-defined fissioning systems are available. Together with the precise measurement of the fragment emission angles and velocities, this technique gives further insight into the nuclear-fission process.

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Complex fragment emission in low energy light-ion reactions

Inclusive energy spectra of the complex fragments (3 $\leq$ Z $\leq$ 5) emitted in the reactions $^{12}$C (77 MeV)+ $^{28}$Si, $^{11}$B (64 MeV)+ $^{28}$Si and $^{12}$C (73 MeV)+ $^{27}$Al (all having the same excitation energy of $ \sim$ 67 MeV), have been measured in the angular range of 10$^\circ$ $\lesssim θ_{lab} \lesssim$ 60$^\circ$. The fully energy damped (fusion-fission) and the partially energy damped (deep inelastic) components of the fragment energy spectra have been extracted. It has been found that the yields of the fully energy damped fragments for all the above reactions are in conformity with the respective statistical model predictions. The time scales of various deep inelastic fragment emissions have been extracted from the angular distribution data. The angular momentum dissipation in deep inelastic collisions has been estimated from the data and it has been found to be close to the corresponding sticking limit value.

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Role of the cluster structure of $^7$Li in the dynamics of fragment capture

Exclusive measurements of prompt $γ$-rays from the heavy-residues with various light charged particles in the $^7$Li + $^{198}$Pt system, at an energy near the Coulomb barrier (E/$V_b$ $\sim$ 1.6) are reported. Recent dynamic classical trajectory calculations, constrained by the measured fusion, $α$ and $t$ capture cross-sections have been used to explain the excitation energy dependence of the residue cross-sections. These calculations distinctly illustrate a two step process, breakup followed by fusion in case of the capture of $t$ and $α$ clusters; whereas for $^{6}$He + $p$ and $^{5}$He + $d$ configurations, massive transfer is inferred to be the dominant mechanism. The present work clearly demonstrates the role played by the cluster structures of $^7$Li in understanding the reaction dynamics at energies around the Coulomb barrier.

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Lifetime measurements in $^{63}$Co and $^{65}$Co

Lifetimes of the $9/2^-_1$ and $3/2^-_1$ states in $^{63}$Co and the $9/2^-_1$ state in $^{65}$Co were measured using the recoil distance Doppler shift and the differential decay curve methods. The nuclei were populated by multi-nucleon transfer reactions in inverse kinematics. Gamma rays were measured with the EXOGAM Ge array and the recoiling fragments were fully identified using the large-acceptance VAMOS spectrometer. The E2 transition probabilities from the $3/2^-_1$ and $9/2^-_1$ states to the $7/2^-$ ground state could be extracted in $^{63}$Co as well as an upper limit for the $9/2^-_1\rightarrow7/2^-_1$ $B$(E2) value in $^{65}$Co. The experimental results were compared to large-scale shell-model calculations in the $pf$ and $pfg_{9/2}$ model spaces, allowing to draw conclusions on the single-particle or collective nature of the various states.

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Probing pre-formed alpha particles in the ground state of nuclei

In this Letter, we report on alpha particle emission through the nuclear break-up in the reaction 40Ca on a 40Ca target at 50A MeV. It is observed that, similarly to nucleons, alpha particles can be emitted to the continuum with very specific angular distribution during the reaction. The alpha particle properties can be understood as resulting from an alpha cluster in the daughter nucleus that is perturbed by the short range nuclear attraction of the collision partner and emitted. A time-dependent theory that describe the alpha particle wave-function evolution is able to reproduce qualitatively the observed angular distribution. This mechanism offers new possibilities to study alpha particle properties in the nuclear medium.

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The study of threshold behaviour of effective potential for $^{6}$Li+$^{58,64}$Ni systems

The elastic scattering for $^6$Li+$^{64}$Ni system was measured in the bombarding energy range of 13 MeV $\leq$ $E_{lab}$ $\leq$ 26 MeV. A phenomenological optical model analysis was performed and the behaviour of the surface strengths of the potential components with decreasing energy was extracted. A further analysis of the measured angular distributions, along with the existing data for $^6$Li+$^{58}$Ni, was performed with two different model potentials - one with the folded potential normalized with a complex factor (OMP1) and the other with a {\it hybrid} potential composed of a renormalized folded real and a phenomenological imaginary (OMP2) potential components - were used in the calculation. All the model potentials predict similar energy dependent behaviour for the interaction potential around the barrier. The observed energy dependence of the strengths of the real and imaginary potentials corroborate with the dispersion relation prediction for both the $^6$Li+$^{64}$Ni and $^6$Li+$^{58}$Ni systems. Though the evidence of breakup is distinct in the energy variation of the potential strengths, close to the barrier the variation is more in the line of conventional threshold anomaly. Also the threshold behaviour of the interaction potential does not indicate any distinct isotopic dependence.

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Evidence for transfer followed by breakup in 7Li + 65Cu

The observation of a large cross-section for the alpha + d channel compared to breakup into the alpha + t channel from an exclusive measurement for the 7Li+65Cu system at 25 MeV is presented. A detailed analysis of the angular distribution using coupled channels Born approximation calculations has provided clear evidence that the observed alpha + d events arise from a two step process, i.e. direct transfer to the 2.186 MeV (3+) resonance in the alpha + d continuum of 6Li followed by breakup, and are not due to final state interaction effects.

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Exclusive light particle measurements for the system $^{19}$F + $^{12}$C at 96 MeV

Decay sequence of hot ${31}^$P nucleus has been investigated through exclusive light charged particle measurements in coincidence with individual evaporation residues using the reaction ${19}^$F (96 MeV) + ${12}^$C. Information on the sequential decay chain have been extracted by confronting the data with the predictions of the statistical model. It is observed from the present analysis that such exclusive light charged particle data may be used as a powerful tool to probe the decay sequence of the hot light compound systems.

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