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A. Simon

Publications and source records attributed to A. Simon.

At least 73 records · Page 4Linked to original sources

Results of the material screening program of the NEXT experiment

The 'Neutrino Experiment with a Xenon TPC (NEXT)', intended to investigate neutrinoless double beta decay, requires extremely low background levels. An extensive material screening and selection process to assess the radioactivity of components is underway combining several techniques, including germanium gamma-ray spectrometry performed at the Canfranc Underground Laboratory; recent results of this material screening program are presented here.

physics.ins-det↗

Novel technique for constraining r-process (n,$γ$) reaction rates

A novel technique has been developed, which will open exciting new opportunities for studying the very neutron-rich nuclei involved in the r-process. As a proof-of-principle, the $γ$-spectra from the $β$-decay of $^{76}$Ga have been measured with the SuN detector at the National Superconducting Cyclotron Laboratory. The nuclear level density and $γ$-ray strength function are extracted and used as input to Hauser-Feshbach calculations. The present technique is shown to strongly constrain the $^{75}$Ge($n,γ$)$^{76}$Ge cross section and reaction rate.

nucl-ex↗

Measurement of the $^{58}$Ni($α$,$γ$)$^{62}$Zn reaction and its astrophysical impact

Cross section measurements of the $^{58}$Ni($α$,$γ$)$^{62}$Zn reaction were performed in the energy range $E_α=5.5-9.5$ MeV at the Nuclear Science Laboratory of the University of Notre Dame, using the NSCL Summing NaI(Tl) detector and the $γ$-summing technique. The measurements are compared to predictions in the statistical Hauser-Feshbach model of nuclear reactions using the SMARAGD code. It is found that the energy dependence of the cross section is reproduced well but the absolute value is overestimated by the prediction. This can be remedied by rescaling the $α$ width by a factor of 0.45. Stellar reactivities were calculated with the rescaled $α$ width and their impact on nucleosynthesis in type Ia supernovae has been studied. It is found that the resulting abundances change by up to 5\% when using the new reactivities.

nucl-ex↗

Classical-Nova Contribution to the Milky Way's $^{26}$Al Abundance: Exit Channel of the Key $^{25}$Al($p,γ$)$^{26}$Si Resonance

Classical novae are expected to contribute to the 1809-keV Galactic $γ$-ray emission by producing its precursor $^{26}$Al, but the yield depends on the thermonuclear rate of the unmeasured $^{25}$Al($p,γ$)$^{26}$Si reaction. Using the $β$ decay of $^{26}$P to populate the key $J^π=3^+$ resonance in this reaction, we report the first evidence for the observation of its exit channel via a $1741.6 \pm 0.6 (\textrm{stat}) \pm 0.3 (\textrm{syst})$ keV primary $γ$ ray, where the uncertainties are statistical and systematic, respectively. By combining the measured $γ$-ray energy and intensity with other experimental data on $^{26}$Si, we find the center-of-mass energy and strength of the resonance to be $E_r = 414.9 \pm 0.6(\textrm{stat}) \pm 0.3 (\textrm{syst}) \pm 0.6(\textrm{lit.})$ keV and $ωγ= 23 \pm 6 (\textrm{stat})^{+11}_{-10}(\textrm{lit.})$ meV, respectively, where the last uncertainties are from adopted literature data. We use hydrodynamic nova simulations to model $^{26}$Al production showing that these measurements effectively eliminate the dominant experimental nuclear-physics uncertainty and we estimate that novae may contribute up to 30% of the Galactic $^{26}$Al.

nucl-ex↗

Characterization of a medium size Xe/TMA TPC instrumented with microbulk Micromegas, using low-energy $γ$-rays

NEXT-MM is a general-purpose high pressure (10 bar, $\sim25$ l active volume) Xenon-based TPC, read out in charge mode with an 8 cm $\times$8 cm-segmented 700 cm$^2$ plane (1152 ch) of the latest microbulk-Micromegas technology. It has been recently commissioned at University of Zaragoza as part of the R&D of the NEXT $0νββ$ experiment, although the experiment's first stage is currently being built based on a SiPM/PMT-readout concept relying on electroluminescence. Around 2 million events were collected during the last months, stemming from the low energy $γ$-rays emitted by a $^{241}$Am source when interacting with the Xenon gas ($ε$ = 26, 30, 59.5 keV). The localized nature of such events above atmospheric pressure, the long drift times, as well as the possibility to determine their production time from the associated $α$ particle in coincidence, allow the extraction of primordial properties of the TPC filling gas, namely the drift velocity, diffusion and attachment coefficients. In this work we focus on the little explored combination of Xe and trimethylamine (TMA) for which, in particular, such properties are largely unknown. This gas mixture offers potential advantages over pure Xenon when aimed at Rare Event Searches, mainly due to its Penning characteristics, wave-length shifting properties and reduced diffusion, and it is being actively investigated by our collaboration. The chamber is currently operated at 2.7 bar, as an intermediate step towards the envisaged 10 bar. We report here its performance as well as a first implementation of the calibration procedures that have allowed the extension of the previously reported energy resolution to the whole readout plane (10.6%FWHM@30keV).

physics.ins-det↗

Measurement of the $^{90, 92}$Zr(p,$γ$)$^{91,93}$Nb reactions for the nucleosynthesis of elements around A=90

Cross section measurements of the reactions $^{90, 92}$Zr(p,$γ$)$^{91,93}$Nb were performed using the NSCL SuN detector at the University of Notre Dame. These reactions are part of the nuclear reaction flow for the synthesis of the light p nuclei. For the $^{90}$Zr(p,$γ$)$^{91}$Nb reaction the new measurement resolves the disagreement between previous results. For the $^{92}$Zr(p,$γ$)$^{93}$Nb reaction the present work reports the first measurement of this reaction cross section. Both reaction cross sections are compared to theoretical calculations and a very good agreement with the standard NON-SMOKER model is observed.

nucl-ex↗

Systematic study of (p,γ) reactions on Ni isotopes

A systematic study of the radiative proton capture reaction for all stable nickel isotopes is presented. The results were obtained using 2.0 - 6.0 MeV protons from the 11 MV tandem Van de Graaff accelerator at the University of Notre Dame. The γ-rays were detected by the NSCL SuN detector utilising the γ-summing technique. The results are compared to a compilation of earlier measurements and discrepancies between the previous data are resolved. The experimental results are also compared to the theoretical predictions obtained using the NON-SMOKER and SMARAGD codes. Based on these comparisons an improved set of astrophysical reaction rates is proposed for the (p,γ) reactions on the stable nickel isotopes as well as for the 56Ni(p,γ)57Cu reaction.

nucl-ex↗

Radiopurity control in the NEXT-100 double beta decay experiment: procedures and initial measurements

The Neutrino Experiment with a Xenon TPC (NEXT) is intended to investigate the neutrinoless double beta decay of 136Xe, which requires a severe suppression of potential backgrounds. An extensive screening and material selection process is underway for NEXT since the control of the radiopurity levels of the materials to be used in the experimental set-up is a must for rare event searches. First measurements based on Glow Discharge Mass Spectrometry and gamma-ray spectroscopy using ultra-low background germanium detectors at the Laboratorio Subterráneo de Canfranc (Spain) are described here. Activity results for natural radioactive chains and other common radionuclides are summarized, being the values obtained for some materials like copper and stainless steel very competitive. The implications of these results for the NEXT experiment are also discussed.

physics.ins-det↗

CuBr2-A New Multiferroic Material with High Critical Temperature

A new multiferroic material, CuBr2, is reported for the first time. CuBr2 has not only a high transition temperature (close to liquid nitrogen temperature) but also low dielectric loss and strong magnetoelectric coupling. These findings reveal the importance of anion effects in the search for the high temperature multiferroics materials among these low-dimensional spin systems.

cond-mat.str-el↗

Unconventional dynamical covalency driven superconductivity in Nb doped SrTiO3

Nb doped SrTiO3, the first discovered two-gap superconductor, is shown to be the most unconventional one of the known multiband superconductors, since the smaller of the two superconducting gaps follows a non BCS temperature dependence. Such a behavior stems from two cooperating effects: an extreme anisotropy in the frequency dependent interactions, involving one very soft mode and an almost vanishing interband interaction. In contrast to all other multiband superconductors, the temperature dependence of the superfluid density of Nb doped SrTiO3 is predicted to exhibit an inflection point close to Tc and not close to T=0.

cond-mat.supr-con↗

Odd p isotope 113In: Measurement of alpha-induced reactions

One of the few p nuclei with an odd number of protons is 113In. Reaction cross sections of 113In(alpha,gamma)117Sb and 113In(alpha,n)116Sb have been measured with the activation method at center-of-mass energies between 8.66 and 13.64 MeV, close to the astrophysically relevant energy range. The experiments were carried out at the cyclotron accelerator of ATOMKI. The activities were determined by off-line detection of the decay gamma rays with a HPGe detector. Measured cross sections and astrophysical S factor results are presented and compared with statistical model calculations using three different alpha+nucleus potentials. The comparison indicates that the standard rates used in the majority of network calculations for these reactions were too fast due to the energy dependence of the optical alpha potential at low energy.

nucl-ex↗

Suppression of the stellar enhancement factor and the reaction 85Rb(p,n)85Sr

It is shown that a Coulomb suppression of the stellar enhancement factor occurs in many endothermic reactions at and far from stability. Contrary to common assumptions, reaction measurements for astrophysics with minimal impact of stellar enhancement should be preferably performed for those reactions instead of their reverses, despite of their negative reaction Q-value. As a demonstration, the cross section of the astrophysically relevant 85Rb(p,n)85Sr reaction has been measured by activation between 2.16<=E_{c.m.}<= 3.96 MeV and the astrophysical reaction rates at p-process temperatures for (p,n) as well as (n,p) are directly inferred from the data. Additionally, our results confirm a previously derived modification of a global optical proton potential. The presented arguments are also relevant for other alpha- and proton-induced reactions in the p-, rp-, and nu-p-processes.

astro-ph.SR↗

Identifying the pairing mechanism in Fe-As based superconductors: gaps and isotope effects

The temperature dependencies of the coupled superconducting gaps, observed in Fe-As based superconducting compounds is calculated and a universal temperature scaling observed which is only present if the coupled order parameters both have s-wave symmetry. Predictions for possible isotope effects on the transition temperature are made if phonons are involved in the pairing or polaronic effects are of importance. Comparison to experimental data is given where these are available.

cond-mat.supr-con↗

Superconductivity in Fe and As based compounds: a bridge between MgB2 and cuprates

By interpreting various experimental data for the new high temperature FeAs type superconductors in terms of lattice mediated multi gap superconductivity, it is shown that these systems strongly resemble MgB2, however, with the distinction that local polaronic lattice effects exist. This fact establishes a connection to cuprate high temperature superconductors where polaron formation is essential for the pseudogap phase and the unconventional isotope effects observed there. However, similar to MgB2 and in contrast to cuprates the two superconducting gaps in the Fe-As based materials are isotropic s-wave gaps.

cond-mat.supr-con↗

Laboratory studies of polycyclic aromatic hydrocarbons: the search for interstellar candidates

Polycyclic Aromatic Hydrocarbons (PAHs) are considered as a major constituent of interstellar dust. They have been proposed as the carriers of the Aromatic Infrared Bands (AIBs) observed in emission in the mid-IR. They likely have a significant contribution to various features of the extinction curve such as the 220 nm bump,the far-UV rise and the diffuse interstellar bands. Emission bands are also expected in the far-IR, which are better fingerprints of molecular identity than the AIBs. They will be searched for with the Herschel Space Observatory. Rotational emission is also expected in the mm range for those molecules which carry significant dipole moments. Despite spectroscopic studies in the laboratory, no individual PAH species could be identified. This emphasises the need for an investigation on where interstellar PAHs come from and how they evolve due to environmental conditions: ionisation and dissociation upon UV irradiation, interactions with electrons, gas and dust. There is also evidence for PAH species to contribute to the depletion of heavy atoms from the gas phase, in particular Si and Fe. This paper illustrates how laboratory work can be inspired from observations. In particular there is a need for understanding the chemical properties of PAHs and PAH-related species, including very small grains, in physical conditions that mimic those found in interstellar space. This motivates a joint effort between astrophysicists, physicists and chemists. Such interdisciplinary studies are currently performed, taking advantage of the PIRENEA set-up, a cold ion trap dedicated to astrochemistry.

astro-ph.GA↗

Magnetic Ordering in the Frustrated Heisenberg Chain System Cupric Chloride, CuCl$_2$

We report a detailed examination the magnetic structure of anhydrous cupric chloride CuCl2 carried out by powder neutron diffraction, magnetic susceptibility and specific heat measurements on polycrystalline and single crystal samples as well as an evaluation of the spin exchange interactions by first principles density functional theory (DFT) calculations. Anhydrous CuCl2 shows one dimensional antiferromagnetic behavior and long range antiferromagnetic ordering below a Neel temperature of 23.9 K. Neutron powder and single crystal diffraction reveal that, below 23.9K, CuCl2 undergoes a phase transition into an incommensurate magnetic structure (propagation vector (1,0.2257,0.5) with a spin-spiral propagating along b and the moments confined in the bc crystallographic plane. Our DFT calculations show that the spin-spiral results from competing ferromagnetic nearest neighbor and antiferromagnetic next-nearest neighbor spin-exchange interaction along the spin chains. Implications for possible multiferroic behavior of CuCl2 are discussed.

cond-mat.str-el↗

Spontaneous stoichiometry change in a single crystal of (Ba1-x Kx)Fe2As2 produced by rapid heating method

To prevent the loss of K in growing single crystals of Ba1-x Kx Fe2 As2 we developed a rapid heating Sn-flux method. Large single crystals with the optimal superconducting transition temperature TC about 38K were obtained and their structural, chemical and superconducting properties were investigated. Additionally, the effect of post growth annealing at different temperatures were also examined on these crystals. Scanning electron microscopy microprobe studies on a samples with the composition goal of Ba.25 K.75 Fe2 As2 revealed a sharp separation of two phases with compositions that are suggestive rational ratios of the K and Ba content.

cond-mat.supr-con↗

Investigation of thermal stability of hydrogenated amorphous Si/Ge multilayers

Thermal stability of hydrogenated amorphous Si/Ge multilayers has been investigated by Scanning Electron Microscopy (SEM), Transmission Electron Microscopy (TEM) and Small-Angle X-Ray Diffraction (SAXRD) techniques. Amorphous H-Si/Ge multilayers were prepared by RF sputtering with 1.5 and 6 ml/min H2 flow-rate. It is shown by Elastic Recoil Detection Analysis (ERDA) that the hydrogen concentration increased by increasing H2 flow-rate. Annealing of the samples was carried out at 400 and 450 oC for several hours. It has been observed that samples prepared with 6 ml/min flow-rate at both annealing temperatures underwent significant structural changes: the surface of the samples was visibly roughened, gas bubbles were formed and craters were created. The decay of the periodic structure of Si and Ge layers in these types of multilayers was faster than in non-hydrogenated samples. Samples prepared with 1.5 ml/min flow-rate have similar behaviour at 450 oC, but at 400 oC the decay of the first order SAXRD peaks was slower than in case of the non-hydrogenated multilayers. Qualitatively the observed behaviour can be explained by the fast desorption of the saturated hydrogen, leading to the formation of bubbles and craters at 450 oC, as well as, at 400oC in the sample with lower H-content, by the possible passivation of the dangling bonds resulting in a slowing down of the diffusion intermixing.

cond-mat.mtrl-sci↗